Опубликована: Ноя. 15, 2024
Язык: Английский
Опубликована: Ноя. 15, 2024
Язык: Английский
Journal of Energy Storage, Год журнала: 2025, Номер 111, С. 115425 - 115425
Опубликована: Янв. 18, 2025
Язык: Английский
Процитировано
7Coordination Chemistry Reviews, Год журнала: 2024, Номер 517, С. 216039 - 216039
Опубликована: Июнь 21, 2024
Язык: Английский
Процитировано
16Molecules, Год журнала: 2025, Номер 30(3), С. 630 - 630
Опубликована: Янв. 31, 2025
As an energy carrier characterized by its high density and eco-friendliness, hydrogen holds a pivotal position in transition. This paper elaborates on the scientific foundations recent progress of photo- electro-catalytic water splitting, including corresponding mechanism, material design optimization, economy production. It systematically reviews research photo(electro)catalytic materials, oxides, sulfides, nitrides, noble metals, non-noble metal, some novel photocatalysts provides in-depth analysis strategies for optimizing these materials through design, component adjustment, surface modification. In particular, it is pointed out that nanostructure regulation, dimensional engineering, defect introduction, doping, alloying, functionalization can remarkably improve catalyst performance. The importance adjusting reaction conditions, such as pH addition sacrificial agents, to boost catalytic efficiency also discussed, along with comparison cost-effectiveness different production technologies. Despite significant advancements made splitting technology, this highlights challenges faced field, development more efficient stable photo(electro)catalysts, improvement system conversion efficiency, cost reduction, promotion technology industrialization, addressing environmental issues.
Язык: Английский
Процитировано
2Journal of Energy Storage, Год журнала: 2025, Номер 111, С. 115341 - 115341
Опубликована: Янв. 24, 2025
Язык: Английский
Процитировано
1ACS Applied Nano Materials, Год журнала: 2025, Номер unknown
Опубликована: Март 27, 2025
In response to the growing challenges posed by increasingly severe electromagnetic radiation environments and diverse personal thermoregulation requirements, development of wearable devices integrating interference (EMI) shielding thermal management functionalities has become critical for enhancing human comfort safety. Inspired hierarchical structure natural leaves, we present a multifunctional material composed MXene/polyaniline (PANI)/polydopamine (PDA) on flexible activated carbon fabric (ACC) substrate. This is fabricated through facile yet efficient mixed-dimensional assembly strategy, combining two-dimensional (2D) MXene nanosheets with one-dimensional (1D) PANI. The architecture mimics biological ACC serving as robust xylem-like substrate, PANI acting phloem-like supporting layer, forming protective outer layer. amino groups ( (−NH2) function binding sites, facilitating formation hydrogen bonds both PDA MXene, thereby interfacial adhesion mechanical stability. Furthermore, synergistic combination PANI's inherent conductivity MXene's exceptional electrical properties significantly improves overall conductive network fabric. resulting MXene/PANI/PDA@ACC (MPPA) demonstrates outstanding performance, including high (384.6 S/m), superior EMI effectiveness (average 45.81 dB), Joule heating (reaching 94 °C at 5 V), excellent camouflage capabilities (infrared emissivity 0.421). Notably, retains flexibility, durability, breathability, moisture permeability, ensuring even under complex environmental conditions. These combined position MPPA promising candidate next-generation technologies, addressing dual demands protection adaptive management.
Язык: Английский
Процитировано
1Fuel, Год журнала: 2025, Номер 387, С. 134386 - 134386
Опубликована: Янв. 17, 2025
Язык: Английский
Процитировано
1ACS Applied Nano Materials, Год журнала: 2024, Номер unknown
Опубликована: Сен. 18, 2024
Язык: Английский
Процитировано
5ACS Sustainable Chemistry & Engineering, Год журнала: 2024, Номер 12(33), С. 12328 - 12340
Опубликована: Авг. 6, 2024
The significant rise in atmospheric carbon dioxide (CO2) levels has prompted the need to develop efficient methods for CO2 conversion and fixation methods. Electrocarboxylation reaction is a highly sustainable method activating utilizing CO2, yielding essential carboxylic acids their analogues, which are important intermediates pharmaceutical fuel industries. This research demonstrates efficiency of 2D Ti3C2Tx Ta2CTx MXene-modified fiber paper electrodes (Ti3C2Tx/CFP Ta2CTx/CFP) with benzophenone tetrabutylammonium bromide/acetonitrile (TBABr/CH3CN) medium, benzilic acid. Ti3C2Tx/CFP exhibited superior electrocatalytic activity lower reduction potential at −1.0 V achieved 72% yield acid an optimum current density 50 mA cm–2. In comparison, Ta2CTx/CFP cathodic peak −1.08 V, producing 66% 70 electron paramagnetic resonance spectrum substantiates generation reactive radical during reaction. showed robust structural stability ∼88% Faradaic turnover frequency 1.90444 × 10–5 s–1, indicating its fixation.
Язык: Английский
Процитировано
4Journal of Materials Chemistry A, Год журнала: 2024, Номер 12(37), С. 25291 - 25303
Опубликована: Янв. 1, 2024
Oxygen reduction electrocatalysis is studied for three Ti 3 C 2 T x MXenes (T = Cl, Br, NH) having single atom Fe, prepared from a AlC precursor by the Lewis acid molten salt etching method using FeX (X Br), and surface modification with LiNH .
Язык: Английский
Процитировано
3The Chemical Record, Год журнала: 2024, Номер unknown
Опубликована: Сен. 24, 2024
Abstract Green energy storage systems play a vital role in enabling sustainable future by facilitating the efficient integration and utilization of renewable sources. The main problems related to two‐dimensional (2D) materials are their difficult synthesis process, high cost, bulk production, which hamper performance. In recent years, MXenes have emerged as highly promising for enhancing performance devices due unique properties, including surface area, excellent electrical thermal conductivity, exceptional chemical stability. This paper presents comprehensive scientific approach that explores potential empowering green systems. Which indicates novelty article. reviews latest advances MXene techniques. Furthermore, investigates application various technologies, such lithium‐ion batteries, supercapacitors, emerging devices. electrodes flexible transparent is also discussed. Moreover, highlights addressing key challenges storage, capacity, improving cycling stability, promoting fast charging discharging rates. Additionally, industrial cost estimation explored. As output work, we analyzed HF modified acid (LiF HCl) established methods synthesis. Due showing extraordinary results applications. Making composite hydrothermal method one methods. underscores significant contributions advancing systems, paving way driven To facilitate research, this article includes technical recommendations further research gaps topic.
Язык: Английский
Процитировано
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