Ultralight Hierarchical Fe3O4/MoS2/rGO/Ti3C2Tx MXene Composite Aerogels for High-Efficiency Electromagnetic Wave Absorption DOI

Shiyao Yan,

Shiping Shao,

Yunxiang Tang

et al.

ACS Applied Materials & Interfaces, Journal Year: 2024, Volume and Issue: 16(28), P. 36962 - 36972

Published: July 3, 2024

Aerogel-based composites, renowned for their three-dimensional (3D) network architecture, are gaining increasing attention as lightweight electromagnetic (EM) wave absorbers. However, attaining high reflection loss, broad effective absorption bandwidth (EAB), and ultrathin thickness concurrently presents a formidable challenge, owing to the stringent demands precise structural regulation incorporation of magnetic/dielectric multicomponents with synergistic loss mechanisms within 3D networks. In this study, we successfully synthesized hierarchical porous Fe

Language: Английский

2D/2D coupled MOF/Fe composite metamaterials enable robust ultra–broadband microwave absorption DOI Creative Commons

Ning Qu,

Hanxu Sun,

Yuyao Sun

et al.

Nature Communications, Journal Year: 2024, Volume and Issue: 15(1)

Published: July 5, 2024

Abstract The combination between macroscopic structure designs and microscopic material offers tremendous possibilities for the development of advanced electromagnetic wave (EMW) absorbers. Herein, we propose a metamaterial design to address persistent challenges in this field, including narrow bandwidth, low–frequency bottlenecks, and, particularly, urgent issue robustness (i.e., oblique, polarized incidence). Our absorber features semiconductive metal-organic framework/iron 2D/2D assembly (CuHT–FCIP) with abundant crystal/crystal heterojunctions strong magneto-electric coupling networks. This achieves remarkable EMW absorption across broad range (2 40 GHz) at thickness just 9.3 mm. Notably, it maintains stable performance against oblique incidence (within 75°) polarizations (both transverse electric magnetic). Furthermore, demonstrates high specific compressive strength (201.01 MPa·cm 3 ·g −1 ) low density (0.89 g·cm −3 ). advancement holds promise developing robust absorbers superior performance.

Language: Английский

Citations

63

Mechanisms, design, and fabrication strategies for emerging electromagnetic wave-absorbing materials DOI Creative Commons
Geng Chen,

Zijing Li,

Limin Zhang

et al.

Cell Reports Physical Science, Journal Year: 2024, Volume and Issue: 5(7), P. 102097 - 102097

Published: July 1, 2024

The rapid development of intelligent devices imposes new demands on electromagnetic wave (EMW)-absorbing materials, especially concerning wide-spectrum absorption, frequency band manipulation, and multifunctional integration. However, conventional investigations EMW-absorbing materials face several challenges that collectively limit the effectiveness existing amid growing demands, including ambiguous (EM) loss mechanisms, impedance mismatches, deficiencies in integrated design. This review elucidates EM delineates key bridge mechanisms linking microscopic macroscopic factors, proposes dielectric polarization models to clarify mechanisms. Additionally, it delves into unique advantages core-shell structures porous optimization. Finally, introduces fabrication approaches integrate detailing design strategies exploring potential applications. By consolidating these cutting-edge achievements, this aims guide scientific advancement materials.

Language: Английский

Citations

61

Modulating magnetic interface layer on porous carbon heterostructures for efficient microwave absorption DOI
Zirui Jia,

Lifu Sun,

Zhenguo Gao

et al.

Nano Research, Journal Year: 2024, Volume and Issue: unknown

Published: Sept. 3, 2024

Language: Английский

Citations

56

Multi-mode tunable electromagnetic wave absorber based on hollow nano-cage structure and self-anticorrosion performance DOI
Yuelei Pan, Di Lan, Zirui Jia

et al.

Advanced Composites and Hybrid Materials, Journal Year: 2024, Volume and Issue: 7(2)

Published: Feb. 24, 2024

Language: Английский

Citations

45

Fabrication of multifunctional Co,N co-doped UIO-rGO aerogel with properties of hydrophobic, anti-corrosion, heat insulation, infrared stealth and electromagnetic wave absorption DOI

Kunyao Cao,

Weiping Ye, Yue Zhang

et al.

Chemical Engineering Journal, Journal Year: 2024, Volume and Issue: 492, P. 152275 - 152275

Published: May 15, 2024

Language: Английский

Citations

43

Porous Structure Fibers Based on Multi‐Element Heterogeneous Components for Optimized Electromagnetic Wave Absorption and Self‐Anticorrosion Performance DOI
Jiahui Zhu, Di Lan, Xuehua Liu

et al.

Small, Journal Year: 2024, Volume and Issue: 20(47)

Published: Aug. 11, 2024

Abstract The excellent performance of electromagnetic wave absorbers primarily depends on the coordination among components and rational design structure. In this study, a series porous fibers with carbon nanotubes uniformly distributed in shape pine leaves are prepared through electrospinning technique, one‐pot hydrothermal synthesis, high‐temperature catalysis method. impedance matching nanofibers structure is optimized by incorporating melamine into spinning solution, as it undergoes gas decomposition during calcination. Moreover, electronic can be modulated controlling NH 4 F content synthesis process. Ultimately, Ni/Co/CrN/CNTs‐CF specimen (P3C NiCrN12) exhibited superior performance, while achieving minimum reflection loss (RL min ) −56.18 dB at thickness 2.2 mm maximum absorption bandwidth (EAB max 5.76 GHz 2.1 mm. This study presents an innovative approach to fabricating lightweight, thin materials exceptional properties wide optimizing three key factors influencing performance.

Language: Английский

Citations

42

Preparation of cellulose derived carbon/reduced graphene oxide composite aerogels for broadband and efficient microwave dissipation DOI
Ruiwen Shu, Lingling Xu, Guan Yang

et al.

Journal of Colloid and Interface Science, Journal Year: 2024, Volume and Issue: 675, P. 401 - 410

Published: July 5, 2024

Language: Английский

Citations

31

Hierarchical Engineering on Built‐In Electric Field of Bimetallic Zeolitic Imidazolate Derivatives Towards Amplified Dielectric Loss DOI Open Access
Shijie Zhang, Jiajun Zheng, Di Lan

et al.

Advanced Functional Materials, Journal Year: 2024, Volume and Issue: unknown

Published: Oct. 7, 2024

Abstract Construction of built‐in electric field (BIEF) in nanohybrids has been demonstrated as an efficacious strategy to boost the dielectric loss by facilitating oriented transfer and transition charges, thus optimizing electromagnetic wave absorption property. However, specific influence BIEF on interface polarization needs explore thoroughly strength should be further augmented. Herein, several systems incorporated Mott–Schottky heterojunctions hollow structures are designed constructed, where bimetallic zeolitic imidazolate framework employed derive Cu‐ZnO heterojunctions, hierarchical enriched introducing structure reduced graphene oxide. The well‐established “double” verified theoretical calculation engineering can regulate conductivity, enhance relaxation effectively. Especially, there always coexisted both enhanced charge separation reversed distribution this BIEF, boosting polarization. Attributing synergy well‐matched impedance amplified loss, obtained hybrids exhibited superior (reflection −46.29 dB ultra‐wide effective bandwidth 7.6 GHz at only 1.6 mm). This work proves innovative model for dissecting mechanisms pioneers a novel advanced absorbers through enhancing BIEF.

Language: Английский

Citations

29

Fabrication of 3D micro-flower structured BiFeO3 growing on rGO nanosheets for enhanced electromagnetic wave absorption DOI

Kunyao Cao,

Weiping Ye, Yue Zhang

et al.

Chemical Engineering Journal, Journal Year: 2024, Volume and Issue: 496, P. 154184 - 154184

Published: July 22, 2024

Language: Английский

Citations

25

Zeolite imidazolate framework derived efficient absorbers: from morphology modulation to component regulation DOI
Jiajun Zheng, Di Lan, Shijie Zhang

et al.

Journal of Alloys and Compounds, Journal Year: 2024, Volume and Issue: 1010, P. 177092 - 177092

Published: Oct. 16, 2024

Language: Английский

Citations

25