Abstract.
PM2.5,
generated
via
both
direct
emission
and
secondary
formation,
can
have
varying
environmental
impacts
due
to
different
physical
chemical
properties
of
its
components.
However,
traditional
methods
quantify
class="inline-formula">2.5
components
are
often
based
on
online
or
offline
observations
numerical
models,
which
generally
high
economic
cost-
labor-intensive.
In
this
study,
we
develop
a
new
method,
named
Multi-Tracer
Estimation
Algorithm
(MTEA),
identify
the
primary
from
routine
observation
class="inline-formula">2.5.
By
comparing
with
long-term
short-term
measurements
aerosol
in
China
United
States,
it
is
proven
that
MTEA
successfully
capture
magnitude
variation
(PPM)
(SPM).
Applying
National
Air
Quality
Network,
find
(1)
SPM
accounted
for
63.5â%
cities
southern
average
during
2014â2018,
while
proportion
dropped
57.1â%
north
China,
at
same
time
regional
background
regions
was
â¼â19â%
higher
than
populous
regions;
(2)
summertime
presented
slight
but
consistent
increasing
trend
(from
58.5â%
59.2â%)
most
cities,
mainly
because
recent
increase
O3
pollution
China;
(3)
Beijing
significantly
increased
by
34â%
COVID-19
lockdown,
might
be
main
reason
observed
unexpected
PM
special
period;
finally,
(4)
showed
similar
positive
correlations
Beijing-Tianjin-Hebei
(BTH)
Yangtze
River
Delta
(YRD)
regions,
between
total
these
two
as
determined
PPM
levels,
were
quite
different.
general,
promising
tool
efficiently
estimating
SPM,
has
huge
potential
future
mitigation.
Atmospheric chemistry and physics,
Год журнала:
2022,
Номер
22(8), С. 5495 - 5514
Опубликована: Апрель 26, 2022
Abstract.
PM2.5,
generated
via
both
direct
emission
and
secondary
formation,
can
have
varying
environmental
impacts
due
to
different
physical
chemical
properties
of
its
components.
However,
traditional
methods
quantify
PM2.5
components
are
often
based
on
online
or
offline
observations
numerical
models,
which
generally
high
economic
cost-
labor-intensive.
In
this
study,
we
develop
a
new
method,
named
Multi-Tracer
Estimation
Algorithm
(MTEA),
identify
the
primary
from
routine
observation
PM2.5.
By
comparing
with
long-term
short-term
measurements
aerosol
in
China
United
States,
it
is
proven
that
MTEA
successfully
capture
magnitude
variation
(PPM)
(SPM).
Applying
National
Air
Quality
Network,
find
(1)
SPM
accounted
for
63.5
%
cities
southern
average
during
2014–2018,
while
proportion
dropped
57.1
north
China,
at
same
time
regional
background
regions
was
∼
19
higher
than
populous
regions;
(2)
summertime
presented
slight
but
consistent
increasing
trend
(from
58.5
59.2
%)
most
cities,
mainly
because
recent
increase
O3
pollution
China;
(3)
Beijing
significantly
increased
by
34
COVID-19
lockdown,
might
be
main
reason
observed
unexpected
PM
special
period;
finally,
(4)
showed
similar
positive
correlations
Beijing-Tianjin-Hebei
(BTH)
Yangtze
River
Delta
(YRD)
regions,
between
total
these
two
as
determined
PPM
levels,
were
quite
different.
general,
promising
tool
efficiently
estimating
SPM,
has
huge
potential
future
mitigation.
Atmospheric chemistry and physics,
Год журнала:
2025,
Номер
25(6), С. 3603 - 3621
Опубликована: Март 26, 2025
Abstract.
We
examined
the
effects
of
2010–2045
climate
change
on
ozone
(O3)
levels
in
China
under
a
carbon
neutrality
scenario
using
Global
Change
and
Air
Pollution
version
2.0
(GCAP
2.0)
model.
In
eastern
(EC),
GCAP
six
other
models
from
Coupled
Model
Intercomparison
Project
Phase
6
(CMIP6)
all
projected
increases
daily
maximum
2
m
temperature
(T2max),
surface
incoming
shortwave
radiation
(SW),
planet
boundary
layer
height
decreases
relative
humidity
(RH)
sea
level
pressure.
Future
is
simulated
by
to
have
large
O3
even
pathway,
with
summertime
regional
seasonal
mean
8
h
average
(MDA8)
concentrations
increasing
2.3
ppbv
(3.9
%)
over
EC,
4.7
(7.3
North
Plain,
3.0
(5.1
Yangtze
River
Delta.
Changes
key
meteorological
parameters
were
found
explain
58
%–76
%
climate-driven
MDA8
changes
EC.
The
most
important
summer
are
T2max
SW
northern
central
EC
RH
southern
Analysis
showed
net
chemical
production
was
process
that
O3,
accounting
for
34.0
%–62.5
sum
processes
within
layer.
also
quantified
uncertainties
climate-induced
CMIP6
multi-model
projections
stepwise
multiple
linear
regression
results
at
lower
end
multi-models.
These
implications
policy-making
regarding
emission
controls
against
background
warming.
Frontiers in Environmental Science,
Год журнала:
2023,
Номер
10
Опубликована: Янв. 16, 2023
Stratospheric
intrusion
(SI)
is
an
important
source
of
tropospheric
ozone
(O
3
).
Here,
we
used
the
online
coupled
Weather
Research
and
Forecasting-Chemistry
(WRF-Chem)
model
to
simulate
a
typical
SI
event
that
occurred
over
eastern
China
on
15–19
July
2016
investigate
impacts
near-surface
O
pollution.
The
results
show
large-scale
circulation
was
characterized
by
deep
trough
central
South
Asia
high
Western
Pacific
Subtropical
located
east
west
trough,
respectively.
With
evolution
strong
downdrafts
behind
lead
-rich
air
injected
into
lower
troposphere
across
China.
By
using
tracer
tagging
method
in
WRF-Chem,
quantified
contributed
up
6.5
ppb
surface
concentration.
According
integrated
process
rate
analyses,
which
were
employed
quantify
contribution
different
physical/chemical
processes
,
advection
dominated
variations
with
positive
ranging
from
0.1
13.8
h
−1
.
As
altitude
decreases,
diminishes
as
intensity
gradually
weakens.
Although
vertical
limited
directly
reached
ground,
revealed
has
significant
impact
large
territory
through
regional
transport
horizontal
process.
Below
691
m,
ranges
1.6
13.4
This
study
highlights
natural
effect
summertime
pollution
will
help
development
future
alert
system.
Atmosphere,
Год журнала:
2022,
Номер
13(9), С. 1450 - 1450
Опубликована: Сен. 7, 2022
Understanding
the
response
of
tropospheric
ozone
(O3)
to
nitrogen
dioxide
(NO2)
change
is
important
for
local
O3
control.
The
relationship
between
and
NO2
at
county
scale
in
China
has
been
extensively
studied
using
models,
but
there
a
lack
results
from
direct
measurements.
In
this
study,
we
used
measurements
O3,
meteorological
conditions
dense
network
Yangtze
River
Delta
(YRD),
satellite
observed
formaldehyde
(HCHO)
column
densities
analysis
variabilities
its
NO2.
As
result,
severe
pollution
occurred
mainly
Shanghai
city,
southern
Jiangsu
northern
Zhejiang
provinces
YRD
during
April–September.
addition,
could
explain
54%
diurnal
variation
over
YRD.
During
April–September
2015–2021,
showed
significant
positive
(r
=
0.61
±
0.10)
with
after
removing
impact
conditions.
However,
be
reversed
concentration
change.
Our
result
suggested
that
controllable
related
up
100
μg·m−3
megacities
province.
much
more
sensitive
reduction
than
surrounding
areas.
evaluate
different
impacts
changes
on
formation,
which
provides
explanation
simultaneously
alleviated
reduced
2020
Zhejiang,
as
well
increased
most
counties
before
2019
October–March.
driving
mechanism
revealed
study
will
valuable
abatement
through
sub-county
China.