Journal of Materials Chemistry A,
Год журнала:
2024,
Номер
12(18), С. 10808 - 10818
Опубликована: Янв. 1, 2024
This
work
presents
a
multifunctional
MXene-composited
organohydrogel
with
high
tensile
strength,
excellent
environmental
stability,
recyclability
and
outstanding
UV-shielding
ability
for
flexible
wearable
sensors.
Advanced Materials,
Год журнала:
2024,
Номер
36(24)
Опубликована: Фев. 21, 2024
In
the
past
decade,
with
rapid
development
of
wearable
electronics,
medical
health
monitoring,
Internet
Things,
and
flexible
intelligent
robots,
pressure
sensors
have
received
unprecedented
attention.
As
a
very
important
kind
electronic
component
for
information
transmission
collection,
gained
wide
application
prospect
in
fields
aerospace,
biomedical
skin,
human-machine
interface.
recent
years,
MXene
has
attracted
extensive
attention
because
its
unique
2D
layered
structure,
high
conductivity,
rich
surface
terminal
groups,
hydrophilicity,
which
brought
new
breakthrough
sensing.
Thus,
it
become
revolutionary
pressure-sensitive
material
great
potential.
this
work,
advances
MXene-based
are
reviewed
from
aspects
sensing
type,
mechanism,
selection,
structural
design,
preparation
strategy,
application.
The
methods
strategies
to
improve
performance
analyzed
details.
Finally,
opportunities
challenges
faced
by
discussed.
This
review
will
bring
research
level,
promoting
wider
exploitation
practical
materials
sensors.
Advanced Functional Materials,
Год журнала:
2023,
Номер
33(42)
Опубликована: Июнь 24, 2023
Abstract
E‐skins
based
on
conductive
hydrogels
are
regarded
as
ideal
candidates
for
sensing
application.
However,
limited
by
the
constructed
materials
and
strategies,
current
have
poor
mechanical
properties,
single
function,
unsatisfactory
conductivity,
which
seriously
hinder
their
development
Herein,
natural
goatskin
with
hierarchical
3D
network
structure
weaved
collagen
fibers
is
used
substrate
material
construction
of
ultra‐tough
hydrogel
through
a
“top‐down”
strategy,
in
acrylic
acid
monomer
first
vacuum‐impregnated
into
interstices
skeleton
then
polymerized
situ
to
produce
skin‐based
unique
wrapping
structure.
Based
hydrogel,
load‐carrying
capacity,
after
loaded
new
multifunctional
nanoscale‐conductive
medium
nanosilver
particles
(AgNPs)
1,3‐propanediol,
goatskin‐derived
organohydrogel
S@HCP
excellent
self‐adhesion,
transparency,
ultraviolet
shielding,
antibacterial,
biocompatibility,
environmental
stability,
conductivity.
Notably,
stretchable
S‐TENG
assembled
using
can
be
perfectly
suited
real‐life
applications
including
biomechanical
energy
harvesting,
self‐powered
tactile‐sensing,
motion
monitoring.
It
believed
that,
combining
animal
skin
different
functional
materials,
it
possible
reuse
skin,
“dead
skin,”
provides
platform
developing
flexible
e‐skin.
Advanced Functional Materials,
Год журнала:
2023,
Номер
33(37)
Опубликована: Май 14, 2023
Abstract
Developing
versatile
and
high
sensitivity
sensors
is
beneficial
for
promoting
flexible
electronic
devices
human‐machine
interactive
systems.
Researchers
are
working
on
the
exploration
of
various
active
sensing
materials
toward
broad
detection,
multifunction,
low‐power
consumption.
Here,
a
ion‐gel
fibrous
membrane
presented
by
electrospinning
technology
utilized
to
construct
capacitive
triboelectric
nanogenerator
(TENG).
The
iontronic
sensor
exhibits
inherently
favorable
repeatability,
which
retains
long‐term
stability
after
5000
cycles.
can
also
detect
clear
pulse
waveform
at
human
wrist
enable
mapping
pressure
distribution
sensory
matrix.
For
TENG,
maximum
peak
power
54.56
µW
be
used
commercial
electronics.
In
addition,
prepared
TENG
array
achieve
interactive,
rapidly
responsive,
accurate
dynamic
monitoring,
broadens
direct
effective
devices.
promising
provide
an
outstanding
approach
physiological
biomechanical
energy
harvesting,
interaction,
self‐powered
monitoring
Nano Letters,
Год журнала:
2024,
Номер
24(12), С. 3826 - 3834
Опубликована: Март 18, 2024
Lightweight,
easily
processed,
and
durable
polymeric
materials
play
a
crucial
role
in
wearable
sensor
devices.
However,
achieving
simultaneously
high
strength
toughness
remains
challenge.
This
study
addresses
this
by
utilizing
an
ion-specific
effect
to
control
crystalline
domains,
enabling
the
fabrication
of
triboelectric
material
with
tunable
mechanical
properties.
The
dense
crystal-domain
cross-linking
enhances
energy
dissipation,
resulting
boasting
both
tensile
(58.0
MPa)
(198.8
MJ
m–3),
alongside
remarkable
416.7%
fracture
elongation
545.0
MPa
modulus.
Leveraging
these
properties,
is
successfully
integrated
into
self-powered
devices,
real-time
feedback
on
human
joint
movement.
work
presents
valuable
strategy
for
overcoming
strength-toughness
trade-off
materials,
paving
way
their
enhanced
applicability
broader
use
diverse
sensing
applications.
Journal of Materials Chemistry A,
Год журнала:
2024,
Номер
12(16), С. 9296 - 9321
Опубликована: Янв. 1, 2024
This
review
covers
recent
advancements
in
flexible
resistive
tactile
pressure
sensors,
including
operational
principles,
performance
metrics,
material
choices,
structural
design,
and
applications,
as
well
future
challenges.
Chemical Reviews,
Год журнала:
2024,
Номер
124(17), С. 9899 - 9948
Опубликована: Авг. 28, 2024
Electronic
skins
(e-skins)
have
seen
intense
research
and
rapid
development
in
the
past
two
decades.
To
mimic
capabilities
of
human
skin,
a
multitude
flexible/stretchable
sensors
that
detect
physiological
environmental
signals
been
designed
integrated
into
functional
systems.
Recently,
researchers
increasingly
deployed
machine
learning
other
artificial
intelligence
(AI)
technologies
to
neural
system
for
processing
analysis
sensory
data
collected
by
e-skins.
Integrating
AI
has
potential
enable
advanced
applications
robotics,
healthcare,
human–machine
interfaces
but
also
presents
challenges
such
as
diversity
model
robustness.
In
this
review,
we
first
summarize
functions
features
e-skins,
followed
feature
extraction
different
models.
Next,
discuss
utilization
design
e-skin
address
key
topic
implementation
e-skins
accomplish
range
tasks.
Subsequently,
explore
hardware-layer
in-skin
before
concluding
with
an
opportunities
various
aspects
AI-enabled
ACS Applied Materials & Interfaces,
Год журнала:
2024,
Номер
16(9), С. 11914 - 11929
Опубликована: Фев. 21, 2024
Conductive
hydrogels
have
shown
promising
application
prospects
in
the
field
of
flexible
sensors,
but
they
often
suffer
from
poor
mechanical
properties,
low
sensitivity,
and
lack
frost
resistance.
Herein,
we
report
a
tough,
highly
sensitive,
antifreeze
strain
sensor
assembled
conductive
organohydrogel
composed
dual-cross-linked
polyacrylamide
poly(vinyl
alcohol)
(PVA)
network,
as
well
MXene
nanosheets
nanofillers
poly(3,4-ethylenedioxythiophene)-doped
poly(styrenesulfonate)
(PEDOT/PSS)
main
conducting
component
(PPMP-OH
organohydrogel).
The
tensile
strength
toughness
PPMP-OH
had
been
greatly
enhanced
by
due
to
reinforcement
nanosheets,
various
strong
noncovalent
interactions
formed
organohydrogels.
PPM1P-OH
organohydrogels
showed
1.48
MPa
at
772%
5.59
MJ/m3.
Moreover,
conductivity
strain-sensing
performance
were
significantly
improved
PEDOT/PSS,
which
can
form
hydrogen
bonds
with
PVA
electrostatic
MXene.
This
was
beneficial
for
constructing
uniformly
distributed
stable
3D
network
helped
obtain
strain-dependent
resistance
PPMP-OH.
sensors
PPMP1-OH
exhibited
high
sensitivity
5.16,
wide
range
detectable
strains
up
500%,
short
response
time
122
ms,
effectively
detect
physiological
activities
human
body
stability.
In
addition,
corresponding
pressure
array
also
identifying
magnitude
position.
ACS Nano,
Год журнала:
2024,
Номер
18(36), С. 24705 - 24740
Опубликована: Авг. 26, 2024
The
gradual
rise
of
personal
healthcare
awareness
is
accelerating
the
deployment
wearable
sensors,
whose
ability
acquiring
physiological
vital
signs
depends
on
sensing
materials.
MXenes
have
distinct
chemical
and
physical
superiorities
over
other
2D
nanomaterials
for
sensors.
This
review
presents
a
comprehensive
summary
latest
advancements
in
MXenes-based
materials
It
begins
with
an
introduction
to
special
structural
features
performance,
followed
by
in-depth
exploration
versatile
functionalities.
A
detailed
description
different
mechanisms
also
included
illustrate
contribution
performance
its
improvement.
In
addition,
real-world
applications
sensors
monitoring
are
as
well.
remaining
challenges
their
promising
opportunities
finally
narrated,
conjunction
prospective
future
development.