Tibetan
Plateau
(TP,
hereafter),
known
as
“Third
Pole”,
is
surrounded
by
the
highly
polluted
regions,
such
Indo-Gangetic
Plain,
Taklimakan
and
Gobi
Deserts
Sichuan
Basin.
However,
previous
in-situ
aerosol
measurements
mainly
focused
on
southern
northern
slopes,
while
less
observations
studies
were
conducted
at
eastern
slope
of
TP
(ESTP).
The
scientific
knowledge
optical
properties
aerosols
extremely
limited
over
ESTP,
varying
altitudes
from
heavily
regions
to
relatively
clean
important
for
better
understanding
light
absorption
radiative
forcing
TP.
Basin
(SCB),
a
region
due
more
rapid
economic
development,
located
in
east
side
Therefore,
we
first
field
experiment
six
sites
(Chengdu,
Sanbacun,
Wenchuan,
Lixian,
Maerkang,
Hongyuan)
along
extending
elevation
500
m
3500
m.
Light-absorbing
are
considered
be
key
climate
driver,
their
role
may
underestimated
high-altitude
regions.
brown
carbon
(BrC)
accounting
that
total
increases
20
%
50
%,
mass
efficiency
BrC
2–3
times
higher
than
inside
SCB,
especially
winter,
which
related
high
ratio
secondary
primary
organic
stronger
formation
emissions
altitudes.
Contrary
aerosols,
EC
(elemental
carbon)
declines
with
altitude
induced
source
difference
between
SCB.
urban
sources
(motor
vehicles,
industries,
etc.)
SCB
fail
transported
stable
air
basin
also
favorable
aging
enhance
efficiency.
relative
varies
0.10
0.42
OC
/
thus
enhanced
pristine
because
concentration
decreases
slowly
does
EC.
South
Asia,
particulate
matter
(PM)
pollution
region,
an
origin
particles
western
Plateau,
significantly
dependent
seasons.
npj Climate and Atmospheric Science,
Год журнала:
2024,
Номер
7(1)
Опубликована: Март 23, 2024
Abstract
As
a
precursor
process
to
cloud
formation,
aerosol
activation
over
the
Tibetan
Plateau
(TP)
plays
pivotal
role
in
regional
cloud-precipitation
and
global
climate.
However,
its
characteristics
remain
unclear
due
absence
of
targeted
observations
TP.
We
conducted
ground
in-situ
aerosol-cloud-precipitation
experiment
southern
TP
(GACPE-STP),
thereby
unveiling
this
crucial
region.
Our
findings
reveal
weak
capacity
with
low
hygroscopicity
(
κ
)
values
less
than
0.1
through
multi-method
measurements,
contrasting
starkly
widely
recommended
value
0.3
for
continental
regions.
A
parameterization
is
developed
predicting
region,
which
can
significantly
reduce
overestimations
droplet
number
concentration
hence
indirect
effects
caused
by
using
0.3.
These
address
contributing
enhancement
precipitation
climate
simulations.
Geophysical Research Letters,
Год журнала:
2023,
Номер
50(5)
Опубликована: Фев. 28, 2023
Abstract
Diverse
urban‐induced
rainfall
anomalies
across
different
cities
highlight
the
need
for
additional
insights
into
land‐atmosphere
interactions
over
complex
urban
environments.
Based
on
empirical
analyses
of
144
warm‐season
storms
and
high‐resolution
numerical
simulations
Nanjing,
China,
we
show
divergent
patterns
with
contrasting
synoptic
conditions,
despite
enhancement
downtown
from
a
climatological
perspective.
We
propose
two
simple
gage‐based
metrics
to
characterize
both
thermal
turbulent
conditions
in
pre‐storm
environment,
classify
groups.
Our
results
that
elevated
magnitudes
heavy
frequency
are
equally
expected
either
or
suburb
regions
(upwind
downwind).
This
is
mainly
dictated
by
relative
dominance
perturbations
mechanical
turbulence
(i.e.,
related
surface
roughness)
under
conditions.
develop
four
paradigms
modification,
thus
provide
predictive
understanding
Environmental Science & Technology,
Год журнала:
2024,
Номер
58(2), С. 1244 - 1254
Опубликована: Янв. 5, 2024
Carbonaceous
aerosols
(CA)
from
anthropogenic
emissions
have
been
significantly
reduced
in
urban
China
recent
years.
However,
the
relative
contributions
of
fossil
and
nonfossil
sources
to
CA
rural
background
regions
remain
unclear.
In
this
study,
different
carbonaceous
fractions
fine
(PM2.5)
five
sites
Meteorological
Administration
Atmosphere
Watch
Network
during
winter
2019
2020
were
quantified
using
radiocarbon
(14C)
organic
markers.
The
results
showed
that
contributed
44–69%
total
carbon
at
these
sites.
Fossil
fuel
combustion
was
predominant
source
elemental
all
(73
±
12%).
Nonfossil
dominated
(OC)
(61
13%),
with
biomass
burning
or
biogenic-derived
secondary
(SOC)
as
most
important
contributors.
OC
(39
13%)
still
exceeds
those
other
regional/background
Asia,
Europe,
USA.
SOC
fuel-derived
OC,
highlighting
impact
regional
transport
on
aerosol
levels.
It
is
therefore
imperative
develop
implement
reduction
policies
technologies
tailored
both
biogenic
mitigate
environmental
health
risks
pollution
across
China.
Geophysical Research Letters,
Год журнала:
2024,
Номер
51(3)
Опубликована: Янв. 30, 2024
Abstract
Accurate
quantification
of
the
absorption
properties
brown
carbon
(BrC)
aerosols
is
crucial
to
assess
Earth‐atmosphere
radiative
impacts
BrC.
However,
BrC
were
often
misestimated
in
field
observations,
due
neglecting
contribution
dust
absorption.
This
study
solved
this
problem
by
coupling
a
method
for
calculating
concentration
into
traditional
model
quantifying
The
results
show
that
was
up
16.8%
sum
and
northwestern
China.
potential
significantly
higher
Asia‐located
studies
(0.4%–16.8%)
than
Americas‐located
(<1.2%)
Europe‐located
(<2.3%)
studies.
work
underscores
necessity
eliminating
negative
effect
quantitative
model.
It
prompts
us
revisit
resolved
previous
studies,
especially
dust‐influenced
areas
such
as
Asia.
Atmospheric chemistry and physics,
Год журнала:
2022,
Номер
22(22), С. 14693 - 14708
Опубликована: Ноя. 18, 2022
Abstract.
Scientific
knowledge
about
light
absorption
by
aerosols
is
extremely
limited
at
the
eastern
slope
of
Tibetan
Plateau
(ESTP).
We
conducted
first
aerosol
field
experiment
six
sites
(Chengdu,
Sanbacun,
Wenchuan,
Lixian,
Maerkang,
Hongyuan)
along
ESTP,
ranging
in
elevation
from
500
to
3500
m.
The
fraction
brown
carbon
(BrC)
total
increases
20
%
50
with
altitude,
and
mass
efficiency
(MAE)
BrC
over
(TP)
2–3
times
higher
than
that
inside
Sichuan
Basin
(SCB),
especially
winter.
In
contrast,
MAE
elemental
(EC)
winter
decreases
altitude.
contrasting
variation
EC
altitude
mainly
attributed
source
differences
between
TP
SCB.
Emissions
more
urban
sources
(motor
vehicles,
industries,
etc.)
SCB
fail
be
transported
due
stable
air
basin,
which
also
favourable
for
ageing
enhance
efficiency.
radiative
forcing
relative
varies
0.10
0.42
as
organic
(OC)
ratio
Thus,
reason
enhanced
polluted
pristine
concentration
slowly
This
study
contributes
understanding
difference
lower-altitude
basins
TP,
provides
a
data
set
regional
climate
model
validation.