Advanced Functional Materials,
Год журнала:
2023,
Номер
33(46)
Опубликована: Июль 8, 2023
Abstract
Semiconductor‐based
photoelectrochemical
(PEC)
fuel
cells
offer
a
feasible
solution
for
sustainable
and
environmentally
friendly
energy
production
by
converting
solar
chemical
into
electrical
energy.
However,
the
low
PEC
activities
of
have
hindered
their
practical
application
due
to
rapid
electron‐hole
recombination
slow
interfacial
reaction
kinetics.
To
address
this
issue,
unique
cell
composed
dual
photoelectrodes
utilizing
low‐cost
biomass,
ascorbic
acid,
as
an
organic
is
reported.
Significantly,
integration
bifunctional
iron
single‐atom
catalysts
(Fe
SACs)
photoactive
materials
has
effectively
constructed
bridge
charge
carrier
transfer,
boosting
kinetics
photoelectric
conversion
efficiency.
Notably,
optimal
dual‐photoelectrode
decorated
with
Fe
SACs
exhibits
superior
performance,
delivering
maximum
power
density
82.82
µW
cm
−2
.
Taking
advantage
peroxidase‐like
activity
SACs,
resultant
self‐powered
are
explored
sensitively
detecting
actual
uric
acid
samples.
This
study
provides
promising
avenue
boost
efficiency
sensitive
biosensing.
Chemical Reviews,
Год журнала:
2022,
Номер
122(16), С. 13478 - 13515
Опубликована: Июль 21, 2022
Electrocatalysts
and
photocatalysts
are
key
to
a
sustainable
future,
generating
clean
fuels,
reducing
the
impact
of
global
warming,
providing
solutions
environmental
pollution.
Improved
processes
for
catalyst
design
better
understanding
electro/photocatalytic
essential
improving
effectiveness.
Recent
advances
in
data
science
artificial
intelligence
have
great
potential
accelerate
electrocatalysis
photocatalysis
research,
particularly
rapid
exploration
large
materials
chemistry
spaces
through
machine
learning.
Here
comprehensive
introduction
to,
critical
review
of,
learning
techniques
used
research
provided.
Sources
electro/photocatalyst
current
approaches
representing
these
by
mathematical
features
described,
most
commonly
methods
summarized,
quality
utility
models
evaluated.
Illustrations
how
applied
novel
discovery
elucidate
electrocatalytic
or
photocatalytic
reaction
mechanisms
The
offers
guide
scientists
on
selection
research.
application
catalysis
represents
paradigm
shift
way
advanced,
next-generation
catalysts
will
be
designed
synthesized.
RSC Applied Interfaces,
Год журнала:
2023,
Номер
1(1), С. 43 - 69
Опубликована: Сен. 27, 2023
Semiconductor
heterojunctions
are
pivotal
in
determining
the
overall
photocatalytic
efficiency.
This
review
explores
recent
advances
diverse
heterojunction
types,
charge
transfer
mechanisms
and
materials.
Advanced Materials,
Год журнала:
2024,
Номер
36(24)
Опубликована: Март 4, 2024
Abstract
High‐entropy
(HE)
materials,
celebrated
for
their
extraordinary
chemical
and
physical
properties,
have
garnered
increasing
attention
broad
applications
across
diverse
disciplines.
The
expansive
compositional
range
of
these
materials
allows
nuanced
tuning
properties
innovative
structural
designs.
Recent
advances
been
centered
on
versatile
photothermal
conversion
capabilities,
effective
the
full
solar
spectrum
(300–2500
nm).
HE
effect,
coupled
with
hysteresis
diffusion,
imparts
desirable
thermal
stability.
These
attributes
position
as
a
revolutionary
alternative
to
traditional
signifying
transformative
shift
in
technology.
This
review
delivers
comprehensive
summary
current
state
knowledge
regarding
emphasizing
intricate
relationship
between
compositions,
structures,
light‐absorbing
mechanisms,
optical
properties.
Furthermore,
outlines
notable
contributions
areas,
such
water
evaporation,
personal
management,
thermoelectric
generation,
catalysis,
biomedical
applications.
culminates
presenting
roadmap
that
prospective
directions
future
research
this
burgeoning
field,
also
fruitful
ways
develop
advanced
expand
promising
