One-step 3D printing of flexible poly(acrylamide-co-acrylic acid) hydrogels for enhanced mechanical and electrical performance in wearable strain sensors DOI Creative Commons

Phanthanyaphon Tsupphayakorn-Aek,

Nuttapol Risangud, Manunya Okhawilai

и другие.

Scientific Reports, Год журнала: 2025, Номер 15(1)

Опубликована: Апрель 7, 2025

This study explored the synthesis and 3D printing of an electrolytic hydrogel based on polyacrylamide acrylic acid copolymer (poly(AM-co-AA)), using lithium phenyl-2,4,6-trimethylbenzoylphosphinate (LAP) as a photoinitiator, along with N,N'-Methylene bisacrylamide (MBA) sodium alginate (SA) for crosslinking. The matrix, incorporated electrolyte fillers, including chloride (NaCl), calcium dihydrate (CaCl2·2H2O), aluminum trichloride hexahydrate (AlCl3·6H2O), was fabricated via one-step approach printed LCD-3D printer, yielding porous structure remarkable water absorption capacity tailored mechanical properties. Scanning electron microscopy (SEM) analysis NaCl poly(AM-co-AA) revealed highly surface structure, contributing to exceeding 800%. electrical properties this 3D-printed were found be intermediate between those MBA crosslinked SA. exhibited efficient conductivity flexibility, making it well-suited potential use in strain sensors wearable devices, enabling real-time monitoring human activities, such finger bending.

Язык: Английский

Modulation and Mechanisms of Cellulose‐Based Hydrogels for Flexible Sensors DOI Creative Commons
Meng Zhang, Ting Xu, Kun Liu

и другие.

SusMat, Год журнала: 2024, Номер unknown

Опубликована: Ноя. 27, 2024

ABSTRACT Flexible sensors exhibit the properties of excellent shape adaptability and deformation ability, which have been applied for environmental monitoring, medical diagnostics, food safety, smart systems, human–computer interaction. Cellulose‐based hydrogels are ideal materials fabrication flexible due to their unique three‐dimensional structure, renewability, ease processing, biodegradability, modifiability, good mechanical properties. This paper comprehensively reviews recent advances cellulose‐based in construction sensor applications. The characteristics, mechanisms, advantages prepared by physical cross‐linking, chemical cross‐linking respectively analyzed summarized detail. focus then turns research development hydrogel sensors, including sensing (pressure/strain, humidity/temperature, optical sensing), (chromium, copper, mercury ion sensing, toxic gas nitrite biosensing (glucose, antibody, cellular sensing). Additionally, limitations along with key challenges future directions, discussed. It is anticipated that this review will furnish invaluable insight advancement novel green, facilitate integration as a fundamental component multifunctional technologies, thereby expediting design innovative near future.

Язык: Английский

Процитировано

15

Direct Ink Writing of Conductive Hydrogels DOI Creative Commons
Monica Ho, Aline Braz Ramirez,

Negar Akbarnia

и другие.

Advanced Functional Materials, Год журнала: 2025, Номер unknown

Опубликована: Янв. 29, 2025

Abstract Direct ink writing (DIW) is an additive manufacturing technique that has garnered notable interest due to its precise and consistent printing of a wide range materials, such as viscoelastic hydrogels, pastes, complex composites, by adjusting the ink's rheology. This material flexibility combined with ability print at room temperature makes DIW ideal for diverse applications scalable from small industrial levels. In recent years, conductive hydrogels gained significant attention across various fields, ranging biomedical scaffolds flexible electronics. Conductive are category which exhibit conductivity in their wet and/or dry state. Precursors like polymers, metallic nanoparticles, carbon‐based materials can be used induce electronic ionic hydrogels. review presents comprehensive overview demonstrating printability using technique. The fundamentals precursors presented. Following, different pathways reaching optimal hydrogel properties, including mechanical, conductive, rheological, focus on synthesis introduced. Finally, emerging electronics medicine highlighted, anticipated challenges advancement printable discussed.

Язык: Английский

Процитировано

1

Advanced Hydrogel Systems for Local Anesthetic Delivery: Toward Prolonged and Targeted Pain Relief DOI Creative Commons

Jin-Oh Jeong,

Min-Joo Kim,

Seonwook Kim

и другие.

Gels, Год журнала: 2025, Номер 11(2), С. 131 - 131

Опубликована: Фев. 12, 2025

Local anesthetics (LAs) have been indispensable in clinical pain management, yet their limitations, such as short duration of action and systemic toxicity, necessitate improved delivery strategies. Hydrogels, with biocompatibility, tunable properties, ability to modulate drug release, extensively explored platforms for enhancing LA efficacy safety. This narrative review explores the historical development LAs, physicochemical applications, providing a foundation understanding integration hydrogels anesthetic delivery. Advances thermoresponsive, stimuli-responsive, multifunctional demonstrated significant potential prolonging analgesia reducing exposure preclinical studies, while early findings highlight feasibility thermoresponsive hydrogel formulations. Despite these advancements, challenges burst mechanical instability, regulatory considerations remain critical barriers translation. Emerging innovations, including nanocomposite hydrogels, biofunctionalized matrices, smart materials, offer solutions limitations. Future research should focus on optimizing formulations, expanding validation, integrating advanced fabrication technologies 3D printing artificial intelligence-driven design enhance personalized management. By bridging materials science pharmacology, this provides comprehensive perspective current trends future directions hydrogel-based systems.

Язык: Английский

Процитировано

0

Development of Hydrogels Fabricated via Stereolithography for Bioengineering Applications DOI Open Access
Young Jin Jeon, Minji Kim, Kwang Hoon Song

и другие.

Polymers, Год журнала: 2025, Номер 17(6), С. 765 - 765

Опубликована: Март 14, 2025

The architectures of hydrogels fabricated with stereolithography (SLA) 3D printing systems have played various roles in bioengineering applications. Typically, the SLA successively illuminated light to a layer photo-crosslinkable hydrogel precursors for fabrication hydrogels. These can be classified into point-scanning types and digital micromirror device (DMD) types. form layers by scanning focused light, while DMD illuminate 2D patterns each at once. Overall, were cost-effective allowed good shape fidelity uniform mechanical properties. As result, constructs used regenerate tissues develop lab-on-a-chip devices native tissue-like models.

Язык: Английский

Процитировано

0

One-step 3D printing of flexible poly(acrylamide-co-acrylic acid) hydrogels for enhanced mechanical and electrical performance in wearable strain sensors DOI Creative Commons

Phanthanyaphon Tsupphayakorn-Aek,

Nuttapol Risangud, Manunya Okhawilai

и другие.

Scientific Reports, Год журнала: 2025, Номер 15(1)

Опубликована: Апрель 7, 2025

This study explored the synthesis and 3D printing of an electrolytic hydrogel based on polyacrylamide acrylic acid copolymer (poly(AM-co-AA)), using lithium phenyl-2,4,6-trimethylbenzoylphosphinate (LAP) as a photoinitiator, along with N,N'-Methylene bisacrylamide (MBA) sodium alginate (SA) for crosslinking. The matrix, incorporated electrolyte fillers, including chloride (NaCl), calcium dihydrate (CaCl2·2H2O), aluminum trichloride hexahydrate (AlCl3·6H2O), was fabricated via one-step approach printed LCD-3D printer, yielding porous structure remarkable water absorption capacity tailored mechanical properties. Scanning electron microscopy (SEM) analysis NaCl poly(AM-co-AA) revealed highly surface structure, contributing to exceeding 800%. electrical properties this 3D-printed were found be intermediate between those MBA crosslinked SA. exhibited efficient conductivity flexibility, making it well-suited potential use in strain sensors wearable devices, enabling real-time monitoring human activities, such finger bending.

Язык: Английский

Процитировано

0