Physical review. E,
Год журнала:
2024,
Номер
109(4)
Опубликована: Апрель 29, 2024
Active
materials
possess
unique
properties
of
being
able
to
respond
autonomously
external
stimuli,
yet
realizing
and
regulating
the
motion
behavior
active
machines
remains
a
major
challenge.
Conventional
control
approaches,
including
sensor
device
control,
are
both
complex
difficult
implement.
In
contrast,
materials--based
self-oscillators
offer
distinct
such
as
periodic
ease
regulation.
Inspired
by
paddle
boats,
we
have
proposed
conceptual
light-fueled
self-paddling
boat
with
photothermally
responsive
liquid
crystal
elastomer
(LCE)--based
motor
that
operates
under
steady
illumination
incorporates
an
LCE
fiber.
Based
on
well-established
dynamic
model
rotation
dynamics,
equations
for
governing
LCE-steered
derived,
driving
torque
LCE-based
paddling
velocity
formulated
successively.
The
numerical
results
show
two
modes
illumination:
static
mode
mode.
regime
arises
from
competition
between
frictional
torque.
Moreover,
critical
conditions
required
trigger
quantitatively
examined
well
significant
system
parameters
affecting
torque,
angular
velocity,
velocity.
exhibits
benefits
customizable
size
untethered
ambient
powered,
which
provides
valuable
insights
into
design
application
micromachines,
soft
robotics,
energy
harvesters,
beyond.
Biological
organisms
such
as
the
octopus
can
reconfigure
their
shape
and
properties
to
perform
diverse
tasks.
However,
soft
machines
struggle
achieve
complex
configurations,
morph
into
support
loads,
go
between
multiple
states
reversibly.
Here,
we
introduce
a
multifunctional
shape-morphing
material
with
reversible
rapid
polymorphic
reconfigurability.
We
couple
elastomeric
kirigami
an
unconventional
plasticity
mechanism
in
metal
alloys
rapidly
(
<
0.1
seconds)
flat
sheets
complex,
load-bearing
shapes,
reversibility
self-healing
through
phase
change.
This
composite
overcomes
trade-offs
deformability
capacity
eliminates
power
requirements
sustain
reconfigured
shapes.
demonstrate
this
integration
onboard
control,
motors,
create
robotic
morphing
drone,
which
autonomously
transforms
from
ground
air
vehicle
underwater
machine,
be
reversibly
deployed
collect
cargo.
Nature Nanotechnology,
Год журнала:
2022,
Номер
17(11), С. 1198 - 1205
Опубликована: Окт. 27, 2022
Abstract
Artificial
muscles
are
indispensable
components
for
next-generation
robotics
capable
of
mimicking
sophisticated
movements
living
systems.
However,
an
optimal
combination
actuation
parameters,
including
strain,
stress,
energy
density
and
high
mechanical
strength,
is
required
their
practical
applications.
Here
we
report
mammalian-skeletal-muscle-inspired
single
fibres
bundles
with
large
strong
contractive
actuation.
The
use
exfoliated
graphene
fillers
within
a
uniaxial
liquid
crystalline
matrix
enables
photothermal
work
capacity
rapid
response.
Moreover,
the
reversible
percolation
induced
by
thermodynamic
conformational
transition
mesoscale
structures
can
be
in
situ
monitored
electrical
switching.
Such
dynamic
behaviour
effectively
strengthens
properties
actuator
fibres,
particularly
contracted
state,
enabling
mammalian-muscle-like
reliable
Taking
advantage
mechanically
compliant
fibre
structure,
smart
actuators
readily
integrated
into
as
well
high-power
soft
light-driven
remote
control.
Advanced Functional Materials,
Год журнала:
2022,
Номер
33(4)
Опубликована: Ноя. 11, 2022
Abstract
Direct
ink
writing
of
liquid
crystal
elastomers
(LCEs)
offers
a
new
opportunity
to
program
geometries
for
wide
variety
shape
transformation
modes
toward
applications
such
as
soft
robotics.
So
far,
most
3D‐printed
LCEs
are
thermally
actuated.
Herein,
3D‐printable
photoresponsive
gold
nanorod
(AuNR)/LCE
composite
is
developed,
allowing
photothermal
actuation
the
structures
with
AuNR
low
0.1
wt.%.
It
shown
that
printed
filament
has
superior
response
27%
strain
upon
irradiation
near‐infrared
(NIR)
light
(808
nm)
at
1.4
W
cm
−2
(corresponding
160
°C)
under
optimal
printing
conditions.
The
can
be
globally
or
locally
actuated
into
different
shapes
by
controlling
area
exposed
NIR
laser.
Taking
advantage
customized
enabled
3D
and
ability
control
light,
light‐responsive
robot
demonstrated
climb
on
ratchet
surface
maximum
speed
0.284
mm
s
−1
(on
flat
surface)
0.216
30°
titled
surface),
respectively,
corresponding
0.428
0.324
body
length
per
min,
large
mass
(0.23
g)
thickness
(1
mm).
Advanced Materials,
Год журнала:
2023,
Номер
35(16)
Опубликована: Фев. 22, 2023
Leveraging
liquid
crystal
elastomers
(LCEs)
to
realize
scalable
fabrication
of
high-performing
fibrous
artificial
muscles
is
particular
interest
because
these
active
soft
materials
can
provide
large,
reversible,
programmable
deformations
upon
environmental
stimuli.
High-performing
LCEs
require
the
used
processing
technology
enable
shaping
into
micro-scale
fine
fibers
as
thin
possible
while
achieving
macroscopic
LC
orientation,
which
however
remains
a
daunting
challenge.
Here,
bioinspired
spinning
reported
that
allows
for
continuous,
high-speed
production
(fabrication
speed
up
8400
m
h-1
)
and
aligned
LCE
microfibers
combined
with
rapid
deformation
(actuation
strain
rate
810%
s-1
),
powerful
actuation
stress
5.3
MPa),
high
response
frequency
(50
Hz),
long
cycle
life
(250
000
cycles
without
obvious
fatigue).
Inspired
by
crystalline
spiders
takes
advantage
multiple
drawdowns
align
their
dragline
silks,
internal
drawdown
via
tapered-wall-induced-shearing
external
mechanical
stretching
are
employed
shape
long,
thin,
desirable
performances,
few
technologies
achieve.
This
capable
would
benefit
development
smart
fabrics,
intelligent
wearable
devices,
humanoid
robotics,
other
areas.
Advanced Functional Materials,
Год журнала:
2023,
Номер
34(7)
Опубликована: Ноя. 3, 2023
Abstract
Advanced
sensation
and
actuation
abilities
of
various
living
organisms
in
nature
have
inspired
researchers
to
design
bioinspired
self‐sensing
soft
actuators.
However,
the
majority
conventional
actuators
primarily
possess
capabilities
while
lacking
a
real‐time
sensing
signal
feedback.
Here,
promising
strategy
is
reported
develop
highly
stretchable
conductive
hydrogels
for
actuators,
which
integrate
strain‐sensing
functions
into
single
materials
system.
The
are
designed
fabricated
by
situ
copolymerization
amino‐functionalized
MXene‐encapsulated
liquid
metal
nanodroplets
(LM@A‐MXene)
poly(
N
‐isopropylacrylamide)
with
controllable
activated
nanogels
as
nano‐cross‐linkers.
resulting
hydrogel
presents
compacted
conducting
network
porous
microstructure,
giving
rise
robust
integration
high
conductivity,
excellent
strain
sensitivity,
broad
stretchability,
stability,
fast
response
speed.
Interestingly,
gradient
structure,
formed
self‐precipitation
LM@A‐MXene,
endows
shape‐programmable
actuation,
light‐driven
remote
control,
function.
As
proof‐of‐concept
application,
gripper
based
on
developed,
can
not
only
grasp,
lift,
release
objects,
but
also
perceive
every
movement
state
monitoring
resistance
changes.
proposed
actuator
offer
new
insights
developing
smart
robotics
other
artificial
intelligent
devices.
Robots
typically
interact
with
their
environments
via
feedback
loops
consisting
of
electronic
sensors,
microcontrollers,
and
actuators,
which
can
be
bulky
complex.
Researchers
have
sought
new
strategies
for
achieving
autonomous
sensing
control
in
next-generation
soft
robots.
We
describe
here
an
electronics-free
approach
robots,
whose
compositional
structural
features
embody
the
sensing,
control,
actuation
loop
bodies.
Specifically,
we
design
multiple
modular
units
that
are
regulated
by
responsive
materials
such
as
liquid
crystal
elastomers.
These
modules
enable
robot
to
sense
respond
different
external
stimuli
(light,
heat,
solvents),
causing
changes
robot's
trajectory.
By
combining
types
modules,
complex
responses
achieved,
logical
evaluations
require
events
occur
environment
before
action
is
performed.
This
framework
embodied
offers
a
strategy
toward
robots
operate
uncertain
or
dynamic
environments.
Light Science & Applications,
Год журнала:
2023,
Номер
12(1)
Опубликована: Янв. 4, 2023
Abstract
Active
metasurfaces
are
emerging
as
the
core
of
next-generation
optical
devices
with
their
tunable
responses
and
flat-compact
topography.
Especially
for
terahertz
band,
active
have
been
developed
fascinating
chopping
compressive
sensing
imaging.
However,
performance
regulation
by
changing
dielectric
parameters
integrated
functional
materials
exhibits
severe
limitations
parasitic
losses.
Here,
we
introduce
a
C-shape-split-ring-based
phase
discontinuity
metasurface
liquid
crystal
elastomer
substrate
infrared
modulation
wavefront.
Line-focused
light
is
applied
to
manipulate
deflection
substrate,
enabling
controllable
broadband
wavefront
steering
maximum
output
angle
change
22°
at
0.68
THz.
Heating
another
control
method
also
investigated
compared
control.
We
further
demonstrate
beam
steerer,
frequency
modulator,
splitter,
which
highly
desired
in
wireless
communication
imaging
systems.
The
proposed
scheme
demonstrates
promising
prospects
mechanically
deformable
metasurfaces,
thereby
paving
path
development
reconfigurable
metasurfaces.
Cyborg and Bionic Systems,
Год журнала:
2023,
Номер
4
Опубликована: Янв. 1, 2023
Untethered
microrobots
can
be
used
for
cargo
delivery
(e.g.,
drug
molecules,
stem
cells,
and
genes)
targeting
designated
areas.
However,
it
is
not
enough
to
just
reach
the
lesion
site,
as
some
drugs
only
play
best
therapeutic
effect
within
cells.
To
this
end,
folic
acid
(FA)
was
introduced
into
in
work
a
key
mediate
endocytosis
of
The
here
were
fabricated
with
biodegradable
gelatin
methacryloyl
(GelMA)
modified
magnetic
metal–organic
framework
(MOF).
porous
structure
MOF
hydrogel
network
polymerized
GelMA
loading
FA
anticancer
doxorubicin
(DOX)
respectively.
Utilizing
property
MOF,
these
gather
around
site
navigation
fields.
combination
effects
substantially
improve
efficiency
microrobots.
result
shows
that
cancer
cells
inhibition
rate
up
93%,
while
ones
without
78%.
introduction
useful
method
transportation
ability
microrobots,
providing
meaningful
reference
further
research.
Materials Horizons,
Год журнала:
2023,
Номер
10(7), С. 2587 - 2598
Опубликована: Янв. 1, 2023
Liquid
crystal
elastomer
(LCE)
fibers
exhibit
large
deformation
and
reversibility,
making
them
an
ideal
candidate
for
soft
actuators.
It
is
still
challenging
to
develop
a
scalable
strategy
endow
fiber
actuators
with
photoelectric
functions
achieve
tailorable
photo-electro-thermal
responsiveness
rapid
actuation
deformation.
Herein,
we
fabricated
multiresponsive
actuator
that
consists
of
LCE
long
obtained
by
continuous
dry
spinning
further
coated
it
polydopamine
(PDA)-modified
MXene
ink.
The
designed
PDA@MXene-integrated
used
shape-deformable
multi-trigger
can
be
photo-
electro-thermally
actuated.
proposed
combines
excellent
photothermal
long-term
electrically
conductive
PDA@MXene
shape-morphing
fiber,
enabling
their
robust
mechanical
flexibility,
multiple
fast
responses
(∼0.4
s),
stable
(∼60%).
As
proof-of-concept,
present
near-infrared
light-driven
artificial
muscle
lift
1000
times
the
weight
intelligent
circuit
switch
controllability
(∼0.1
s).
Importantly,
adaptive
smart
window
system
integrates
energy
harvesting/conversion
ingeniously
constructed
integration
propellable
curtain
woven
solar
cells.
This
work
provide
insights
into
development
advanced
materials
toward
robotics,
sustainable
savings
beyond.
Advanced Materials,
Год журнала:
2023,
Номер
35(14)
Опубликована: Янв. 14, 2023
Active
fabrics,
responding
autonomously
to
environmental
changes,
are
the
"Holy
Grail"
of
development
smart
textiles.
Liquid
crystal
elastomers
(LCEs)
promise
be
base
materials
for
large-stroke
reversible
actuation.
The
mechanical
behavior
LCEs
matches
almost
exactly
human
muscle.
Yet,
it
has
not
been
possible
produce
filaments
from
that
will
suitable
standard
textile
production
methods,
such
as
weaving.
Based
on
recent
LCE
fibers,
here,
crafting
active
fabrics
incorporating
yarn,
woven
a
loom,
giving
control
over
weave
density
and
structure,
is
presented.
Two
types
yarns
(soft
stiff)
their
incorporation
into
several
weaving
patterns
tested,
"champions"
identified:
twill
pattern
with
stiffer
yarn
shows
greatest
blocking
force
1-2
N
cm-1
,
weft
rib
10%
actuation
strain
repeated
heating
cycles.
Reversible
3D
shape
changes
fabric
utilize
circular
lead
cone
shapes
upon
heating.
seamless
combination
rich
portfolio
existing
passive
can
transformative
in
creating
new
stimuli-responsive
actuating