Separation and Purification Technology, Journal Year: 2024, Volume and Issue: unknown, P. 131146 - 131146
Published: Dec. 1, 2024
Language: Английский
Separation and Purification Technology, Journal Year: 2024, Volume and Issue: unknown, P. 131146 - 131146
Published: Dec. 1, 2024
Language: Английский
Journal of environmental chemical engineering, Journal Year: 2024, Volume and Issue: 12(6), P. 114202 - 114202
Published: Sept. 20, 2024
Language: Английский
Citations
1Journal of Colloid and Interface Science, Journal Year: 2024, Volume and Issue: 681, P. 71 - 81
Published: Nov. 22, 2024
Language: Английский
Citations
1Published: Jan. 1, 2024
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Language: Английский
Citations
0Published: Jan. 1, 2024
The interplay between high-energy holes and reactive oxygen species (ROS) in the deep mineralization of organic pollutants remains a relatively uncharted domain. Unlocking mechanisms by which facilitate contaminants during photocatalysis is critical for achieving mineralization. Here, we synthesized an oxygen-doped/biochar-modified 2D C3N4 (termed A-CN) via calcination supramolecular precursor assembled on hydroxyl-rich aloe fiber. This dual modification strategy altered interlayer electronic structure in-plane configuration A-CN, promoting its photocatalytic activity. synchronized evaluation removal efficiency toxicity analysis attests to antibiotic contaminant, while continuous degradation system underscores stability A-CN. A-CN exhibited 95% within 1 h, 2.23-fold more efficient than bulk carbon nitride (B-CN), 88% rate, 4.81-fold higher B-CN. In flow device (a rate 2 mL/min), about 92%. mechanism primarily involves hole-mediated deamidation ROS-driven oxidative ring-opening reactions, facilitating structural disassembly antibiotics. investigation potential biochar/oxygen doping-induced ROS pollutant remediation, providing effective protocol degradation.
Language: Английский
Citations
0Separation and Purification Technology, Journal Year: 2024, Volume and Issue: unknown, P. 131146 - 131146
Published: Dec. 1, 2024
Language: Английский
Citations
0