Inhibitors of dihydroorotate dehydrogenase synergize with the broad antiviral activity of 4′-fluorouridine DOI Creative Commons

Leon Schrell,

Hannah L Fuchs,

Antje Dickmanns

и другие.

bioRxiv (Cold Spring Harbor Laboratory), Год журнала: 2024, Номер unknown

Опубликована: Окт. 6, 2024

ABSTRACT RNA viruses present a constant threat to human health, often with limited options for vaccination or therapy. Notable examples include influenza and coronaviruses, which have pandemic potential. Filo- henipaviruses cause more outbreaks, but high case fatality rates. All rely on the activity of virus-encoded RNA-dependent polymerase (RdRp). An antiviral nucleoside analogue, 4′-Fluorouridine (4′-FlU), targets RdRp diminishes replication several viruses, including A virus SARS-CoV-2, through incorporation into nascent viral delayed chain termination. However, effective concentration 4′-FlU varied among different raising need fortify its efficacy. Here we show that inhibitors dihydroorotate dehydrogenase (DHODH), an enzyme essential pyrimidine biosynthesis, can synergistically enhance effect against henipaviruses, Ebola virus. Even 4′-FlU-resistant mutant was re-sensitized towards by DHODH inhibition. The addition uridine rescued replication, strongly suggesting depletion as mechanism this synergy. also highly SARS-CoV-2 in hamster model COVID. We propose impairment endogenous synthesis inhibition enhances RNAs. This strategy may be broadly applicable efficacy analogues Graphical Abstract HIGHLIGHTS Strong synergy Activity combination previously resistant Broadly active diverse set Successful pathogenic Nipah

Язык: Английский

Randomized controlled trial of molnupiravir SARS-CoV-2 viral and antibody response in at-risk adult outpatients DOI Creative Commons
Joseph F. Standing, Laura Buggiotti, José Afonso Guerra‐Assunção

и другие.

Nature Communications, Год журнала: 2024, Номер 15(1)

Опубликована: Фев. 23, 2024

Abstract Viral clearance, antibody response and the mutagenic effect of molnupiravir has not been elucidated in at-risk populations. Non-hospitalised participants within 5 days SARS-CoV-2 symptoms randomised to receive (n = 253) or Usual Care 324) were recruited study viral dynamics on whole genome sequence from 1437 genomes. Molnupiravir accelerates load decline, but virus is detectable by Day most cases. At 14 (9 post-treatment), associated with significantly higher persistence lower anti-SARS-CoV-2 spike titres compared Care. Serial sequencing reveals increased mutagenesis treatment. Persistence RNA at group transition mutations following treatment cessation. viability similar both groups post-molnupiravir treated samples cultured up 9 post cessation The current 5-day course too short. Longer courses should be tested reduce risk potentially transmissible molnupiravir-mutated variants being generated. Trial registration: ISRCTN30448031

Язык: Английский

Процитировано

21

COVID-19 therapeutics DOI
Daniele Focosi, Massimo Franchini, Fabrizio Maggi

и другие.

Clinical Microbiology Reviews, Год журнала: 2024, Номер 37(2)

Опубликована: Май 21, 2024

SUMMARYSince the emergence of COVID-19 in 2020, an unprecedented range therapeutic options has been studied and deployed. Healthcare providers have multiple treatment approaches to choose from, but efficacy those often remains controversial or compromised by viral evolution. Uncertainties still persist regarding best therapies for high-risk patients, drug pipeline is suffering fatigue shortage funding. In this article, we review antiviral activity, mechanism action, pharmacokinetics, safety therapies. Additionally, summarize evidence from randomized controlled trials on various antivirals discuss unmet needs which should be addressed.

Язык: Английский

Процитировано

12

Nanobodies to multiple spike variants and inhalation of nanobody-containing aerosols neutralize SARS-CoV-2 in cell culture and hamsters DOI Creative Commons
Metin Aksu, Priya Kumar, Thomas Güttler

и другие.

Antiviral Research, Год журнала: 2023, Номер 221, С. 105778 - 105778

Опубликована: Дек. 7, 2023

The ongoing threat of COVID-19 has highlighted the need for effective prophylaxis and convenient therapies, especially outpatient settings. We have previously developed highly potent single-domain (VHH) antibodies, also known as nanobodies, that target Receptor Binding Domain (RBD) SARS-CoV-2 Spike protein neutralize Wuhan strain virus. In this study, we present a new generation anti-RBD nanobodies with superior properties. primary representative group, Re32D03, neutralizes Alpha to Delta well Omicron BA.2.75; other members neutralize, in addition, BA.1, BA.2, BA.4/5, XBB.1. Crystal structures RBD-nanobody complexes reveal how ACE2-binding is blocked explain nanobodies' tolerance immune escape mutations. Through cryo-EM structure Ma16B06-BA.1 complex, demonstrated single nanobody molecule can trimeric spike. describe method large-scale production these Pichia pastoris, formulating them into aerosols. Exposing hamsters aerosols, before or even 24 h after infection SARS-CoV-2, significantly reduced virus load, weight loss pathogenicity. These results show potential aerosolized therapy coronavirus infections.

Язык: Английский

Процитировано

12

Potential of traditional medicines in alleviating COVID-19 symptoms DOI Creative Commons
Moragot Chatatikun, Hiroko P. Indo,

Motoki Imai

и другие.

Frontiers in Pharmacology, Год журнала: 2024, Номер 15

Опубликована: Сен. 26, 2024

This review discusses the prevention and treatment of coronavirus disease 2019 (COVID-19) caused by infection with severe acute respiratory syndrome 2 (SARS-CoV-2). Mutations in its spike glycoprotein have driven emergence variants high transmissibility immune escape capabilities. Some antiviral drugs are ineffective against BA.2 subvariant at authorized dose. Recently, 150 natural metabolites been identified as potential candidates for development new anti-COVID-19 higher efficacy lower toxicity than those existing therapeutic agents. Botanical drug-derived bioactive molecules shown promise dampening COVID-19 cytokine storm thus preventing pulmonary fibrosis, they exert a strong binding affinity viral proteins inhibit their activity. The Health Ministry Thailand has approved Andrographis paniculata (Jap. Senshinren) extracts to treat COVID-19. In China, over 85% patients infected SARS-CoV-2 receive treatments based on traditional Chinese medicine. A comprehensive map stages pathogenetic mechanisms related effective products prevent presented. Approximately 10% affected long COVID, impairs mitochondrial DNA. As number agents is limited, adjuvant botanical drug including vitamin C E supplementation may reduce symptoms progression COVID.

Язык: Английский

Процитировано

3

Inhibitors of dihydroorotate dehydrogenase synergize with the broad antiviral activity of 4′-fluorouridine DOI Creative Commons

Leon Schrell,

Hannah L Fuchs,

Antje Dickmanns

и другие.

Antiviral Research, Год журнала: 2024, Номер 233, С. 106046 - 106046

Опубликована: Дек. 3, 2024

RNA viruses present a constant threat to human health, often with limited options for vaccination or therapy. Notable examples include influenza and coronaviruses, which have pandemic potential. Filo- henipaviruses cause more outbreaks, but high case fatality rates. All rely on the activity of virus-encoded RNA-dependent polymerase (RdRp). An antiviral nucleoside analogue, 4'-Fluorouridine (4'-FlU), targets RdRp diminishes replication several viruses, including A virus SARS-CoV-2, through incorporation into nascent viral delayed chain termination. However, effective concentration 4'-FlU varied among different raising need fortify its efficacy. Here we show that inhibitors dihydroorotate dehydrogenase (DHODH), an enzyme essential pyrimidine biosynthesis, can synergistically enhance effect against henipaviruses, Ebola virus. Even 4'-FlU-resistant mutant was re-sensitized towards by DHODH inhibition. The addition uridine rescued replication, strongly suggesting depletion as mechanism this synergy. also highly SARS-CoV-2 in hamster model COVID. We propose impairment endogenous synthesis inhibition enhances RNAs. This strategy may be broadly applicable efficacy analogues

Язык: Английский

Процитировано

3

The Tautomeric State of N4-Hydroxycytidine within Base-Paired RNA DOI Creative Commons
Irene Bessi, Carina Stiller, Till Schroeder

и другие.

ACS Central Science, Год журнала: 2024, Номер 10(5), С. 1084 - 1093

Опубликована: Апрель 25, 2024

Antiviral nucleoside analogues (e.g., Molnupiravir, Remdesivir) played key roles in the treatment of COVID-19 by targeting SARS-CoV-2 RNA-dependent RNA polymerase (RdRp). The N4-hydroxycytidine (NHC), exists two tautomeric forms that pair either with G or A within RdRp active site, causing an accumulation viral mutations during replication. Detailed insights into states base pairs and structural influence NHC are still missing. In this study, we investigate properties NHC:G NHC:A a self-complementary duplex UV thermal melting NMR spectroscopy using atom-specifically 15N-labeled versions were incorporated oligonucleotides solid-phase synthesis. analysis revealed Watson–Crick via its amino form, whereas equally populated conformations detected for pair: weakly hydrogen-bonded imino form another conformation shifted toward minor groove. Moreover, found variable on neighboring environment. This study provides conclusive experimental evidence existence pairs.

Язык: Английский

Процитировано

2

Efficacy of late-onset antiviral treatment in immunocompromised hosts with persistent SARS-CoV-2 infection DOI

Carolin M. Lieber,

Hae-Ji Kang,

Elizabeth B. Sobolik

и другие.

Journal of Virology, Год журнала: 2024, Номер 98(9)

Опубликована: Авг. 29, 2024

Immunocompromised people are at high risk of prolonged severe acute respiratory syndrome coronavirus 2 (SARS-CoV-2) infection and progression to disease 2019 (COVID-19). However, the efficacy late-onset direct-acting antiviral (DAA) therapy with therapeutics in clinical use experimental drugs mitigate persistent viral replication is unclear. In this study, we employed an immunocompromised mouse model, which supports SARS-CoV-2 explore treatment options. Tandem immuno-depletion CD4

Язык: Английский

Процитировано

2

Identification of antibody-resistant SARS-CoV-2 mutants via N4-Hydroxycytidine mutagenesis DOI Creative Commons
Priya Kumar, Xiaoxiao Zhang,

Rahul Shaha

и другие.

Antiviral Research, Год журнала: 2024, Номер 231, С. 106006 - 106006

Опубликована: Сен. 16, 2024

Язык: Английский

Процитировано

2

Efficacy of late-onset antiviral treatment in immune-compromised hosts with persistent SARS-CoV-2 infection DOI Open Access

Carolin M. Lieber,

Hae-Ji Kang,

Elizabeth B. Sobolik

и другие.

bioRxiv (Cold Spring Harbor Laboratory), Год журнала: 2024, Номер unknown

Опубликована: Май 23, 2024

The immunocompromised are at high risk of prolonged SARS-CoV-2 infection and progression to severe COVID-19. However, efficacy late-onset direct-acting antiviral (DAA) therapy with therapeutics in clinical use experimental drugs mitigate persistent viral replication is unclear. In this study, we employed an mouse model, which supports explore treatment options. Tandem immuno-depletion CD4

Язык: Английский

Процитировано

1

Inhibitors of dihydroorotate dehydrogenase synergize with the broad antiviral activity of 4′-fluorouridine DOI Creative Commons

Leon Schrell,

Hannah L Fuchs,

Antje Dickmanns

и другие.

bioRxiv (Cold Spring Harbor Laboratory), Год журнала: 2024, Номер unknown

Опубликована: Окт. 6, 2024

ABSTRACT RNA viruses present a constant threat to human health, often with limited options for vaccination or therapy. Notable examples include influenza and coronaviruses, which have pandemic potential. Filo- henipaviruses cause more outbreaks, but high case fatality rates. All rely on the activity of virus-encoded RNA-dependent polymerase (RdRp). An antiviral nucleoside analogue, 4′-Fluorouridine (4′-FlU), targets RdRp diminishes replication several viruses, including A virus SARS-CoV-2, through incorporation into nascent viral delayed chain termination. However, effective concentration 4′-FlU varied among different raising need fortify its efficacy. Here we show that inhibitors dihydroorotate dehydrogenase (DHODH), an enzyme essential pyrimidine biosynthesis, can synergistically enhance effect against henipaviruses, Ebola virus. Even 4′-FlU-resistant mutant was re-sensitized towards by DHODH inhibition. The addition uridine rescued replication, strongly suggesting depletion as mechanism this synergy. also highly SARS-CoV-2 in hamster model COVID. We propose impairment endogenous synthesis inhibition enhances RNAs. This strategy may be broadly applicable efficacy analogues Graphical Abstract HIGHLIGHTS Strong synergy Activity combination previously resistant Broadly active diverse set Successful pathogenic Nipah

Язык: Английский

Процитировано

0