Copper and Iron Make the Difference: Developing Sustainable Photoredox Catalyzed Transformations DOI
Oliver Reiser

Опубликована: Июль 22, 2024

Synthetic organic chemistry undertakes significant efforts to develop new catalytic transformations that utilize greener reagents and avoid stoichiometric additives. In this regard, visible-light photoredox catalysis offers a unique activation mode of molecules, which serves as an alternative many thermal transition-metals catalyzed reactions. Most photoredox-catalyzed processes capitalize on heavy metals, namely, Ru(II) or Ir(III)-complexes, can serve single electron oxidants reductants in their photoexcited states. Copper-and iron-based photo¬catalysts are rapidly emerging, offering economic ecologic advantages but, addition, interact with substrates beyond transfer via inner sphere mechanisms, have been successfully utilized achieve challenging transformations. Emphasizing the principles catalysis, selected synthetic applications from our laboratory will be discussed, highlighting opportunities copper- iron-photocatalysts offer area.

Язык: Английский

An overview on copper in industrial chemistry: From ancient pigment to modern catalysis DOI
Mohammad Soleiman‐Beigi, Masoud Mohammadi,

Homa Kohzadi

и другие.

Coordination Chemistry Reviews, Год журнала: 2025, Номер 529, С. 216438 - 216438

Опубликована: Янв. 17, 2025

Язык: Английский

Процитировано

2

Towards a more Sustainable Photocatalysis using Copper and Iron DOI Creative Commons
Youssef Abderrazak, Oliver Reiser

Current Opinion in Green and Sustainable Chemistry, Год журнала: 2025, Номер unknown, С. 100998 - 100998

Опубликована: Янв. 1, 2025

Язык: Английский

Процитировано

1

Observation of Solvent Enantio-Isotope Effect in Asymmetric Ring-Opening of Cyclic Diaryliodoniums with Selenocyanate DOI Creative Commons
Yuanyuan Li,

Chunlin Tao,

Longhui Duan

и другие.

Chemical Science, Год журнала: 2025, Номер unknown

Опубликована: Янв. 1, 2025

The deuterium isotope effect of D 2 O enhanced the enantioselectivity in an aqueous emulsion reaction, enabling Cu/PyBox-catalyzed highly chemo- and enantioselective ring-opening cyclic diaryliodoniums with KSeCN.

Язык: Английский

Процитировано

0

Efficient and regioselective C=S bond difunctionalization through a three-component radical relay strategy DOI
Shanshan Li, Juan Luo,

S. K. Liang

и другие.

Chinese Chemical Letters, Год журнала: 2024, Номер unknown, С. 110424 - 110424

Опубликована: Сен. 1, 2024

Язык: Английский

Процитировано

2

Visible Light-Induced Copper-Catalyzed Regio- and Stereoselective Difluoroalkylthiocyanation of Alkynes DOI

Xiaoxue Hu,

Yanzhao Wang, Shibo Xu

и другие.

The Journal of Organic Chemistry, Год журнала: 2024, Номер 89(12), С. 9118 - 9124

Опубликована: Июнь 6, 2024

The first regio- and stereoselective difluoroalkylthiocyanation of alkynes with BrCF

Язык: Английский

Процитировано

1

Electrophotocatalytic Thiocyanation and Sulfonylation Cyclization of Unactivated Alkenes DOI
Yingchun Ma,

Ping Yu,

Ruoyu Qin

и другие.

The Journal of Organic Chemistry, Год журнала: 2024, Номер unknown

Опубликована: Дек. 18, 2024

We report an electrophotocatalytic process that enables the thiocyanation and sulfonylation/cyclization of alkenes. It is applicable to a wide range unactivated alkenes, using inexpensive photocatalyst 2,4,6-triphenylpyrylium tetrafluoroborate (TPPT) produce diverse array heterocycles containing sulfonyl thiocyano groups with good functional group tolerance. The protocol operates under mild, chemical oxidant- transition-metal-free, broad scope substrates. Preliminary mechanistic studies suggest reaction involves combination electrolysis reductive quenching photocatalytic cycle TPPT.

Язык: Английский

Процитировано

1

Copper and Iron Make the Difference: Developing Sustainable Photoredox Catalyzed Transformations DOI
Oliver Reiser

Опубликована: Июль 22, 2024

Synthetic organic chemistry undertakes significant efforts to develop new catalytic transformations that utilize greener reagents and avoid stoichiometric additives. In this regard, visible-light photoredox catalysis offers a unique activation mode of molecules, which serves as an alternative many thermal transition-metals catalyzed reactions. Most photoredox-catalyzed processes capitalize on heavy metals, namely, Ru(II) or Ir(III)-complexes, can serve single electron oxidants reductants in their photoexcited states. Copper-and iron-based photo¬catalysts are rapidly emerging, offering economic ecologic advantages but, addition, interact with substrates beyond transfer via inner sphere mechanisms, have been successfully utilized achieve challenging transformations. Emphasizing the principles catalysis, selected synthetic applications from our laboratory will be discussed, highlighting opportunities copper- iron-photocatalysts offer area.

Язык: Английский

Процитировано

0