Unlocking the Potential of Isopropanol as an Eco-Friendly Eluent for Large-Scale Fractionation of Fulvic Acids via Preparative Reversed-Phase High-Performance Liquid Chromatography and Multidimensional RP-HPLC: Evaluation of Molecular Diversity and Element Composition DOI
Dmitry S. Volkov, Sophia Mikhailovna Byvsheva, Мikhail А. Proskurnin

и другие.

Environmental Science & Technology, Год журнала: 2024, Номер 58(46), С. 20444 - 20456

Опубликована: Ноя. 7, 2024

Humic substances are organic mixtures of extreme complexity, which significantly complicate their analysis by any method. Fractionation into more homogeneous seems to be almost the only way overcome these difficulties. Preparative high-performance liquid chromatography (HPLC) provides amounts required for both further fractionation and studies other methods. For first time, isopropyl alcohol (IPA) is proposed purposes; its advantages shown example groundwater fulvic acids (FA). IPA much safer than conventional solvents elutes most nonpolar compounds that nonelutable methanol acetonitrile. The isolated fractions differ in molecular composition, confirmed ultrahigh-resolution mass spectrometry spectroscopy. Stepwise IPA-gradient HPLC-UV each preparative fraction demonstrates possibilities multidimensional HPLC FA. were studied contents a broad range elements, relationships between trace-element compositions revealed. Our data reveals existence numerous different organometal FA composition; thus, approach can used in-depth study mechanisms element migration environment.

Язык: Английский

Advances in Research and Technology of Hydrothermal Carbonization: Achievements and Future Directions DOI Creative Commons
Giulia Ischia,

Nicole D. Berge,

Sunyoung Bae

и другие.

Agronomy, Год журнала: 2024, Номер 14(5), С. 955 - 955

Опубликована: Май 2, 2024

Hydrothermal carbonization (HTC) has emerged as a pivotal technology in the battle against climate change and fosters circular economies. Operating within unique reaction environment characterized by water solvent moderate temperatures at self-generated pressures, HTC efficiently converts biomass residues into valuable bio-based products. Despite HTC’s potential—from management of challenging wastes to synthesis advanced carbons implementation biorefineries—it encounters hurdles transitioning from academic exploration industrial implementation. Gaps persist, general comprehension intricacies difficulty large-scale integration with wastewater treatments, process water, absence standardized assessment techniques for Addressing these challenges demands collaboration bridge many scientific sectors touched HTC. Thus, this article reviews current state some hot topics considered crucial development: It emphasizes role cornerstone waste biorefineries, highlighting potentialities its development. In particular, it surveys fundamental research aspects, delving pathways, predictive models, analytical techniques, modifications while exploring technological applications challenges, peculiar focus on combined HTC, integration, plant energy efficiency.

Язык: Английский

Процитировано

12

Lime-assisted hydrothermal humification and carbonization of sugar beet pulp: Unveiling the yield, quality, and phytotoxicity of products DOI Creative Commons
Mona Ghaslani, Reza Rezaee, Omid Aboubakri

и другие.

Biofuel Research Journal, Год журнала: 2024, Номер 11(01), С. 2025 - 2039

Опубликована: Март 1, 2024

Hydrothermal carbonization (HTC) solid and liquid products may inhibit seed germination, necessitating post-treatment. The hydrothermal humification (HTH) method addresses this drawback by transforming inhibitory compounds, such as aromatics, into artificial humic acids (AHAs) fulvic (AFAs). This study introduces a novel approach investigating the substitution of commonly used alkaline agent in HTH, KOH, with hydrated lime to develop cost-effective fertilizers from sugar beet pulp, enriching them AHAs. It assesses effects on AHA production soluble organic compounds compared KOH. results indicate that significantly reduces furans (from 560 3.15 mg/kg DM 344 3.86 mg/L process liquid) boosts sugars acids, especially lactic acid 4.70 65.82 g/kg 4.05 22.89 liquid), increasing hydrochar yield (68.8% vs. 27.4% KOH). Despite lower KOH (3.47% 15.50%), lime-treated are abundant calcium magnesium, boasting pH 7. property presents safer more efficient alternative fertilizers. characterization AHAs aligns standard natural substances, while lime-assisted HTH products, applied at level 0.01% w/w, could enhance wheat growth nutrient uptake control group. Importantly, these show no toxicity Daphnia magna, underscoring their potential for sustainable agriculture.

Язык: Английский

Процитировано

9

Efficient extraction and formation mechanism of fulvic acid from lignite: Experimental and DFT studies DOI
Na Li, Hang Ma, Guodong Wang

и другие.

Journal of Environmental Management, Год журнала: 2024, Номер 365, С. 121650 - 121650

Опубликована: Июль 4, 2024

Язык: Английский

Процитировано

3

Unlocking the Potential of Isopropanol as an Eco-Friendly Eluent for Large-Scale Fractionation of Fulvic Acids via Preparative Reversed-Phase High-Performance Liquid Chromatography and Multidimensional RP-HPLC: Evaluation of Molecular Diversity and Element Composition DOI
Dmitry S. Volkov, Sophia Mikhailovna Byvsheva, Мikhail А. Proskurnin

и другие.

Environmental Science & Technology, Год журнала: 2024, Номер 58(46), С. 20444 - 20456

Опубликована: Ноя. 7, 2024

Humic substances are organic mixtures of extreme complexity, which significantly complicate their analysis by any method. Fractionation into more homogeneous seems to be almost the only way overcome these difficulties. Preparative high-performance liquid chromatography (HPLC) provides amounts required for both further fractionation and studies other methods. For first time, isopropyl alcohol (IPA) is proposed purposes; its advantages shown example groundwater fulvic acids (FA). IPA much safer than conventional solvents elutes most nonpolar compounds that nonelutable methanol acetonitrile. The isolated fractions differ in molecular composition, confirmed ultrahigh-resolution mass spectrometry spectroscopy. Stepwise IPA-gradient HPLC-UV each preparative fraction demonstrates possibilities multidimensional HPLC FA. were studied contents a broad range elements, relationships between trace-element compositions revealed. Our data reveals existence numerous different organometal FA composition; thus, approach can used in-depth study mechanisms element migration environment.

Язык: Английский

Процитировано

0