International Journal of Molecular Sciences,
Год журнала:
2021,
Номер
22(24), С. 13463 - 13463
Опубликована: Дек. 15, 2021
The
extension
of
the
pump-probe
approach
known
from
UV/VIS
spectroscopy
to
very
short
wavelengths
together
with
advanced
simulation
techniques
allows
a
detailed
analysis
excited-state
dynamics
in
organic
molecules
or
biomolecular
structures
on
nanosecond
femtosecond
time
level.
Optical
pump
soft
X-ray
probe
is
relatively
new
detect
and
characterize
optically
dark
states
molecules,
exciton
transient
ligand-to-metal
charge
transfer
states.
In
this
paper,
we
describe
two
experimental
setups
for
absorption
based
an
LPP
emitting
picosecond
sub-nanosecond
pulses
photon
energy
range
between
50
1500
eV.
We
apply
these
near-edge
fine
structure
(NEXAFS)
investigations
thin
films
metal-free
porphyrin,
aggregate
forming
carbocyanine
nickel
oxide
molecule.
NEXAFS
have
been
carried
out
at
carbon,
nitrogen
oxygen
K-edge
as
well
Ni
L-edge.
From
time-resolved
measurements
porphyrin
first
insights
into
long-lived
trap
state
are
gained.
Our
findings
discussed
compared
density
functional
theory
calculations.
Optics Express,
Год журнала:
2020,
Номер
28(20), С. 30164 - 30164
Опубликована: Сен. 14, 2020
We
present
an
ultrafast
thin-disk
based
multipass
amplifier
operating
at
a
wavelength
of
1030
nm,
designed
for
atmospheric
research
in
the
framework
Laser
Lightning
Rod
project.
The
CPA
system
delivers
pulse
energy
720
mJ
and
duration
920
fs
repetition
rate
1
kHz.
240
seed
pulses
generated
by
regenerative
are
amplified
to
final
via
four
industrial
laser
heads.
beam
quality
factor
remains
∼
2.1
output.
First
results
on
horizontal
long-range
filament
generation
presented.
Advances in Optics and Photonics,
Год журнала:
2022,
Номер
14(4), С. 652 - 652
Опубликована: Авг. 31, 2022
The
advent
of
chirped-pulse
amplification
in
the
1980s
and
femtosecond
Ti:sapphire
lasers
1990s
enabled
transformative
advances
intense
laser–matter
interaction
physics.
Whereas
most
experiments
have
been
conducted
limited
near-infrared
range
0.8–1
μm,
theories
predict
that
many
physical
phenomena
such
as
high
harmonic
generation
gases
favor
long
laser
wavelengths
terms
extending
high-energy
cutoff.
Significant
progress
has
made
developing
few-cycle,
carrier-envelope
phase-stabilized,
high-peak-power
1.6–2
μm
laid
foundation
for
attosecond
X
ray
sources
water
window.
Even
longer
wavelength
are
becoming
available
suitable
to
study
light
filamentation,
generation,
laser–plasma
relativistic
regime.
Long-wavelength
sub-bandgap
strong-field
excitation
a
wide
solid
materials,
including
semiconductors.
In
limit,
bulk
crystals
also
produce
high-order
harmonics.
this
review,
we
first
introduce
several
important
scaling
laws
physics,
then
describe
recent
breakthroughs
short-
(1.4–3
μm),
mid-
(3–8
long-wave
(8–15
μm)
infrared
technology,
finally
provide
examples
applications
these
novel
lasers.
Some
broadband
ultrafast
will
profound
effects
on
medicine,
environmental
protection,
national
defense,
because
their
cover
absorption
band,
molecular
fingerprint
region,
well
atmospheric
transparent
Light Science & Applications,
Год журнала:
2021,
Номер
10(1)
Опубликована: Фев. 12, 2021
Abstract
Bright,
coherent
soft
X-ray
radiation
is
essential
to
a
variety
of
applications
in
fundamental
research
and
life
sciences.
To
date,
high
photon
flux
this
spectral
region
can
only
be
delivered
by
synchrotrons,
free-electron
lasers
or
high-order
harmonic
generation
sources,
which
are
driven
kHz-class
repetition
rate
with
very
peak
powers.
Here,
we
establish
novel
route
toward
powerful
easy-to-use
SXR
sources
presenting
compact
experiment
nonlinear
pulse
self-compression
the
few-cycle
regime
combined
phase-matched
single,
helium-filled
antiresonant
hollow-core
fibre.
This
enables
first
100
rate,
table-top
source
that
delivers
an
application-relevant
2.8
×
10
6
s
−1
eV
around
300
eV.
The
fibre
integration
temporal
(leading
formation
necessary
strong-field
waveforms)
pressure-controlled
phase
matching
will
allow
compact,
high-repetition-rate
laser
technology,
including
commercially
available
systems,
drive
simple
cost-effective,
high-flux
sources.
Opto-Electronic Advances,
Год журнала:
2022,
Номер
6(3), С. 220046 - 220046
Опубликована: Сен. 30, 2022
The
generation
of
power-
and
wavelength-scalable
few
optical
cycle
pulses
remains
one
the
major
challenges
in
modern
laser
physics.
Over
past
decade,
development
table-top
parametric
chirped
pulse
amplification-based
systems
was
progressing
at
amazing
speed,
demonstrating
excellent
performance
characteristics
terms
duration,
energy,
peak
power
repetition
rate,
which
place
them
front
line
ultrafast
technology.
At
present,
amplifiers
comprise
a
unique
class
light
sources,
currently
amplify
octave-spanning
spectra
produce
carrier-envelope
phase-stable,
with
multi-gigawatt
to
multi-terawatt
powers
multi-watt
average
powers,
carrier
wavelengths
spanning
considerable
range
spectrum.
This
article
gives
an
overview
on
state
art
amplifiers,
addressing
their
relevant
scientific
technological
aspects,
provides
short
outlook
practical
applications
growing
field
science.
Optics Express,
Год журнала:
2022,
Номер
30(8), С. 13009 - 13009
Опубликована: Март 17, 2022
We
present
a
setup
for
generating
broadband
(up
to
1050
cm-1)
and
broadly
tunable
(2.5-15
µm)
mid-infrared
pulses
using
an
Yb-doped
femtosecond
laser
as
the
pump
source.
Our
scheme,
comprising
two
parametric
amplifiers
mixing
stage,
exploits
favorable
group
velocity
matching
conditions
in
GaSe
pumped
at
2
µm
directly
produce
sub-70
fs
throughout
tuning
range
without
any
additional
dispersion
compensation,
while
30-50
pulse
durations
are
achieved
with
simple
compensation
by
propagation
through
thin
bulk
media.
The
generated
have
sub-1%
short-
long-term
energy
noise,
well
stable
spectral
parameters,
delivering
0.5-2
W
average
mid-IR
power.
expect
source
be
useful
various
spectroscopic
applications
mid-IR.
Optics Letters,
Год журнала:
2022,
Номер
47(12), С. 3095 - 3095
Опубликована: Май 26, 2022
High-energy,
ultrafast,
short-wavelength
infrared
laser
sources
with
high
average
power
are
important
tools
for
industrial
and
scientific
applications.
Through
the
coherent
combination
of
four
ultrafast
thulium-doped
rod-type
fiber
amplifiers,
we
demonstrate
a
Tm-doped
chirped
pulse
amplification
system
compressed
energy
1.65
mJ
167
W
output
at
repetition
rate
101
kHz.
The
delivers
85
fs
pulses
peak
15
GW.
Additionally,
presents
long-
short-term
stability.
To
best
our
knowledge,
this
is
highest
short
wavelength
IR,
mJ-class
source
to
date.
This
result
shows
potential
beam
combining
techniques
in
spectral
region
scalability
these
systems.
Laser & Photonics Review,
Год журнала:
2023,
Номер
17(4)
Опубликована: Янв. 31, 2023
Abstract
The
quest
for
ever‐shorter
optical
pulses
has
been
ongoing
over
half
a
century.
Although
few‐cycle
have
generated
nearly
40
years,
pulse
lengths
below
the
single‐cycle
limit
remained
an
elusive
goal
long
time.
For
this
purpose,
waveform
synthesizers,
generating
high‐energy,
high‐average‐power
via
coherent
combination
of
multiple
covering
different
spectral
regions,
recently
developed.
They
allow
unprecedented
control
waveforms,
spanning
extremely
broad
range
from
ultraviolet
to
infrared.
Such
allows
steering
strong‐field
interactions
with
increased
degrees
freedom.
When
driving
high‐harmonic
generation,
tailored
waveforms
can
produce
bright
attosecond
trains
and
even
isolated
tunable
spectra
up
soft
X‐ray
range.
In
paper
recent
progress
on
parametric
hollow‐core
fiber
synthesizers
is
discussed.
Newly
developed
seeding
schemes;
absolute,
relative,
phase
measurement;
techniques
suitable
are
described.
serial
parallel
synthesis
based
Ti:sapphire
Ytterbium
laser
systems
their
latest
applications
in
generation
gaseous
solid
media,
science,
wakefield
acceleration
Photonics,
Год журнала:
2021,
Номер
8(8), С. 290 - 290
Опубликована: Июль 21, 2021
In
the
past
decade,
mid-infrared
(MIR)
few-cycle
lasers
have
attracted
remarkable
research
efforts
for
their
applications
in
strong-field
physics,
MIR
spectroscopy,
and
bio-medical
research.
Here
we
present
a
review
of
pulse
generation
amplification
wavelength
range
spanning
from
2
to
~20
μm.
first
section,
brief
introduction
on
importance
ultrafast
corresponding
methods
is
provided.
second
different
nonlinear
crystals
including
emerging
non-oxide
crystals,
such
as
CdSiP2,
ZnGeP2,
GaSe,
LiGaS2,
BaGa4Se7,
well
new
periodically
poled
OP-GaAs
OP-GaP
are
reviewed.
Subsequently,
third
various
techniques
optical
parametric
amplification,
chirped-pulse
intra-pulse
difference-frequency
with
all
sorts
designs,
pumped
by
miscellaneous
lasers,
output
specifications
terms
energy,
average
power,
width
addition,
high-energy
single-cycle
pulses
ideal
tools
isolated
attosecond
generation,
electron
dynamic
investigation,
tunneling
ionization
harness.
Thus,
fourth
examples
state-of-the-art
work
field
reviewed
discussed.
last
prospects
high-fidelity
molecule
detection,
cold
tissue
ablation
Optical
parametric
chirped
pulse
amplification
(OPCPA)
provides
an
excellent
platform
to
generate
ultrashort
mid-infrared
pulses
in
the
spectral
window
beyond
scope
of
traditional
mode-locked
lasers.
This
technology
has
paved
path
toward
tabletop
coherent
soft
x-ray
(SXR)
sources
recent
years.
Commercial
availability
high-power
Yb:YAG
lasers
as
pump
enabled
OPCPA
high-energy
femtosecond
mid-IR
at
a
high
repetition
rate.
However,
it
is
still
difficult
achieve
above
mJ,
rate
3
μm
with
less
than
100
fs
pulsewidth.
Here,
we
present
10
kHz,
few-cycle
3.1
generating
compressed
1.1
mJ
energy
record
temporal
width
58
and
rms
stability
0.8%.
Our
experimental
results
are
further
compared
two
different
simulation
codes
for
optimization.
To
increase
efficiency,
utilize
pulse-front
tilt
matching
configuration
resulting
80%
more
first
power
stage
expect
up
total
all
three
stages.
These
open
opportunity
access,
particular,
magnetically
dichroic
L-absorption
edges
3d
metals
through
generation
SXRs
via
harmonic
water
(500–900
eV)
laboratory
setup.
prospect
availing
pump-probe
spectroscopy
SXR
studying
electronic
structure
dynamics
numerous
condensed
phase
systems
resonant
transitions
from
core
levels
functionally
relevant
without
having
resort
large-scale
facilities.