Construction and identification of highly active single-atom Fe1-NC catalytic site for electrocatalytic nitrate reduction DOI
Lingyue Liu, Ting Xiao, Heyun Fu

и другие.

Applied Catalysis B Environment and Energy, Год журнала: 2022, Номер 323, С. 122181 - 122181

Опубликована: Ноя. 14, 2022

Язык: Английский

Regulating intermediate adsorption and H2O dissociation on a diatomic catalyst to promote electrocatalytic nitrate reduction to ammonia DOI
Xiaoxue Zhang, Xiaokang Liu, Zhen‐Feng Huang

и другие.

Energy & Environmental Science, Год журнала: 2024, Номер 17(18), С. 6717 - 6727

Опубликована: Янв. 1, 2024

Cu–Fe–N–C demonstrates excellent electrocatalytic activity for nitrate reduction by optimizing intermediate adsorption and generating a substantial supply of H* the thorough hydrogenation N-containing intermediates.

Язык: Английский

Процитировано

22

Recent Progress and Perspectives on Transition Metal-Based Electrocatalysts for Efficient Nitrate Reduction DOI
Jun Zhou,

Sanshuang Gao,

Guangzhi Hu

и другие.

Energy & Fuels, Год журнала: 2024, Номер 38(8), С. 6701 - 6722

Опубликована: Апрель 8, 2024

Electrochemical nitrate reduction is the process of converting into ammonia or nitrogen using electric energy. This saves energy, protects environment, and an important technology for resource recovery water purification. paper examines recent advances in electrochemical research analyzes reaction mechanism path as well influence various factors on through thermodynamic kinetic principles. Second, catalytic performances transition metal electrocatalysts form single metals, alloys, oxides, composites are analyzed detail, which lays foundation rational development new, efficient, stable electrocatalysts. Finally, future directions prospects envisioned.

Язык: Английский

Процитировано

20

Graphene quantum dots as metal-free nanozymes for chemodynamic therapy of cancer DOI Creative Commons
Hongji Liu, Zhiming Deng, Yue‐Biao Zhang

и другие.

Matter, Год журнала: 2024, Номер 7(3), С. 977 - 990

Опубликована: Янв. 10, 2024

Язык: Английский

Процитировано

16

High‐Throughput Screening and General Synthesis Strategy of Single‐Atom Nanozymes for Oral Squamous Cell Carcinoma Therapy DOI Open Access

Ji Shen,

Guan-Meng Zhang,

Zedong Zhang

и другие.

Advanced Materials, Год журнала: 2025, Номер unknown

Опубликована: Янв. 5, 2025

Abstract Single‐atom nanozymes (SAzymes), with their superior enzyme‐like catalytic activity, have emerged as promising candidates for oncology therapeutics. The well‐defined structures of SAzymes make them well predictable by experiences and theoretical calculation. However, the effects metal center species coordination environments on activity are variable, screening artificial experiments is challenging. High‐throughput can rapidly select optimal thus better application in tumor therapy highly desirable. Herein, a “high‐throughput screening‐SAzymes structures” system established efficient drug preparation density functional theory oxidase‐like processes screened differences brought about different metals environments. Through this process, transition (Mn, Fe, Co, Ni) active centers synthesized then tested multi‐enzyme activities. It found that SAzyme Co exhibited best further showed good anti‐oral squamous cell carcinoma properties both vitro vivo. This study opens up new avenue rational design oral cancer combining computational experimental validation.

Язык: Английский

Процитировано

2

Construction and identification of highly active single-atom Fe1-NC catalytic site for electrocatalytic nitrate reduction DOI
Lingyue Liu, Ting Xiao, Heyun Fu

и другие.

Applied Catalysis B Environment and Energy, Год журнала: 2022, Номер 323, С. 122181 - 122181

Опубликована: Ноя. 14, 2022

Язык: Английский

Процитировано

66