Conductivity optimisation of graphene oxide-M13 bacteriophage nanocomposites: towards graphene-based gas micronano-sensors DOI Creative Commons
Kate Stokes, Yiwei Sun,

Jarrod L Thomas

и другие.

Discover Nano, Год журнала: 2024, Номер 19(1)

Опубликована: Сен. 18, 2024

Abstract Graphene oxide (GO) and M13 bacteriophage can self-assemble to form ultra-low density porous structures, known as GraPhage13 aerogels (GPA). Due the insulating nature of GPA challenges in producing highly conductive aerogels, it is paramount explore ways enhance conductivity GPA. Herein, we have developed a method GPA, via integration optimisation 5 nm 20 diameter gold nanoparticles (AuNPs) into aerogel structure systematically analysed morphology, composition spectroscopic properties resulting GPA-Au nanocomposite. The fabricated nanocomposites exhibited remarkable increases conductivity, with AuNPs leading 53-fold increase compared achieving performance up 360 nS/cm, which within range suitable for miniaturised semiconductor devices. mechanism behind enhancement was further investigated attributed GO-AuNP interactions increasing carrier by introducing new energy levels GO band gap or shifting its Fermi level towards conduction band. These findings demonstrate potential functionalised significantly improve electrical paving way their application gas sensors biological chemical detection advanced

Язык: Английский

Removal of Pb2+from Aqueous Media by Solidago canadensis L.-Derived and Crab Shell-Derived Biochar: Adsorption Behavior and Optimization of Adsorption Conditions DOI

Shuyu Ye,

Xinyu Jiang,

Yirong Yang

и другие.

Water Air & Soil Pollution, Год журнала: 2025, Номер 236(2)

Опубликована: Янв. 7, 2025

Язык: Английский

Процитировано

1

Fabrication of 3D Graphene-Silk Elastic Aerogels for Sustainable and Efficient Removal of Organic Dyes from an Aqueous Medium DOI

Aniqa Jadoon,

Weiqi Xiao,

Yu Gao

и другие.

Langmuir, Год журнала: 2025, Номер unknown

Опубликована: Фев. 14, 2025

Water pollution by dyes is a serious environmental issue of modern society that needs to be addressed effectively. Herein, promising adsorbent, i.e., 3D composite aerogel, was developed using reduced graphene oxide and silk fibroin (rGO-SF) via hydrothermal freeze-drying techniques. The efficiency the prepared aerogel toward methylene blue (MB) dye adsorption explored in batch experiments. A study revealed capacity rGO-SF120 as 249.89 mg/g dye. also selectively adsorbs MB over other dyes, such rhodamine B (RhB) orange (MO). process mainly chemical (as data fitted well both pseudo-second-order Elovich kinetic models) followed Langmuir model, indicating it formed single layer on its surface. Overall, an effective potential candidate for treating dye-loaded water with high efficiency.

Язык: Английский

Процитировано

1

Comprehensive insights into the application of graphene-based aerogels for metals removal from aqueous media: Surface chemistry, mechanisms, and key features DOI Creative Commons
Abdelnasser Abidli, Zeineb Ben Rejeb, Aniss Zaoui

и другие.

Advances in Colloid and Interface Science, Год журнала: 2024, Номер 335, С. 103338 - 103338

Опубликована: Ноя. 14, 2024

Efficient removal of heavy metals and other toxic metal pollutants from wastewater is essential to protect human health the surrounding vulnerable ecosystems. Therefore, significant efforts have been invested in developing practical sustainable tools address this issue, including high-performance adsorbents. In respect, within last few years, graphene-based aerogels/xerogels/cryogels (GBAs) emerged drawn attention as excellent materials for removing recovering harmful valuable different aqueous media. Such an upward trend mainly due features aerogel combined with properties graphene derivatives aerogel's network, GBAs' unique three-dimensional (3D) porous structure, high porosity, low density, large specific surface area, exceptional electron mobility, adjustable rich chemistry, remarkable mechanical features, tremendous stability. This review offers a comprehensive analysis fundamental aspects phenomena related application GBAs removal. Herein, we cover all types (bottom-up) synthesized GBAs, true microporous aerogels well 3D open-cell interconnected mesoporous macroporous aerogels, foams, sponges. Indeed, provide insights into understanding suitability such important by revealing mechanisms involved factors inducing controlling highly selective behavior these distinctive Besides conventional adsorptive pathways, critically analyzed ability electrochemically capture (i.e., electrosorption) their efficiency detoxification through reductive adsorption-reduction-readsorption). We also covered reusability aspect (GAs)-based adsorbents, which strongly linked outstanding stability efficient desorption captured metals. Furthermore, view numerous environmental benefits, development magnetically recoverable GAs highlighted. Moreover, shed light on potential scalable implementation evaluating performance continuous processes while highlighting versatility demonstrated remove multiple contaminants along Finally, provides readers accessible overview critical discussion major recent achievements regarding applications GAs-based adsorbents ions Along our recommendations suggestions future work new research directions opportunities, aims serve resource researchers field treatment inspire further progress towards next-generation expanding application.

Язык: Английский

Процитировано

7

Recent advances in the environmental application of graphene-based composites DOI

Rongbo Hou,

Weiyu Zhu,

Yanxue Yue

и другие.

Environmental Science Nano, Год журнала: 2024, Номер 11(6), С. 2302 - 2323

Опубликована: Янв. 1, 2024

Graphene-based composites have been widely applied in environmental remediation owing to their high removal capacity.

Язык: Английский

Процитировано

4

Advances in cellulose/graphene oxide-based polymer composites as a versatile platform for the diminution of water toxicants DOI

Komal Komal,

Shikha Awasthi

Journal of Molecular Liquids, Год журнала: 2025, Номер unknown, С. 127261 - 127261

Опубликована: Фев. 1, 2025

Язык: Английский

Процитировано

0

A versatile alginate aerogel with spatially separated sorption sites for simultaneously and collaboratively scavenging Pb(II) and tetracycline in wastewater: Insight into behavior and mechanisms in the mixture system DOI
Bo Chen, Yuning Chen, Yi-Cheng Chen

и другие.

International Journal of Biological Macromolecules, Год журнала: 2025, Номер unknown, С. 141839 - 141839

Опубликована: Март 1, 2025

Язык: Английский

Процитировано

0

Highly Efficient Adsorption of Cr(VI) by Mechanically Enhanced Chitosan Oligosaccharide Aerogel with Hierarchical Porosity DOI
Dandan Liu, Hui Zhang, Jinfeng Mei

и другие.

Langmuir, Год журнала: 2025, Номер unknown

Опубликована: Март 24, 2025

A three-dimensional porous aerogel was synthesized by combining soft chitosan oligosaccharide to hard multi-walled carbon nanotubes (MWCNTs) under mild conditions. Owing the support of MWCNTs, mesopores can be detected on inner surfaces aerogel. The cross-linking tetraethylenepentamine forms a macropore structure after freeze drying, using water as template. hydrogel bear 30% recoverable compression with aid hydrogen bonds between amide groups. exhibits excellent adsorption capabilities for Cr(VI) in water. capacity reach 367.6 mg/g within 100 min. Notably, demonstrated an extremely high efficiency removal trace Cr(VI). Soluble 1 mg/L completely removed at dosage 0.2 g/L. This work provides new strategy synthesize adsorbents hierarchical pores that exhibit porosity and fast mass transfer rate.

Язык: Английский

Процитировано

0

Soybean hull hemicellulose–soybean protein isolate composite aerogel: Adsorption material for remediation of heavy metal-polluted water DOI

Sinian Li,

Ying Duan, Jun Fang

и другие.

International Journal of Biological Macromolecules, Год журнала: 2025, Номер unknown, С. 143298 - 143298

Опубликована: Апрель 1, 2025

Язык: Английский

Процитировано

0

Standalone Highly Efficient Graphene Oxide as an Emerging Visible Light-Driven Photocatalyst and Recyclable Adsorbent for the Sustainable Removal of Organic Pollutants DOI

Sahil Thakur,

Ayush Badoni,

Samriti

и другие.

Langmuir, Год журнала: 2024, Номер 40(35), С. 18486 - 18502

Опубликована: Авг. 22, 2024

Carbon-based nanostructures are promising eco-friendly multifunctional nanomaterials because of their tunable surface and optoelectronic properties for a variety energy environmental applications. The present study focuses on the synthesis graphene oxide (GO) with particular emphasis engineering its optical making it an excellent adsorbent as well visible light-active photocatalyst. It was achieved by modifying improved Hummers method through optimizing parameters involved in oxidation process. This controlled allows systematic tailoring structural, optical, functionality, leading to adsorption photocatalytic sustainable removal organic pollutants water treatment. Several spectroscopic microscopic characterization techniques, such XRD, SEM, Raman, UV-visible, FTIR, TEM, XPS, BET, etc. were employed analyze degree oxidation, chemistry/functionalization, morphological, structural synthesized GO nanostructures. analyses showed functionality active sites better adsorptive band gap from 2.51 2.76 eV exhibiting natural sunlight activity (>99%) pollutant. Various isotherms have been studied capability (

Язык: Английский

Процитировано

3

Conductivity optimisation of graphene oxide-M13 bacteriophage nanocomposites: towards graphene-based gas micronano-sensors DOI Creative Commons
Kate Stokes, Yiwei Sun,

Jarrod L Thomas

и другие.

Discover Nano, Год журнала: 2024, Номер 19(1)

Опубликована: Сен. 18, 2024

Abstract Graphene oxide (GO) and M13 bacteriophage can self-assemble to form ultra-low density porous structures, known as GraPhage13 aerogels (GPA). Due the insulating nature of GPA challenges in producing highly conductive aerogels, it is paramount explore ways enhance conductivity GPA. Herein, we have developed a method GPA, via integration optimisation 5 nm 20 diameter gold nanoparticles (AuNPs) into aerogel structure systematically analysed morphology, composition spectroscopic properties resulting GPA-Au nanocomposite. The fabricated nanocomposites exhibited remarkable increases conductivity, with AuNPs leading 53-fold increase compared achieving performance up 360 nS/cm, which within range suitable for miniaturised semiconductor devices. mechanism behind enhancement was further investigated attributed GO-AuNP interactions increasing carrier by introducing new energy levels GO band gap or shifting its Fermi level towards conduction band. These findings demonstrate potential functionalised significantly improve electrical paving way their application gas sensors biological chemical detection advanced

Язык: Английский

Процитировано

1