Essential protocols for decoding the composition and the functional effects of the nanoparticle protein corona DOI Creative Commons
Massimo Morbidelli, Emanuele Papini, Regina Tavano

и другие.

Frontiers in Nanotechnology, Год журнала: 2024, Номер 6

Опубликована: Окт. 23, 2024

Identifying the function and composition of protein corona (i.e., set host proteins interacting with nanoparticles) is considered a crucial step in development nanoparticles for medical pharmacological applications. Evidence suggests that can alter NP stability, biocompatibility, pharmacokinetics features. Therefore, this review, we provide an updated conceptual, methodological, experimental guideline study corona. We surveyed recent literature (2009–2024) focusing on vitro vivo studies. show several methods, including shot-gun proteomics, identification after in-gel digestion, TMT must be carefully applied integrated to shed light complex phenomenon. Hence, discuss detail relative protocols, highlighting importance conditions, ranging from administration route basic, but determinant, parameters like kind biological fluids, incubation times concentrations. Additionally, propose series protocols involve studying using purified serum or plasma proteins, as well sera depleted specific complement investigate role their deposition nanoparticle surface. also explore how inducing uptake by phagocytic cells examined; finally, methodological approaches effects different coatings Available data indicated it possible characterize punctually differential adsorption onto This allows designing chemical features actively guide formation, thus improving nanotheranostic development.

Язык: Английский

Biological Effects of Micro-/Nano-Plastics in Macrophages DOI Creative Commons
Massimiliano G. Bianchi, Lavinia Casati,

Giulia Sauro

и другие.

Nanomaterials, Год журнала: 2025, Номер 15(5), С. 394 - 394

Опубликована: Март 4, 2025

The environmental impact of plastics is worsened by their inadequate end-of-life disposal, leading to the ubiquitous presence micro- (MPs) and nanosized (NPs) plastic particles. MPs NPs are thus widely present in water air inevitably enter food chain, with inhalation ingestion as main exposure routes for humans. Many recent studies have demonstrated that gain access several body compartments, where they taken up cells, increase production reactive oxygen species, lead inflammatory changes. In most tissues, resident macrophages engage first approach foreign materials, this interaction largely affects subsequent fate material possible pathological outcomes. On other hand, organizers controllers both responses tissue repair. Here, we aim summarize available information on NPs. Particular attention will be devoted consequences macrophage viability functions, well implications pathology.

Язык: Английский

Процитировано

0

Predicting Protein Corona Formation on Polylactic Acid Microplastics Pre- and Post-Photoaging: The Importance of Optimal Imputation Methods DOI

Xuri Wu,

Liping Huang, Lina Zhou

и другие.

Environmental Science & Technology Letters, Год журнала: 2025, Номер unknown

Опубликована: Март 4, 2025

Micro-nanoplastics (MNPs) enter biological systems, forming a protein corona (PC) by adsorbing proteins from bodily fluids, influencing their effects. Mass spectrometry-based proteomics characterizes PC composition, and recent advances have leveraged amino acid sequence-derived features to predict formation using supervised random forest (RF) classifier. However, mass spectrometry often generates substantial missing values (MVs), which may hinder the model's predictive performance understanding of protein–particle interactions. This study assessed impact 20 imputation methods on RF classifier in predicting human plasma polylactic (PLA) photoaged PLA microplastics (MPs), considering rising ecological health concerns. The results showed that five left-censored (Zero, Half-min, Min, QRILC, GSimp) achieved best performance, with high accuracy (0.80–0.82), AUC (0.78–0.84), precision (0.78–0.80), recall (0.97–0.98). Protein spatial features, including secondary sheet structure (negative) absolute solvent-accessible area (positive), were identified as key factors adsorption onto MPs. Additionally, UV aging increased importance ranking frac_aa_S fraction_exposed_exposed_S, highlighting altered protein–MPs interactions, likely through hydrogen bonding electrostatic forces. demonstrates potential enhancing for formation.

Язык: Английский

Процитировано

0

A Review of Eco-Corona Formation on Micro/Nanoplastics and Its Effects on Stability, Bioavailability, and Toxicity DOI Open Access

Haohan Yang,

Zhuoyu Chen,

Linghui Kong

и другие.

Water, Год журнала: 2025, Номер 17(8), С. 1124 - 1124

Опубликована: Апрель 10, 2025

Micro/nanoplastics (M/NPs) have become prevalent in aquatic environments due to their widespread applications. Likewise, ubiquitous ecological macromolecules can adsorb onto M/NPs form an “eco-corona”, which significantly alters environmental behaviors including aggregation dynamics, adsorption/desorption, and bioavailability. Therefore, it is necessary analyze the role of eco-corona assessing risks M/NPs. This review systematically summarizes formation mechanisms evaluates its regulatory effects on stability ecotoxicity Compared with other (e.g., natural organic matter extracellular polymeric substances), humic acid (HA) tightly binds through electrostatic hydrophobic interactions, affecting hetero-aggregation behavior colloidal stability. In terms bioavailability, various functional groups HA surface regulate charge hydrophobicity M/NPs, thereby bioaccumulation “Trojan horse” effect. Notably, corona alleviates M/NPs-induced growth inhibition oxidative stress. Genotoxicity assessment further showed that expression genes related stress response detoxification pathways. Future studies should focus synergistic between co-existing pollutants complex elucidate long-term associated formation.

Язык: Английский

Процитировано

0

Essential protocols for decoding the composition and the functional effects of the nanoparticle protein corona DOI Creative Commons
Massimo Morbidelli, Emanuele Papini, Regina Tavano

и другие.

Frontiers in Nanotechnology, Год журнала: 2024, Номер 6

Опубликована: Окт. 23, 2024

Identifying the function and composition of protein corona (i.e., set host proteins interacting with nanoparticles) is considered a crucial step in development nanoparticles for medical pharmacological applications. Evidence suggests that can alter NP stability, biocompatibility, pharmacokinetics features. Therefore, this review, we provide an updated conceptual, methodological, experimental guideline study corona. We surveyed recent literature (2009–2024) focusing on vitro vivo studies. show several methods, including shot-gun proteomics, identification after in-gel digestion, TMT must be carefully applied integrated to shed light complex phenomenon. Hence, discuss detail relative protocols, highlighting importance conditions, ranging from administration route basic, but determinant, parameters like kind biological fluids, incubation times concentrations. Additionally, propose series protocols involve studying using purified serum or plasma proteins, as well sera depleted specific complement investigate role their deposition nanoparticle surface. also explore how inducing uptake by phagocytic cells examined; finally, methodological approaches effects different coatings Available data indicated it possible characterize punctually differential adsorption onto This allows designing chemical features actively guide formation, thus improving nanotheranostic development.

Язык: Английский

Процитировано

1