Dual Strategy of Ca2+ Influx and Collagen Denaturation to Remodel the Extracellular Matrix and Amplify Sonopiezoelectric Therapy DOI
Chenghao Yu, Desheng Chen, Dingcheng Zhu

и другие.

Advanced Materials, Год журнала: 2025, Номер unknown

Опубликована: Май 30, 2025

Abstract Extracellular matrix (ECM), a core member of tumor microenvironment, is ≈1.5‐fold harder than the surrounding normal tissues. Regulating stiffness ECM can significantly impact physiological activities cells, such as growth, differentiation, and migration. Herein, sonopiezoelectric‐response nanoplatform consisting Cu 3 BiS nanospheres (CBS NSs) constructed for remodeling. Sonopiezoelectric therapy (SPT) chemodynamic (CDT) are conducted using ultrasound (US) near‐infrared irradiation. Under US irradiation, mechanical strain CBS NSs causes piezoelectric polarization promotes redox reaction through energy band bending. The built‐in electric field generated by irradiation amplifies efficiency Fenton‐like substantially enhances reactive oxygen species production. Moreover, property‐mediated electrical signals allow Ca 2+ influx, upregulating levels metalloproteinase (MMP)‐2 MMP‐9. Integrating with generates localized heat, which effectively denature collagen, reduce stiffness, enhance permeability into solid tumors, thus improving SPT effect. combination MMP upregulation collagen degradation maximize benefits remodeling synergistically cancer therapeutic efficacy SPT/CDT. This SPT/CDT synergistic platform an innovative strategy therapy.

Язык: Английский

Nanomaterial-based regulation of redox metabolism for enhancing cancer therapy DOI

Xiaodan Jia,

Yue Wang, Yue Qiao

и другие.

Chemical Society Reviews, Год журнала: 2024, Номер unknown

Опубликована: Янв. 1, 2024

This review provides a comprehensive summary of the dysregulation redox metabolism in cancer cells and advantages latest advances nanomaterial-assisted metabolic regulation therapy.

Язык: Английский

Процитировано

12

Recent advances of piezoelectric materials used in sonodynamic therapy of tumor DOI

Hsin-I Huang,

Yuqing Miao, Yuhao Li

и другие.

Coordination Chemistry Reviews, Год журнала: 2024, Номер 523, С. 216282 - 216282

Опубликована: Окт. 22, 2024

Язык: Английский

Процитировано

10

Ultrasound-Responsive Nanobubbles for Breast Cancer: Synergistic Sonodynamic, Chemotherapy, and Immune Activation through the cGAS-STING Pathway DOI

Huan Pu,

Jia Huang,

Bin Gui

и другие.

ACS Applied Materials & Interfaces, Год журнала: 2025, Номер unknown

Опубликована: Март 24, 2025

Breast cancer remains the leading cause of cancer-related deaths among women worldwide, necessitating more effective treatment strategies. Chemotherapy combined with immunotherapy is first-line for breast cancer, but it still suffers from limited therapeutic efficiency and serious side effects, which are usually due to poor delivery efficiency, drug resistance tumor cells, immunosuppressive microenvironment. This study explores development ultrasound-responsive nanobubbles (Ce6/PTX Nbs) targeted imaging sonoimmunotherapy in treatment. By integrating sonodynamic therapy (SDT), chemotherapy, immunotherapy, aim address challenges such as delivery, systemic toxicity, immune suppression conventional therapies. The nanobubbles, composed sonosensitizer chlorin e6 (Ce6)-modified phospholipid loaded chemotherapeutic agent paclitaxel (PTX) enhancing drug-loading capacity, designed precisely target sites via cyclic-RGD peptides. Upon ultrasound activation, Ce6 induces reactive oxygen species (ROS), promoting immunogenic cell death (ICD), while PTX disrupts mitosis, response. nanobubbles' responsiveness facilitates real-time controlled release, maximizing efficacy minimizing effects. Key findings demonstrate that Ce6/PTX Nbs significantly reduced growth a 4T1 model, enhanced activation cGAS-STING pathway, increased infiltration CD8+ T cells both primary distant tumors. In combination anti-PD-L1 checkpoint inhibitors, achieved substantial metastasis. innovative approach offers highly targeted, effective, minimally toxic potential clinical translation its dual capabilities.

Язык: Английский

Процитировано

2

Ruthenium Single‐Atom Nanozyme Driven Sonosensitizer with Oxygen Vacancies Enhances Electron–Hole Separation Efficacy and Remodels Tumor Microenvironment for Sonodynamic‐Amplified Ferroptosis DOI Creative Commons
Yang Zhu,

Dengliang Wang,

Chengzhong Du

и другие.

Advanced Science, Год журнала: 2025, Номер unknown

Опубликована: Апрель 25, 2025

Abstract Sonodynamic therapy (SDT) has emerged as a promising noninvasive approach for tumor therapy. However, the effectiveness of traditional inorganic semiconductor sonosensitizers is hindered by rapid electron (e − ) and hole (h + recombination under ultrasonic (US) stimulation, well hypoxic reductive conditions microenvironment (TME), which limit generation reactive oxygen species (ROS). Herein, ruthenium (Ru) single‐atom nanozyme‐driven superimposition‐enhanced titanium dioxide‐based sonosensitizer (Ru/TiO 2‐x SAE) presented that features sufficient vacancies high e /h separation efficiency. Through synchrotron radiation‐based X‐ray absorption spectroscopy extended fine structure analysis it confirmed in TiO nanoparticles promote immobilization single‐atomic Ru, forming Ru‐O₄ active sites. Density functional theory calculations demonstrate alter electronic nanosensitizer, enhanced separation, increasing adsorption, accelerating reaction kinetics US ultimately improving ROS production. Moreover, Ru/TiO SAE boosts sonodynamic efficacy mitigating TME. This attributed to its catalase‐ glutathione peroxidase 4‐like activities, facilitate trigger lipid peroxidation‐mediated ferroptosis. These findings highlight innovative role Ru optimizing SDT‐induced ferroptosis, demonstrating potential advancing cancer

Язык: Английский

Процитировано

2

Microcrystalline Bi2WO6 co-modified by oxygen vacancies and bismuth metal deposits for the efficient photocatalytic oxidation of nitric oxide DOI
Long Zeng, Qingyun Tian, Ting Gao

и другие.

Surfaces and Interfaces, Год журнала: 2025, Номер unknown, С. 106262 - 106262

Опубликована: Март 1, 2025

Язык: Английский

Процитировано

1

Dual-engineered strategy of Ni-CeO nanozyme with enhanced oxidase activity for sensitive colorimetric detection of total antioxidant capacity DOI
Chang Xie,

Jiahe Peng,

Jizhou Jiang

и другие.

Talanta, Год журнала: 2025, Номер unknown, С. 128307 - 128307

Опубликована: Май 1, 2025

Язык: Английский

Процитировано

0

Dual Strategy of Ca2+ Influx and Collagen Denaturation to Remodel the Extracellular Matrix and Amplify Sonopiezoelectric Therapy DOI
Chenghao Yu, Desheng Chen, Dingcheng Zhu

и другие.

Advanced Materials, Год журнала: 2025, Номер unknown

Опубликована: Май 30, 2025

Abstract Extracellular matrix (ECM), a core member of tumor microenvironment, is ≈1.5‐fold harder than the surrounding normal tissues. Regulating stiffness ECM can significantly impact physiological activities cells, such as growth, differentiation, and migration. Herein, sonopiezoelectric‐response nanoplatform consisting Cu 3 BiS nanospheres (CBS NSs) constructed for remodeling. Sonopiezoelectric therapy (SPT) chemodynamic (CDT) are conducted using ultrasound (US) near‐infrared irradiation. Under US irradiation, mechanical strain CBS NSs causes piezoelectric polarization promotes redox reaction through energy band bending. The built‐in electric field generated by irradiation amplifies efficiency Fenton‐like substantially enhances reactive oxygen species production. Moreover, property‐mediated electrical signals allow Ca 2+ influx, upregulating levels metalloproteinase (MMP)‐2 MMP‐9. Integrating with generates localized heat, which effectively denature collagen, reduce stiffness, enhance permeability into solid tumors, thus improving SPT effect. combination MMP upregulation collagen degradation maximize benefits remodeling synergistically cancer therapeutic efficacy SPT/CDT. This SPT/CDT synergistic platform an innovative strategy therapy.

Язык: Английский

Процитировано

0