Nanoscale, Год журнала: 2024, Номер 17(1), С. 158 - 186
Опубликована: Окт. 31, 2024
Review of synthesis strategies for circularly polarized luminescence (CPL) inorganic quantum dots, influencing factors, theoretical insight into CPL mechanisms, and future applications/prospects. Images reproduced with permission, details in article.
Язык: Английский
Nature, Год журнала: 2025, Номер 638(8050), С. 418 - 424
Опубликована: Фев. 5, 2025
Язык: Английский
Процитировано
2
Advanced Optical Materials, Год журнала: 2024, Номер 12(19)
Опубликована: Апрель 30, 2024
Abstract Functional materials that exhibit circularly polarized luminescence (CPL) have shown immense potential in applications such as 3D optical displays and advanced information encryption. However, facile efficient regulation of the multiple emission properties chiral systems has remained a challenge due to scarcity suitable complexity systems. Herein, CPL platform is fabricated by helical co‐assembly an aldehyde‐functionalized fluorane dye (Rhodol‐CHO, 6′‐(diethylamino)‐3′‐hydroxy‐3‐oxo‐3H‐spiro[isobenzofuran‐1,9′‐xanthene]‐4′‐carbaldehyde) liquid crystals, which can efficiently combine stimuli‐responsive characteristics high activity. By introducing acid, base, compounds containing primary amino (─NH 2 ) groups, property system be easily modified. The obtained apparent asymmetry, with g lum values reaching 0.54–0.75). Further, these modules are successfully applied multi‐mode encryption, highlighting their practical utility. Therefore, this study presents novel strategy for developing diverse behaviors based on simple‐designed platform, advancing further materials.
Язык: Английский
Процитировано
8
Chinese Chemical Letters, Год журнала: 2024, Номер 35(10), С. 109862 - 109862
Опубликована: Апрель 29, 2024
Язык: Английский
Процитировано
7
Analytical Chemistry, Год журнала: 2024, Номер 96(36), С. 14550 - 14559
Опубликована: Авг. 24, 2024
In this work, we explored the potential of thiol-capped CdZnTe quantum dots (QDs) as an exceptional signal tag for fluorescence aptasensing applications. Employing a one-pot hydrothermal approach, modulated terminal functional groups QDs using l-cysteine (Lcys), 3-mercaptopropionic acid (MPA), and N-acetyl-l-cysteine (NAC) ligands. Our comparative analysis revealed that NAC-capped (NAC-CdZnTe QDs) exhibited superior anti-interference capabilities storage stability across various temperatures, pH levels, durations. Encouraged by these promising results, further optimized use ultrastable NAC-CdZnTe encapsulated in dendritic mesoporous silica nanoparticles (DMSN@QDs) development advanced aptasensor aflatoxin B1 (AFB1) detection. The developed DMSN@QDs tags achieved remarkable amplification approximately 10.2 fold compared to coated (SiO2@QDs) labeled aptasensor. This was able detect AFB1 within wide range 1 pg mL–1 200 ng mL–1, achieving limit detection low 0.41 (S/N = 3). Crucially, specific binding affinity between aptamer target enabled be easily customized targets simply replacing sequence with desired one. QDs, particularly when DMSNs, leads highly sensitive selective aptasensors targets, thereby, paving way advancements diverse
Язык: Английский
Процитировано
7
Nano Research, Год журнала: 2024, Номер unknown
Опубликована: Авг. 1, 2024
Язык: Английский
Процитировано
6
Analytical Chemistry, Год журнала: 2025, Номер 97(5), С. 3161 - 3170
Опубликована: Янв. 31, 2025
The development of sophisticated nanomaterials with synergistically enhanced functionalities and applications has been greatly promoted via the construction Janus nanoparticles controlled compositions. In this work, we described demonstrated formation Au-PbS (NPs) by Au NPs-mediated spontaneous epitaxial nucleation growth. mechanism NPs was investigated in detail. Then, also found that there a strong electronic interaction between PbS quantum dots (QDs) NPs, where electrons were transferred from domain to QDs domain. Moreover, integrated high-brightness tunable second near-infrared (NIR-II) photoluminescence emission surface-enhanced Raman scattering (SERS), which achieved good intraoperative tumor resection. This complementary dual-functional imaging had potential enable more accurate
Язык: Английский
Процитировано
0
Chemical Physics Impact, Год журнала: 2025, Номер unknown, С. 100859 - 100859
Опубликована: Март 1, 2025
Язык: Английский
Процитировано
0
Nanoscale, Год журнала: 2025, Номер unknown
Опубликована: Янв. 1, 2025
The confined synthesis of carbon dots (CDs) in solid matrixes is a promising avenue for developing new afterglow materials.
Язык: Английский
Процитировано
0
Diamond and Related Materials, Год журнала: 2025, Номер unknown, С. 112249 - 112249
Опубликована: Март 1, 2025
Язык: Английский
Процитировано
0
Science Advances, Год журнала: 2025, Номер 11(20)
Опубликована: Май 16, 2025
Printing materials with circularly polarized light (CPL) emission holds promise for flexible stereoscopic displays and multilevel anticounterfeiting solutions. However, a key challenge lies in developing printable CPL that exhibit both high photoluminescence quantum yield (PLQY) luminescence dissymmetry factor ( g lum ) values. In this study, we present the macroscopic controllable production of efficient full-color carbon dot (CDs) photonic paint materials. These materials, consisting heavy metal-free CDs as emitters, liquid crystals host matrices, are produced using helical coassembly strategy. Our systems based on achieve PLQY (more than 80%) values 1.4), figure merit (a performance indicator properties calculated by multiplying glum) 1.12, outperforming other material systems. Furthermore, CDs-CPL is successfully used printing luminous patterns features. This research provides insights into advanced highlighting their broad potential applications.
Язык: Английский
Процитировано
0