Biomass Conversion and Biorefinery, Год журнала: 2024, Номер unknown
Опубликована: Ноя. 15, 2024
Язык: Английский
Biomass Conversion and Biorefinery, Год журнала: 2024, Номер unknown
Опубликована: Ноя. 15, 2024
Язык: Английский
Angewandte Chemie International Edition, Год журнала: 2025, Номер unknown
Опубликована: Март 11, 2025
Abstract Upcycling carbon dioxide (CO 2 ) into long‐chain compounds has attracted considerable attention with respect to mitigating environmental problems and obtaining value‐added feedstocks, but remains a great challenge. Herein, we report tandem photocatalysis‐biosynthesis strategy for efficient CO reduction energy‐rich sucrose or α‐farnesene. Firstly, photocatalytic of CH 4 was optimized over the transitional metal doped ZnO (M−ZnO). The as‐prepared Ni−ZnO preferentially reduces production rate 1539.1 μmol g −1 h selectivity 90 %, owing unique interface structure (Zn δ + −O−Ni β ). Subsequently, Methylomicrobium buryatense 5GB1C genetically engineered produce α‐farnesene using photocatalytically‐obtained as sole source, titer 96.3 43.9 mg L , respectively. This study provides green, low‐energy pathway synthesis from which sheds new light on tackling long‐term energy demands sustainable upcycling.
Язык: Английский
Процитировано
3Journal of Inorganic and Organometallic Polymers and Materials, Год журнала: 2025, Номер unknown
Опубликована: Янв. 14, 2025
Язык: Английский
Процитировано
1Journal of Water Process Engineering, Год журнала: 2025, Номер 70, С. 107103 - 107103
Опубликована: Фев. 1, 2025
Язык: Английский
Процитировано
0Angewandte Chemie, Год журнала: 2025, Номер unknown
Опубликована: Март 11, 2025
Abstract Upcycling carbon dioxide (CO 2 ) into long‐chain compounds has attracted considerable attention with respect to mitigating environmental problems and obtaining value‐added feedstocks, but remains a great challenge. Herein, we report tandem photocatalysis‐biosynthesis strategy for efficient CO reduction energy‐rich sucrose or α‐farnesene. Firstly, photocatalytic of CH 4 was optimized over the transitional metal doped ZnO (M−ZnO). The as‐prepared Ni−ZnO preferentially reduces production rate 1539.1 μmol g −1 h selectivity 90 %, owing unique interface structure (Zn δ + −O−Ni β ). Subsequently, Methylomicrobium buryatense 5GB1C genetically engineered produce α‐farnesene using photocatalytically‐obtained as sole source, titer 96.3 43.9 mg L , respectively. This study provides green, low‐energy pathway synthesis from which sheds new light on tackling long‐term energy demands sustainable upcycling.
Язык: Английский
Процитировано
0Chemical Research in Chinese Universities, Год журнала: 2025, Номер unknown
Опубликована: Апрель 12, 2025
Язык: Английский
Процитировано
0Environmental Science and Pollution Research, Год журнала: 2024, Номер unknown
Опубликована: Сен. 19, 2024
Язык: Английский
Процитировано
2Advanced Energy Materials, Год журнала: 2024, Номер unknown
Опубликована: Дек. 30, 2024
Abstract Photocatalytic carbon dioxide reduction reaction (CO 2 RR) is widely recognized as an attractive technology for simultaneously addressing environmental issues and energy crises. CO RR encompasses three primary processes: electron‐hole generation, separation, surface catalysis. Consequently, the light absorption capacity, charge separation ability, selectivity of catalytic site photocatalyst significantly influence rate RR. The significant role strain engineering in photocatalytic to solar fuel using semiconductor catalysts reviewed this paper. Specifically, design strategies crucial on are examined. In paper, mechanisms strain‐enhanced absorption, photoelectron‐hole product reviewed, along with most recent advancements field. This review offers valuable information photocatalysts supplements various photocatalysts.
Язык: Английский
Процитировано
1Water Air & Soil Pollution, Год журнала: 2024, Номер 235(11)
Опубликована: Сен. 26, 2024
Язык: Английский
Процитировано
0Biomass Conversion and Biorefinery, Год журнала: 2024, Номер unknown
Опубликована: Ноя. 15, 2024
Язык: Английский
Процитировано
0