Advanced Science,
Journal Year:
2023,
Volume and Issue:
10(25)
Published: June 28, 2023
Special
separation
membranes
are
widely
employed
for
and
purification
purposes
under
challenging
operating
conditions
due
to
their
low
energy
consumption,
excellent
solvent,
corrosion
resistance.
However,
the
development
of
is
limited
by
corrosion-resistant
polymer
substrates
precise
interfacial
layers.
Herein,
polyaniline
(PANI)
achieve
insitu
anchoring
multiple
interfaces,
resulting
in
fabrication
polyaniline@graphene
oxide/polyether
ether
ketone
(PANI@GO/PEEK)
membranes.
Insitu
growth
PANI
achieves
adequate
bonding
PEEK
substrate
GO
interface,
which
solves
problem
solution
processing
instability
By
bottom-up
confined
polymerization
aniline,
it
could
control
pore
size
layer,
correct
defects,
anchor
among
polymer,
nano-separation
nano-sheet.
The
mechanism
membrane
construction
within
domain
micro-nano
structure
modulation
further
explored.
demonstrate
exceptional
stability
realizing
over
90%
rejection
2
m
HCl,
NaOH,
high
temperatures.
Additionally,
-membranes
exhibit
remarkable
durability
after
240
days
immersion
100
h
long-term
operation,
display
methanol
flux
50.2
L
m-2
h-1
92%
AF
(585
g
mol-1
).
This
method
substantially
contributes
special
offering
a
novel
strategy.
Angewandte Chemie International Edition,
Journal Year:
2023,
Volume and Issue:
62(13)
Published: Jan. 3, 2023
Abstract
Two‐dimensional
(2D)
transition
metal
dichalcogenides
(TMDs),
a
rising
star
in
the
post‐graphene
era,
are
fundamentally
and
technologically
intriguing
for
photocatalysis.
Their
extraordinary
electronic,
optical,
chemical
properties
endow
them
as
promising
materials
effectively
harvesting
light
catalyzing
redox
reaction
Here,
we
present
tutorial‐style
review
of
field
2D
TMDs
photocatalysis
to
educate
researchers
(especially
new‐comers),
which
begins
with
brief
introduction
fundamentals
along
synthesis
this
type
material,
then
look
deeply
into
merits
co‐catalysts
active
photocatalysts,
followed
by
an
overview
challenges
corresponding
strategies
photocatalysis,
finally
ahead
topic.
Angewandte Chemie International Edition,
Journal Year:
2023,
Volume and Issue:
62(19)
Published: Jan. 31, 2023
Precise
and
ultrafast
ion
sieving
is
highly
desirable
for
many
applications
in
environment-,
energy-,
resource-related
fields.
The
development
of
a
permselective
lamellar
membrane
constructed
from
parallel
stacked
two-dimensional
(2D)
nanosheets
opened
new
avenue
the
next-generation
separation
technology
because
unprecedented
diversity
designable
interior
nanochannels.
In
this
Review,
we
first
discuss
construction
homo-
heterolaminar
nanoarchitectures
starting
materials
to
emerging
preparation
strategies.
We
then
explore
property-performance
relationships,
with
particular
emphasis
on
effects
physical
structural
features,
chemical
properties,
external
environment
stimuli
transport
behavior
under
nanoconfinement.
also
present
existing
potential
2D
membranes
desalination,
recovery,
energy
conversion.
Finally,
challenges
outline
research
directions
promising
field.
Angewandte Chemie,
Journal Year:
2023,
Volume and Issue:
135(13)
Published: Jan. 3, 2023
Abstract
Two‐dimensional
(2D)
transition
metal
dichalcogenides
(TMDs),
a
rising
star
in
the
post‐graphene
era,
are
fundamentally
and
technologically
intriguing
for
photocatalysis.
Their
extraordinary
electronic,
optical,
chemical
properties
endow
them
as
promising
materials
effectively
harvesting
light
catalyzing
redox
reaction
Here,
we
present
tutorial‐style
review
of
field
2D
TMDs
photocatalysis
to
educate
researchers
(especially
new‐comers),
which
begins
with
brief
introduction
fundamentals
along
synthesis
this
type
material,
then
look
deeply
into
merits
co‐catalysts
active
photocatalysts,
followed
by
an
overview
challenges
corresponding
strategies
photocatalysis,
finally
ahead
topic.
Advanced Materials,
Journal Year:
2024,
Volume and Issue:
36(31)
Published: May 21, 2024
Capacitive
deionization
(CDI)
has
emerged
as
a
promising
technology
for
freshwater
recovery
from
low-salinity
brackish
water.
It
is
still
inapplicable
in
specific
scenarios
(e.g.,
households,
islands,
or
offshore
platforms)
due
to
too
low
volumetric
adsorption
capacities.
In
this
study,
high-density
semi-metallic
molybdenum
disulfide
(1T'-MoS
Chemical Reviews,
Journal Year:
2024,
Volume and Issue:
124(9), P. 5795 - 5845
Published: April 19, 2024
Two-dimensional
(2D)
transition
metal
dichalcogenides
(TMDs)
with
layered
crystal
structures
have
been
attracting
enormous
research
interest
for
their
atomic
thickness,
mechanical
flexibility,
and
excellent
electronic/optoelectronic
properties
applications
in
diverse
technological
areas.
Solution-processable
2D
TMD
inks
are
promising
large-scale
production
of
functional
thin
films
at
an
affordable
cost,
using
high-throughput
solution-based
processing
techniques
such
as
printing
roll-to-roll
fabrications.
This
paper
provides
a
comprehensive
review
the
chemical
synthesis
solution-processable
printable
ink
materials
subsequent
assembly
into
applications.
We
start
principles
protocols
various
methods
nanosheet
crystals
solution
phase.
The
depositing
solid-state
discussed.
Then,
we
these
areas
including
electronics,
optoelectronics,
others.
To
conclude,
summary
key
scientific/technical
challenges
future
opportunities
is
provided.
Advanced Materials,
Journal Year:
2022,
Volume and Issue:
35(8)
Published: Nov. 10, 2022
Synthesis
of
large-area
patterned
MoS2
is
considered
the
principle
base
for
realizing
high-performance
-based
flexible
electronic
devices.
Patterning
and
transferring
films
to
target
substrates,
however,
require
conventional
multi-step
photolithography
patterning
process,
despite
tremendous
progress
in
facilitation
practical
applications.
Herein,
an
approach
directly
synthesize
large-scale
patterns
that
combines
inkjet
printing
thermal
annealing
reported.
An
optimal
precursor
ink
prepared
can
deposit
arbitrary
on
polyimide
films.
By
introducing
a
gas
atmosphere
argon/hydrogen
(Ar/H2
),
treatment
at
350
°C
enables
situ
decomposition
crystallization
precursors
and,
consequently,
results
formation
.
Without
complicated
processes,
obtained
polymer
substrate,
exhibiting
superior
mechanical
flexibility
durability
(≈2%
variation
resistance
over
10,000
bending
cycles),
as
well
excellent
chemical
stability,
which
attributed
generated
continuous
thin
microstructures,
their
strong
adhesion
with
substrate.
As
step
further,
this
employed
manufacture
various
sensing
devices
are
insensitive
body
motions
moisture,
including
temperature
sensors
biopotential
systems
real-time,
continuously
monitoring
skin
temperature,
electrocardiography,
electromyography
signals.
