Characteristics of NH3–H2 Reducing Pellets DOI Creative Commons
Xiaoping Zhang,

Zihao Fan,

Ao Mi

и другие.

Metals, Год журнала: 2024, Номер 14(12), С. 1314 - 1314

Опубликована: Ноя. 21, 2024

The reduction of hematite with ammonia is a potentially environmentally friendly method ironmaking. Previous studies on pellets typically involved samples weighing only 2.8 g and lacked detailed activation energy analysis for the ammonia-hydrogen co-reduction pellets. Therefore, to further investigate thermodynamics kinetics NH3–H2 pellets, this study uses 50 experiments. By increasing pellet mass, expands scope kinetic research results indicate that nitrogen gas produced from decomposition reduces equilibrium components reducing gas. In temperature range 700–850 °C, formation iron nitride exhibits narrow during hematite. rate using 100% NH3 lower than 50% H2 mixed gas, which is, in turn, slower H2. As increases, effect approaches Among common gas-solid reaction mathematical models, Phase-boundary-controlled model Contracting Cylinder Model selected as most plausible mechanistic function. For energies reactions NH3, H2, are 65.42, 54.37, 29.17 kJ/mol, respectively. has negative Fe2O3. XRD electron microscopy element line scanning show Fe4N formed Fe2O3 NH3. use mixture significantly

Язык: Английский

Study on Hydrogen Reduction Kinetics of Iron Oxide by-Product from Steel Industry DOI
Kameswara Srikar Sista,

Bilal Murtuza Pirjade,

Abhijeet Premkumar Moon

и другие.

Journal of Sustainable Metallurgy, Год журнала: 2025, Номер unknown

Опубликована: Фев. 24, 2025

Язык: Английский

Процитировано

0

Experiments and Simulations on the Low-Temperature Reduction of Iron Ore Oxide Pellets with Hydrogen DOI Creative Commons

Róbert Findorák,

Zuzana Miškovičová,

Jaroslav Legemza

и другие.

Metals, Год журнала: 2025, Номер 15(3), С. 289 - 289

Опубликована: Март 6, 2025

This article examines the low-temperature reducibility of four types iron ore pellets in a pure hydrogen atmosphere, with aim understanding thermodynamic aspects process. The research focuses on optimizing conditions for pellet reduction order to reduce CO2 emissions and improve production efficiency. Experimental tests were conducted at temperatures 600 °C 800 °C, supplemented by simulations predicting equilibrium composition energy requirements. Chemical microstructural analyses revealed that porosity, mineralogical composition, phase distribution homogeneity significantly affect High-quality low SiO2 content demonstrated best ability, while fluxed presence calcium silicate ferrites higher showed lower potential due hard-to-reduce phases such as silicates. results highlight importance controlling process properties enhance minimize environmental impacts. study provides valuable insights application industrial conditions, contributing decarbonization metallurgical industry.

Язык: Английский

Процитировано

0

Anisotropic Porous Iron-Based Nanoparticles through Two-Step Hydrothermal and Hydrogen-Based Reduction: Enhanced Magnetic Performance for Potential Biomedical Applications DOI
Sofia Caspani, Francisco Javier Fernández-Alonso, Sofia Gonçalves

и другие.

ACS Applied Materials & Interfaces, Год журнала: 2025, Номер unknown

Опубликована: Март 7, 2025

Iron-based nanoparticles have emerged as promising candidates for diverse biomedical applications, including cell separation, targeted drug delivery, hyperthermia therapy, and magnetic resonance imaging. This study reports the scalable synthesis of high-magnetization iron-based with controlled anisotropic shapes, achieved via a two-step process. Hematite nanoparticles, featuring nanocube, nanoellipse, nanoneedle morphologies, were synthesized through hydrolysis ferric chloride in presence ammonium dihydrogen phosphate, morphology precisely tuned by adjusting reagent concentrations. These hematite subsequently reduced hydrogen-based direct reduction at 480 °C, yielding iron-magnetite nanocomposites that retained their exhibited significant porosity, an exceptional saturation magnetization 207 emu/g - approximately 150% higher than conventional magnetite nanoparticles. Comprehensive characterization SQUID magnetometry, Mössbauer spectroscopy, Rietveld refinement X-ray diffraction data, XPS surface analysis confirmed formation metallic iron covered shell. Biocompatibility studies demonstrated biocompatibility these across wide concentration range, underscoring suitability applications.

Язык: Английский

Процитировано

0

Eco-Friendly Catalyst Design: Transforming volcanic lava ashes into sustainable synthesis of glycerol carbonate from glycerol in one pot solvent-free route DOI

Isack Kandola,

Thomas Kivevele, Askwar Hilonga

и другие.

Journal of environmental chemical engineering, Год журнала: 2025, Номер unknown, С. 116030 - 116030

Опубликована: Март 1, 2025

Язык: Английский

Процитировано

0

Hydrogen-Induced Transformations in Dolomite: Unlocking Natural Hydrogen Exploration and Subsurface Storage in Carbonates DOI Creative Commons
Krista Davies, Lionel Esteban, Joël Sarout

и другие.

Energy & Fuels, Год журнала: 2025, Номер unknown

Опубликована: Март 21, 2025

Язык: Английский

Процитировано

0

Reduction of Iron Oxide (Alpha-Fe2o3) with a Hydrogen Rich Plasma Produced by an Electron Cyclotron Wave Resonance Source DOI

Marko Sikirić,

Patrick Choquet, Adrian‐Marie Philippe

и другие.

Опубликована: Янв. 1, 2025

Язык: Английский

Процитировано

0

Characteristics of NH3–H2 Reducing Pellets DOI Creative Commons
Xiaoping Zhang,

Zihao Fan,

Ao Mi

и другие.

Metals, Год журнала: 2024, Номер 14(12), С. 1314 - 1314

Опубликована: Ноя. 21, 2024

The reduction of hematite with ammonia is a potentially environmentally friendly method ironmaking. Previous studies on pellets typically involved samples weighing only 2.8 g and lacked detailed activation energy analysis for the ammonia-hydrogen co-reduction pellets. Therefore, to further investigate thermodynamics kinetics NH3–H2 pellets, this study uses 50 experiments. By increasing pellet mass, expands scope kinetic research results indicate that nitrogen gas produced from decomposition reduces equilibrium components reducing gas. In temperature range 700–850 °C, formation iron nitride exhibits narrow during hematite. rate using 100% NH3 lower than 50% H2 mixed gas, which is, in turn, slower H2. As increases, effect approaches Among common gas-solid reaction mathematical models, Phase-boundary-controlled model Contracting Cylinder Model selected as most plausible mechanistic function. For energies reactions NH3, H2, are 65.42, 54.37, 29.17 kJ/mol, respectively. has negative Fe2O3. XRD electron microscopy element line scanning show Fe4N formed Fe2O3 NH3. use mixture significantly

Язык: Английский

Процитировано

3