Nature Communications,
Journal Year:
2023,
Volume and Issue:
14(1)
Published: Aug. 26, 2023
Timely
and
remote
biomarker
detection
is
highly
desired
in
personalized
medicine
health
protection
but
presents
great
challenges
the
devices
reported
so
far.
Here,
we
present
a
cost-effective,
flexible
self-powered
sensing
device
for
H2S
analysis
various
application
scenarios
based
on
structure
of
galvanic
cells.
The
mechanism
attributed
to
change
electrode
potential
resulting
from
chemical
adsorption
gas
molecules
surfaces.
Intrinsically
stretchable
organohydrogels
are
used
as
solid-state
electrolytes
enable
stable
long-term
operation
under
stretching
deformation
or
environments.
open-circuit
exhibits
high
sensitivity,
low
limit,
excellent
selectivity
H2S.
Its
non-invasive
halitosis
diagnosis
identification
meat
spoilage
demonstrated,
emerging
commercial
value
portable
medical
electronics
food
security.
A
wireless
sensory
system
has
also
been
developed
monitoring
with
participation
Bluetooth
cloud
technologies.
This
work
breaks
through
shortcomings
traditional
chemiresistive
sensors,
offering
direction
theoretical
foundation
designing
wearable
sensors
catering
other
stimulus
requirements.
Advanced Materials,
Journal Year:
2022,
Volume and Issue:
35(14)
Published: Aug. 29, 2022
Abstract
Flexible
electronics
is
an
emerging
field
of
research
involving
multiple
disciplines,
which
include
but
not
limited
to
physics,
chemistry,
materials
science,
electronic
engineering,
and
biology.
However,
the
broad
applications
flexible
are
still
restricted
due
several
limitations,
including
high
Young's
modulus,
poor
biocompatibility,
responsiveness.
Innovative
aiming
for
overcoming
these
drawbacks
boost
its
practical
application
highly
desirable.
Hydrogel
a
class
3D
crosslinked
hydrated
polymer
networks,
exceptional
material
properties
render
it
as
promising
candidate
next
generation
electronics.
Here,
latest
methods
synthesizing
advanced
functional
hydrogels
state‐of‐art
hydrogel‐based
in
various
fields
reviewed.
More
importantly,
correlation
between
hydrogel
device
performance
discussed
here,
have
better
understanding
development
by
using
environmentally
responsive
hydrogels.
Last,
perspectives
on
current
challenges
future
directions
multifunctional
provided.
Advanced Science,
Journal Year:
2022,
Volume and Issue:
9(10)
Published: Jan. 31, 2022
Abstract
Rapid
advances
in
wearable
electronics
and
mechno‐sensational
human–machine
interfaces
impose
great
challenges
developing
flexible
deformable
tactile
sensors
with
high
efficiency,
ultra‐sensitivity,
environment‐tolerance,
self‐sustainability.
Herein,
a
hydrogel
sensor
(THS)
based
on
micro‐pyramid‐patterned
double‐network
(DN)
ionic
organohydrogels
to
detect
subtle
pressure
changes
by
measuring
the
variations
of
triboelectric
output
signal
without
an
external
power
supply
is
reported.
By
first
time
pyramidal‐patterned
fabrication
method
laminated
polydimethylsiloxane
(PDMS)
encapsulation
process,
self‐powered
THS
shows
advantages
remarkable
flexibility,
good
transparency
(≈85%),
excellent
sensing
performance,
including
extraordinary
sensitivity
(45.97
mV
Pa
−1
),
fast
response
(≈20
ms),
very
low
limit
detection
(50
Pa)
as
well
stability
(36
000
cycles).
Moreover,
LiBr
immersion
treatment
method,
possesses
long‐term
hyper
anti‐freezing
anti‐dehydrating
properties,
broad
environmental
tolerance
(−20
60
°C),
instantaneous
peak
density
20
µW
cm
−2
,
providing
reliable
contact
outputs
different
materials
detecting
slight
human
motions.
integrating
acquisition/process
circuit,
self‐power
ability
utilized
switching
button
control
electric
appliances
robotic
hands
simulating
finger
gestures,
offering
its
potentials
for
multi‐functional
electronic
applications.
Advanced Functional Materials,
Journal Year:
2021,
Volume and Issue:
31(40)
Published: July 11, 2021
Abstract
Electronic
skin
(e‐skin)
is
driving
significant
advances
in
flexible
electronics
as
it
holds
great
promise
health
monitoring,
human–machine
interfaces,
soft
robotics,
and
so
on.
Flexible
sensors
that
can
detect
various
stimuli
or
have
multiple
properties
play
an
indispensable
role
e‐skin.
Despite
tremendous
research
efforts
devoted
to
with
excellent
performance
regarding
a
certain
sensing
mode
property,
emerging
e‐skin
demands
multifunctional
be
endowed
the
skin‐like
capability
beyond.
Considering
outstanding
superiorities
of
electrical
conductivity,
chemical
stability,
ease
functionalization,
carbon
materials
are
adopted
implement
sensors.
In
this
review,
latest
carbon‐based
regard
types
detection
modes
abundant
introduced.
The
corresponding
preparation
process,
device
structure,
mechanism,
obtained
performance,
intriguing
applications
highlighted.
Furthermore,
diverse
systems
by
integrating
current
cutting‐edge
technologies
(e.g.,
data
acquisition
transmission,
neuromorphic
technology,
artificial
intelligence)
systematically
investigated
detail.
Finally,
existing
problems
future
developing
directions
also
proposed.
ACS Applied Materials & Interfaces,
Journal Year:
2023,
Volume and Issue:
15(4), P. 5128 - 5138
Published: Jan. 19, 2023
The
rapid
development
of
wearable
electronic
devices
and
virtual
reality
technology
has
revived
interest
in
flexible
sensing
control
devices.
Here,
we
report
an
ionic
hydrogel
(PTSM)
prepared
from
polypropylene
amine
(PAM),
tannic
acid
(TA),
sodium
alginate
(SA),
MXene.
Based
on
the
multiple
weak
H-bonds,
this
exhibits
excellent
stretchability
(strain
>4600%),
adhesion,
self-healing.
introduction
MXene
nanosheets
endows
sensor
with
a
high
gauge
factor
(GF)
6.6.
Meanwhile,
it
also
enables
triboelectric
nanogenerators
(PTSM-TENGs)
fabricated
silicone
rubber-encapsulated
hydrogels
to
have
energy
harvesting
efficiency,
instantaneous
output
power
density
54.24
mW/m2.
We
build
glove-based
human-computer
interaction
(HMI)
system
using
PTSM-TENGs.
multidimensional
signal
features
PTSM-TENG
are
extracted
analyzed
by
HMI
system,
functions
gesture
visualization
robot
hand
realized.
In
addition,
signals
can
be
used
for
object
recognition
help
machine
learning
techniques.
glove
based
achieves
classification
five
objects
through
contact,
accuracy
rate
98.7%.
Therefore,
strain
sensors
broad
application
prospects
man-machine
interface,
intelligent
systems,
auxiliary
other
fields
due
their
stretchable
self-healing
performance.
Nano-Micro Letters,
Journal Year:
2022,
Volume and Issue:
14(1)
Published: March 21, 2022
Conductive
hydrogels
have
potential
applications
in
shielding
electromagnetic
(EM)
radiation
interference
deformable
and
wearable
electronic
devices,
but
usually
suffer
from
poor
environmental
stability
stretching-induced
performance
degradation.
Although
organohydrogels
can
improve
the
of
materials,
their
development
is
at
expense
reducing
electrical
conductivity
thus
weakening
EM
ability.
Here,
a
MXene
organohydrogel
prepared
which
composed
network
for
electron
conduction,
binary
solvent
channels
ion
abundant
solvent-polymer-MXene
interfaces
wave
scattering.
This
possesses
excellent
anti-drying
ability,
low-temperature
tolerance,
stretchability,
shape
adaptability,
adhesion
rapid
self-healing
Two
effective
strategies
been
proposed
to
solve
problems
current
materials.
By
reasonably
controlling
content
glycerol-water
ratio
gel,
exhibit
exceptionally
enhanced
performances
compared
hydrogel
due
increased
physical
cross-linking
density
gel.
Moreover,
shows
attractive
stretching-enhanced
effectiveness,
caused
by
connection
parallel
arrangement
nanosheets.
well-designed
has
devices.
Advanced Functional Materials,
Journal Year:
2021,
Volume and Issue:
32(1)
Published: Oct. 1, 2021
Abstract
Flexible
electronic
devices
(FEDs)
based
on
hydrogels
are
attracting
increasing
interest,
but
the
fabrication
of
for
FEDs
with
adhesiveness
and
high
robustness
in
harsh‐temperature
conditions
long‐term
use
remains
a
challenge.
Herein,
glutinous‐rice‐inspired
adhesive
organohydrogels
developed
by
introducing
amylopectin
into
copolymer
network
through
“one‐pot”
crosslinking
procedure
glycerol–water
mixed
solvent
containing
potassium
chloride
as
conductive
ingredient.
The
exhibit
excellent
transparency
(>90%),
conductivity,
stretchability,
tensile
strength,
adhesiveness,
anti‐freezing
property,
moisture
retention
ability.
wearable
strain
sensor
assembled
from
achieves
wide
working
range,
sensitivity
(gauge
factor:
8.82),
low
response
time,
reversibility,
properly
responds
long‐time
storage
(90
days).
is
further
integrated
Bluetooth
transmitter
receiver
fabricating
wireless
sensors.
Notably,
sandwich‐structured
capacitive
pressure
reliefs
electrodes
records
new
gauge
factor
9.43
kPa
−1
detection
limit,
outstanding
reversibility.
Furthermore,
detachable
durable
batteries
all‐in‐one
supercapacitors
also
fabricated
utilizing
electrolytes.
Overall,
this
work
offers
strategy
to
fabricate
robust
toward
sensing,
power
supply,
energy
storage.
Advanced Functional Materials,
Journal Year:
2023,
Volume and Issue:
33(42)
Published: July 14, 2023
Abstract
Conducting
polymer
hydrogels
are
widely
used
as
strain
sensors
in
light
of
their
distinct
skin‐like
softness,
sensitivity,
and
environmental
adaptiveness
the
fields
wearable
devices,
soft
robots,
human‐machine
interface.
However,
mechanical
electrical
properties
existing
conducting
hydrogels,
especially
fatigue‐resistance
sensing
robustness
during
long‐term
application,
unsatisfactory,
which
severely
hamper
practical
utilities.
Herein,
a
strategy
to
fabricate
with
anisotropic
structures
mechanics
is
presented
through
combined
freeze‐casting
salting‐out
process.
The
as‐fabricated
exhibit
high
fatigue
threshold
(>300
J
m
−2
),
low
Young's
modulus
(≈100
kPa),
well
(over
10
000
cycles).
Such
superior
performance
enables
application
monitor
real‐time
movement
underwater
robotics.
design
fabrication
for
reported
this
study
may
open
up
an
enticing
avenue
functional
materials
electronics
Materials Horizons,
Journal Year:
2021,
Volume and Issue:
8(12), P. 3409 - 3416
Published: Jan. 1, 2021
By
leveraging
tannic-acid-enabled
dynamic
interactions,
we
designed
an
ionic
hydrogel
with
boosted
bulk
and
interfacial
properties
such
as
ultra-stretchability,
remarkable
self-healing
capability
robust
adhesion.