Reviews of Geophysics,
Год журнала:
2023,
Номер
61(4)
Опубликована: Окт. 18, 2023
Abstract
Atmospheric
aerosols
affect
the
Earth's
climate
in
many
ways,
including
acting
as
seeds
on
which
cloud
droplets
form.
Since
a
large
fraction
of
these
particles
is
anthropogenic,
clouds'
microphysical
and
radiative
characteristics
are
influenced
by
human
activity
global
scale
leading
to
important
climatic
effects.
The
respective
change
energy
budget
at
top
atmosphere
defined
effective
forcing
due
aerosol‐cloud
interaction
(ERF
aci
).
It
estimated
that
ERF
offsets
presently
nearly
1/4
greenhouse‐induced
warming,
but
uncertainty
within
factor
two.
A
common
method
calculate
multiplication
susceptibility
effect
changes
anthropogenic
aerosol
concentration.
This
has
be
done
integrating
it
over
all
regimes.
Here
we
review
various
methods
estimation.
Global
measurements
require
satellites'
coverage.
challenge
quantifying
amounts
cloudy
atmospheres
met
with
rapid
development
novel
methodologies
reviewed
here.
can
retrieved
from
space
based
their
optical
properties,
polarization.
concentrations
serve
drop
condensation
nuclei
also
impact
satellite‐retrieved
number
concentrations.
These
observations
critical
for
reducing
calculated
models
(GCMs),
further
required
allow
GCMs
properly
simulate
benefit
observables.
Oxford Open Climate Change,
Год журнала:
2023,
Номер
3(1)
Опубликована: Янв. 1, 2023
Abstract
Improved
knowledge
of
glacial-to-interglacial
global
temperature
change
yields
Charney
(fast-feedback)
equilibrium
climate
sensitivity
1.2
±
0.3°C
(2σ)
per
W/m2,
which
is
4.8°C
1.2°C
for
doubled
CO2.
Consistent
analysis
over
the
full
Cenozoic
era—including
‘slow’
feedbacks
by
ice
sheets
and
trace
gases—supports
this
implies
that
CO2
was
300–350
ppm
in
Pliocene
about
450
at
transition
to
a
nearly
ice-free
planet,
exposing
unrealistic
lethargy
sheet
models.
Equilibrium
warming
today’s
GHG
amount
10°C,
reduced
8°C
human-made
aerosols.
not
‘committed’
warming;
rapid
phaseout
emissions
would
prevent
most
from
occurring.
However,
decline
aerosol
since
2010
should
increase
1970–2010
rate
0.18°C
decade
post-2010
least
0.27°C
decade.
Thus,
under
present
geopolitical
approach
emissions,
will
exceed
1.5°C
2020s
2°C
before
2050.
Impacts
on
people
nature
accelerate
as
increases
hydrologic
(weather)
extremes.
The
enormity
consequences
demands
return
Holocene-level
temperature.
Required
actions
include:
(1)
increasing
price
accompanied
development
abundant,
affordable,
dispatchable
clean
energy,
(2)
East-West
cooperation
way
accommodates
developing
world
needs,
(3)
intervention
with
Earth’s
radiation
imbalance
phase
down
massive
‘geo-transformation’
climate.
Current
political
crises
an
opportunity
reset,
especially
if
young
can
grasp
their
situation.
Atmospheric chemistry and physics,
Год журнала:
2022,
Номер
22(1), С. 641 - 674
Опубликована: Янв. 17, 2022
Aerosol-cloud
interactions
(ACIs)
are
considered
to
be
the
most
uncertain
driver
of
present-day
radiative
forcing
due
human
activities.
The
nonlinearity
cloud-state
changes
aerosol
perturbations
make
it
challenging
attribute
causality
in
observed
relationships
forcing.
Using
correlations
infer
can
when
meteorological
variability
also
drives
both
and
cloud
independently.
Natural
anthropogenic
from
well-defined
sources
provide
"opportunistic
experiments"
(also
known
as
natural
experiments)
investigate
ACI
cases
where
may
more
confidently
inferred.
These
cover
a
wide
range
locations
spatiotemporal
scales,
including
point
such
volcanic
eruptions
or
industrial
sources,
plumes
biomass
burning
forest
fires,
tracks
individual
ships
shipping
corridors.
We
review
different
experimental
conditions
conduct
synthesis
available
satellite
datasets
field
campaigns
place
these
opportunistic
experiments
on
common
footing,
facilitating
new
insights
clearer
understanding
key
uncertainties
Cloud
albedo
strongly
sensitive
background
conditions.
Strong
liquid
water
path
increases
largely
ruled
out
by
averaging
across
experiments.
Opportunistic
have
significantly
improved
process-level
ACI,
but
remains
unclear
how
reliably
found
scaled
global
level,
thus
demonstrating
need
for
deeper
investigation
order
improve
assessments
climate
change.
Communications Earth & Environment,
Год журнала:
2024,
Номер
5(1)
Опубликована: Май 30, 2024
Abstract
Human
activities
affect
the
Earth’s
climate
through
modifying
composition
of
atmosphere,
which
then
creates
radiative
forcing
that
drives
change.
The
warming
effect
anthropogenic
greenhouse
gases
has
been
partially
balanced
by
cooling
aerosols.
In
2020,
fuel
regulations
abruptly
reduced
emission
sulfur
dioxide
from
international
shipping
about
80%
and
created
an
inadvertent
geoengineering
termination
shock
with
global
impact.
Here
we
estimate
regulation
leads
to
a
$$+0.2\pm
0.11$$
+0.2±0.11
Wm
−2
averaged
over
ocean.
amount
could
lead
doubling
(or
more)
rate
in
2020
s
compared
since
1980
strong
spatiotemporal
heterogeneity.
is
consistent
recent
observed
2023
expected
make
anomalously
warm.
equivalent
magnitude
measured
increase
planetary
heat
uptake
2020.
also
hemispheric
contrast,
important
implications
for
precipitation
pattern
changes.
Our
result
suggests
marine
cloud
brightening
may
be
viable
method
temporarily
its
unique
challenges
due
inherent
Marine
cloud
brightening
(MCB)
is
the
deliberate
injection
of
aerosol
particles
into
shallow
marine
clouds
to
increase
their
reflection
solar
radiation
and
reduce
amount
energy
absorbed
by
climate
system.
From
physical
science
perspective,
consensus
a
broad
international
group
scientists
that
viability
MCB
will
ultimately
depend
on
whether
observations
models
can
robustly
assess
scale-up
local-to-global
in
today's
identify
strategies
ensure
an
equitable
geographical
distribution
benefits
risks
associated
with
projected
regional
changes
temperature
precipitation.
To
address
knowledge
gaps
required
societal
implications
MCB,
we
propose
substantial
targeted
program
research-field
laboratory
experiments,
monitoring,
numerical
modeling
across
range
scales.
Nature Geoscience,
Год журнала:
2024,
Номер
17(5), С. 404 - 410
Опубликована: Апрель 11, 2024
Abstract
With
global
warming
currently
standing
at
approximately
+1.2
°C
since
pre-industrial
times,
climate
change
is
a
pressing
issue.
Marine
cloud
brightening
one
proposed
method
to
tackle
through
injecting
aerosols
into
marine
clouds
enhance
their
reflectivity
and
thereby
planetary
albedo.
However,
because
it
unclear
how
influence
clouds,
especially
cover,
both
projections
the
effectiveness
of
remain
uncertain.
Here
we
use
satellite
observations
volcanic
eruptions
in
Hawaii
quantify
aerosol
fingerprint
on
tropical
clouds.
We
observe
large
enhancement
reflected
sunlight,
mainly
due
an
aerosol-induced
increase
cover.
This
observed
strong
negative
forcing
suggests
that
current
level
driven
by
weaker
net
radiative
than
previously
thought,
arising
from
competing
effects
greenhouse
gases
aerosols.
implies
greater
sensitivity
Earth’s
therefore
larger
response
rising
gas
concentrations
reductions
atmospheric
air
quality
measures.
our
findings
also
indicate
mitigation
via
plausible
most
effective
humid
stable
conditions
tropics
where
solar
radiation
strong.
Nature,
Год журнала:
2022,
Номер
610(7930), С. 101 - 106
Опубликована: Окт. 5, 2022
Abstract
Cloud
reflectivity
is
sensitive
to
atmospheric
aerosol
concentrations
because
aerosols
provide
the
condensation
nuclei
on
which
water
condenses
1
.
Increased
due
human
activity
affect
droplet
number
concentration,
liquid
and
cloud
fraction
2
,
but
these
changes
are
subject
large
uncertainties
3
Ship
tracks,
long
lines
of
polluted
clouds
that
visible
in
satellite
images,
one
main
tools
for
quantifying
aerosol–cloud
interactions
4
However,
only
a
small
by
shipping
show
ship
tracks
5,6
Here
we
even
when
no
emissions
change
properties
substantially.
We
develop
new
method
quantify
effect
all
clouds,
showing
increase
more
positive
response
there
tracks.
directly
detect
shipping-induced
property
trade
cumulus
regions
Atlantic,
known
display
almost
Our
results
indicate
previous
studies
were
suffering
from
selection
biases
focusing
imagery.
The
strong
path
find
translates
larger
cooling
climate,
potentially
masking
higher
climate
sensitivity
than
observed
temperature
trends
would
otherwise
suggest.
Atmospheric chemistry and physics,
Год журнала:
2022,
Номер
22(2), С. 861 - 880
Опубликована: Янв. 19, 2022
Abstract.
Quantification
of
the
radiative
adjustment
marine
low
clouds
to
aerosol
perturbations,
regionally
and
globally,
remains
largest
source
uncertainty
in
assessing
current
future
climate.
One
important
steps
towards
quantifying
role
modifying
cloud
properties
is
quantify
susceptibility
albedo
liquid
water
path
(LWP)
perturbations
droplet
number
concentration
(Nd).
We
use
10
years
spaceborne
observations
from
polar-orbiting
Aqua
satellite
Nd
over
northeast
(NE)
Pacific
stratocumulus
(Sc)
region.
Mutual
information
analysis
reveals
a
dominating
control
state
(e.g.,
LWP
Nd)
on
low-cloud
susceptibility,
relative
meteorological
states
that
drive
these
states.
Through
LWP–Nd
space
decomposition
susceptibilities,
we
show
clear
separation
among
regimes
(brightening
or
darkening),
consistent
with
previously
established
mechanisms
through
which
modulates
properties.
These
include
(i)
thin
non-precipitating
(LWP
<
55
g
m−2)
exhibit
brightening
(occurring
37
%
time),
corresponding
Twomey
effect;
(ii)
thicker
clouds,
entrainment-driven
negative
adjustments
manifest
as
darkening
regime
(36
time);
(iii)
another
(22
time)
consisting
mostly
precipitating
precipitation-suppression
positive
adjustments.
Overall,
find
an
annual-mean
regional
potential
20.8±2.68
W
m−2
ln(Nd)−1,
despite
overall
for
stratocumulus,
owing
high
occurrence
Twomey–brightening
regime.
Over
NE
Pacific,
seasonal
covariabilities
factors
related
large-scale
circulation
are
found
play
grouping
conditions
favorable
each
When
considering
covarying
conditions,
our
results
indicate
northeastern
strongest
occur
most
frequently
within
shallow
boundary
layers
cool
ocean
surface
stable
atmosphere
dry
free
troposphere
above.
Clouds
associated
deep
atmospheric
instability
not
strong
warm
enough
produce
frequent
precipitation.
Cloud
warm-rain
suppression
preferably
either
under
unstable
humid
free-tropospheric
co-occur
surface.
Proceedings of the National Academy of Sciences,
Год журнала:
2022,
Номер
119(41)
Опубликована: Окт. 3, 2022
Global
shipping
accounts
for
13%
of
global
emissions
SO
2
,
which,
once
oxidized
to
sulfate
aerosol,
acts
cool
the
planet
both
directly
by
scattering
sunlight
and
indirectly
increasing
albedo
clouds.
This
cooling
due
aerosol
offsets
some
warming
effect
greenhouse
gasses
is
largest
uncertainty
in
determining
change
Earth’s
radiative
balance
human
activity.
Ship
tracks—the
visible
manifestation
indirect
ship
on
clouds
as
quasi-linear
features—have
long
provided
an
opportunity
quantify
these
effects.
However,
they
have
been
arduous
catalog
typically
studied
only
particular
regions
short
periods
time.
Using
a
machine-learning
algorithm
automate
their
detection
we
more
than
1
million
tracks
provide
climatology.
We
use
this
investigate
stringent
fuel
regulations
introduced
International
Maritime
Organization
2020
prevalence
since
then,
while
accounting
disruption
commerce
caused
COVID-19.
find
marked,
but
clearly
nonlinear,
decline
globally:
An
80%
reduction
x
causes
25%
number
detected.
Nature Communications,
Год журнала:
2022,
Номер
13(1)
Опубликована: Авг. 31, 2022
Incomplete
understanding
of
the
sources
secondary
organic
aerosol
(SOA)
leads
to
large
uncertainty
in
both
air
quality
management
and
climate
change
assessment.
Chemical
reactions
occurring
atmospheric
aqueous
phase
represent
an
important
source
SOA
mass,
yet,
effects
anthropogenic
emissions
on
(aqSOA)
are
not
well
constrained.
Here
we
use
compound-specific
dual-carbon
isotopic
fingerprints
(δ13C
Δ14C)
dominant
aqSOA
molecules,
such
as
oxalic
acid,
track
precursor
formation
mechanisms
aqSOA.
Substantial
stable
carbon
isotope
fractionation
molecules
provides
robust
evidence
for
extensive
aqueous-phase
processing.
Contrary
paradigm
that
these
compounds
largely
biogenic,
radiocarbon-based
apportionments
show
fossil
precursors
produced
over
one-half
molecules.
Large
fractions
fossil-derived
contribute
substantially
total
water-soluble
load
hence
impact
projections
radiative
forcing.
Our
findings
reveal
importance
with
quality.