Cited by Ameliorated trap density and energetic disorder <i>via</i> a strengthened intermolecular interaction strategy to construct efficient non-halogenated organic solar cells

A high-efficiency and stable organic solar cell with balanced crystallization kinetics DOI

Weichao Zhang,

Yaochang Yue,

Rongsheng Yang

et al.

Energy & Environmental Science, Journal Year: 2024, Volume and Issue: 17(6), P. 2182 - 2192

Published: Jan. 1, 2024

In this work, we present a conceptual strategy based on multi-acceptor components to realize balanced crystallization kinetics in organic solar cells (OSC) that deliver 19.35% power conversion efficiency with superior photostability.

Language: Английский

Citations

Sequentially Processed Bulk‐Heterojunction‐Buried Structure for Efficient Organic Solar Cells with 500 nm Thickness DOI

Huarui Zhang, Yuqiang Liu, Guangliu Ran

et al.

Advanced Materials, Journal Year: 2024, Volume and Issue: 36(25)

Published: March 13, 2024

Abstract Large‐area printing fabrication is a distinctive feature of organic solar cells (OSCs). However, the advance upscalable challenged by thickness active layers considering importance both exciton dissociation and charge collection. In this work, bulk‐heterojunction‐buried (buried‐BHJ) structure introduced sequential deposition to realize efficient collection, thereby contributing OSCs with 500 nm thick layers. The buried‐BHJ distributes donor acceptor phases in vertical direction as transport channels, while numerous BHJ interfaces are buried each phase facilitate simultaneously. It found that configurations possess rapid transport, resulting reduced recombination losses. comparison traditional structures, displays decent tolerance film thickness. particular, power conversion efficiency 16.0% achieved at nm. To best authors’ knowledge, represents champion OSCs.

Language: Английский

Citations

A Pseudo Planar Heterojunction Structure for Eco‐Friendly Printable Organic Solar Cells Achieving 19.05% Efficiency DOI

Pei Wang, Jiayou Zhang, Dou Luo

et al.

Advanced Functional Materials, Journal Year: 2024, Volume and Issue: 34(38)

Published: April 27, 2024

Abstract Obtaining a well‐accurate vertical distribution active layer morphology through the air‐printing process is an essential task for achieving efficient scalable large‐area organic solar cells (OSCs). In this target, desired and controllable pseudo planar heterojunction (PPHJ) structure with suitable phase separation developed by pre‐deposited D18‐Cl under PM6:BTP‐eC9 film via eco‐friendly manufacturing method. The addition of regulates molecular crystallization leads to ideal stratification while simultaneously suppressing voltage loss, optimizing energetic disorder, carrier management. Impressively, optimal PPHJ devices perform superior power conversion efficiencies (PCEs) 19.05% (100 nm), 17.33% (300 14.14% (4 cm 2 ) compared BHJ devices. Importantly, OSCs also exhibit impressive extrapolated T 80 (the time required reach 80% initial PCE) long‐time storage operational stability, as well thermal stability.

Language: Английский

Citations

Solid Additive Dual‐Regulates Spectral Response Enabling High‐Performance Semitransparent Organic Solar Cells DOI

Xiaopeng Duan,

Yinuo Yang,

Jifa Yu

et al.

Advanced Materials, Journal Year: 2024, Volume and Issue: 36(18)

Published: Jan. 30, 2024

Abstract Semi‐transparent organic solar cells (ST‐OSCs) possess significant potential for applications in vehicles and buildings due to their distinctive visual transparency. Conventional device engineering strategies are typically used optimize photon selection utilization at the expense of power conversion efficiency (PCE); moreover, fixed spectral range always imposes an unsatisfactory upper limit its light (LUE). Herein, a novel solid additive named 1,3‐diphenoxybenzene (DB) is employed dual‐regulate donor/acceptor molecular aggregation crystallinity, which effectively broadens response ST‐OSCs near‐infrared region. Besides, more visible allowed pass through devices, enables satisfactory photocurrent high average transmittance (AVT) simultaneously. Consequently, optimal ST‐OSC based on PP2+DB/BTP‐eC9+DB achieves superior LUE 4.77%, representing highest value within AVT 40–50%, also correlates with formation multi‐scale phase‐separated morphology. Such results indicate that can simultaneously meet requirements minimum commercial plant photosynthesis when integrated roofs agricultural greenhouses. This work emphasizes significance additives tune ST‐OSCs, charts way photovoltaics economically sustainable development.

Language: Английский

Citations

Ameliorated trap density and energetic disorder via a strengthened intermolecular interaction strategy to construct efficient non-halogenated organic solar cells DOI

Shenzheng Gao,

Yimin Zhang, Seonghun Jeong

et al.

Energy & Environmental Science, Journal Year: 2024, Volume and Issue: 17(15), P. 5542 - 5551

Published: Jan. 1, 2024

The efficiency of non-halogenated organic solar cells is improved from 17.1% to 19.4% after dibenzyl ether (DBE) additive treatment. More strikingly, the thick-film devices achieved a champion 17.4%.

Language: Английский

Citations