Bioresource Technology, Год журнала: 2024, Номер 415, С. 131699 - 131699
Опубликована: Окт. 24, 2024
Язык: Английский
Bioresource Technology, Год журнала: 2024, Номер 415, С. 131699 - 131699
Опубликована: Окт. 24, 2024
Язык: Английский
Environmental Science & Technology, Год журнала: 2025, Номер unknown
Опубликована: Май 15, 2025
Molecular oxygen (O2) activation is pivotal in advancing green chemistry and catalysis, addressing processes such as energy conversion environmental remediation. However, the inherent inertness of O2 necessitates highly efficient catalysts. In this study, an electron-rich CuOx@Al2O3 catalyst with high metal loading dispersion was synthesized via ion-exchange inverse-loading method. The novel significantly enhanced due to accelerated Cu0 → Cu+ Cu2+ redox cycle, achieving 85% chlorobenzene removal Fenton-like reaction. This substantially higher than observed conventional CuOx/Al2O3 (45%). Experiments density functional theory (DFT) calculations revealed that Cu-Cu sites over greatly facilitated charge transfer, weakened O-O bonds, promoted synergistic H2O2 produce •OH O2•-, thereby enhancing oxidants utilization efficiency. study provides a sustainable pathway for pollutant degradation by offers valuable insights designing advanced Cu-based catalysts oxidation
Язык: Английский
Процитировано
0Chemical Engineering Journal, Год журнала: 2025, Номер unknown, С. 163872 - 163872
Опубликована: Май 1, 2025
Язык: Английский
Процитировано
0Journal of Water Process Engineering, Год журнала: 2025, Номер 75, С. 107898 - 107898
Опубликована: Май 19, 2025
Язык: Английский
Процитировано
0Separation and Purification Technology, Год журнала: 2024, Номер 355, С. 129649 - 129649
Опубликована: Сен. 11, 2024
Язык: Английский
Процитировано
3Bioresource Technology, Год журнала: 2024, Номер 415, С. 131699 - 131699
Опубликована: Окт. 24, 2024
Язык: Английский
Процитировано
2