Chemical Reviews,
Год журнала:
2024,
Номер
124(22), С. 12738 - 12843
Опубликована: Ноя. 5, 2024
The
quest
to
imbue
machines
with
intelligence
akin
that
of
humans,
through
the
development
adaptable
neuromorphic
devices
and
creation
artificial
neural
systems,
has
long
stood
as
a
pivotal
goal
in
both
scientific
inquiry
industrial
advancement.
Recent
advancements
flexible
electronics
primarily
rely
on
nanomaterials
polymers
owing
their
inherent
uniformity,
superior
mechanical
electrical
capabilities,
versatile
functionalities.
However,
this
field
is
still
its
nascent
stage,
necessitating
continuous
efforts
materials
innovation
device/system
design.
Therefore,
it
imperative
conduct
an
extensive
comprehensive
analysis
summarize
current
progress.
This
review
highlights
applications
neuromorphics,
involving
inorganic
(zero-/one-/two-dimensional,
heterostructure),
carbon-based
such
carbon
nanotubes
(CNTs)
graphene,
polymers.
Additionally,
comparison
summary
structural
compositions,
design
strategies,
key
performance,
significant
these
are
provided.
Furthermore,
challenges
future
directions
pertaining
materials/devices/systems
associated
neuromorphics
also
addressed.
aim
shed
light
rapidly
growing
attract
experts
from
diverse
disciplines
(e.g.,
electronics,
science,
neurobiology),
foster
further
for
accelerated
development.
Chemical Reviews,
Год журнала:
2022,
Номер
122(6), С. 6514 - 6613
Опубликована: Фев. 8, 2022
A
grand
family
of
two-dimensional
(2D)
materials
and
their
heterostructures
have
been
discovered
through
the
extensive
experimental
theoretical
efforts
chemists,
material
scientists,
physicists,
technologists.
These
pioneering
works
contribute
to
realizing
fundamental
platforms
explore
analyze
new
physical/chemical
properties
technological
phenomena
at
micro-nano-pico
scales.
Engineering
2D
van
der
Waals
(vdW)
via
chemical
physical
methods
with
a
suitable
choice
stacking
order,
thickness,
interlayer
interactions
enable
exotic
carrier
dynamics,
showing
potential
in
high-frequency
electronics,
broadband
optoelectronics,
low-power
neuromorphic
computing,
ubiquitous
electronics.
This
comprehensive
review
addresses
recent
advances
terms
representative
materials,
general
fabrication
methods,
characterization
techniques
vital
role
parameters
affecting
quality
heterostructures.
The
main
emphasis
is
on
3D-bulk
(3D)
hybrid
systems
exhibiting
intrinsic
quantum
mechanical
responses
optical,
valley,
topological
states.
Finally,
we
discuss
universality
applications
trends
for
future
electronics
optoelectronics
(FEO)
under
challenges
opportunities
from
physical,
nanotechnological,
synthesis
perspectives.
Angewandte Chemie International Edition,
Год журнала:
2022,
Номер
62(11)
Опубликована: Дек. 22, 2022
Abstract
Polymer
electrolyte
membrane
water
electrolysis
(PEMWE)
has
been
regarded
as
a
promising
technology
for
renewable
hydrogen
production.
However,
acidic
oxygen
evolution
reaction
(OER)
catalysts
with
long‐term
stability
impose
grand
challenge
in
its
large‐scale
industrialization.
In
this
review,
critical
factors
that
may
lead
to
catalyst's
instability
couple
potential
solutions
are
comprehensively
discussed,
including
mechanical
peeling,
substrate
corrosion,
active‐site
over‐oxidation/dissolution,
reconstruction,
oxide
crystal
structure
collapse
through
the
lattice
oxygen‐participated
pathway,
etc.
Last
but
not
least,
personal
prospects
provided
terms
of
rigorous
evaluation
criteria,
situ
/
operando
characterizations,
economic
feasibility
and
practical
electrolyzer
consideration,
highlighting
ternary
relationship
evolution,
industrial‐relevant
activity
serve
roadmap
towards
ultimate
application
PEMWE.
ACS Applied Nano Materials,
Год журнала:
2023,
Номер
6(9), С. 7077 - 7106
Опубликована: Апрель 20, 2023
The
rapid
development
of
population,
industry,
and
urbanization
have
generated
significant
issues
including
energy
consumption
water
contamination.
Advanced
materials
are
needed
to
clean
up
the
surroundings
develop
potential
storage
devices.
Metal
sulfides
(MSs)
nanomaterials
prospective
candidates
for
multidimensional
applications
in
medicine,
biology,
environmental
sciences,
production/utilization
due
their
light
absorption,
optical
characteristics,
high
specific
capacitance,
catalytic/photocatalytic
capability.
Recent
developments
showed
its
use
as
electrode
material
Li,
Na,
K,
Mg
ion
batteries,
solar
cells,
supercapacitors,
electrocatalysts
oxygen/hydrogen
evolution
reaction,
sensors
gases/chemicals,
catalysts/photocatalysts
remediation.
Scalable
techniques
producing
high-quality,
low-cost
metal
sulfides,
heterostructures,
hybrids
realize
these
interesting
fully.
This
review
summarizes
current
achievements
MSs
notably,
manganese
sulfide
(MnS),
iron
(FeS),
cobalt
(CoS),
nickel
(NiS),
copper
(CuS),
zinc
(ZnS),
silver
(AgS),
cadmium
(CdS),
tungsten
sufide
(WS),
tin
(SnS),
lead
(PbS),
molybdenum
disufide
(MOS2)
efficient
physiochemical
biological
production
get
controlled
morphologies,
sizes,
compositions.
Chemical Society Reviews,
Год журнала:
2023,
Номер
52(5), С. 1650 - 1671
Опубликована: Янв. 1, 2023
This
review
focuses
on
the
existing
strategies
and
underlying
mechanisms,
discusses
future
directions
in
epitaxial
substrate
engineering
to
deliver
wafer-scale
2D
materials
for
integrated
electronics
photonics.
Advanced Energy Materials,
Год журнала:
2024,
Номер
14(23)
Опубликована: Апрель 3, 2024
Abstract
Solar
energy
can
be
utilized
in
photocatalysis
technology
to
realize
light‐driven
hydrogen
peroxide
(H
2
O
)
production,
a
green
chemical
synthesis
route.
Designing
high‐performance
photocatalysts
is
critical
achieving
practical
solar
H
production.
During
the
past
decade,
significant
research
progress
made
photocatalytic
materials
for
Particularly
2D
materials‐based
stand
out
due
their
unique
physical
and
properties.
This
review
highlights
intricate
relationship
between
material
innovation
photochemical
It
starts
with
fundamental
principles
of
generation,
focusing
on
crucial
steps
such
as
photon
absorption,
carrier
dynamics,
surface
reactions,
challenges
that
solve
at
each
step.
Then,
various
production
are
introduced
detail.
Engineering
strategies
optimize
performance
discussed
afterward.
Finally,
future
opportunities
designing
outlined.
expected
inspire
engineering
conversion
other
chemicals.
