Macromolecules,
Journal Year:
2024,
Volume and Issue:
57(5), P. 2339 - 2350
Published: Feb. 28, 2024
Polymer
ionic
conductors
have
shown
great
promise
as
iontronic
sensors
for
flexible
wearable
devices
and
intelligent
machines.
A
series
of
exquisitely
designed
hydrogels,
ionogels,
elastomers
good
mechanical
properties,
such
super
stretchability
high
elasticity.
However,
most
gels
tend
to
exhibit
softening
or
linear
mechanoresponsive
behavior
when
subjected
stress,
which
is
completely
different
from
the
strain-stiffening
biological
tissues.
Therefore,
designing
polymer
with
properties
ability
remains
a
challenge,
critical
in
improving
reliability
durability
sensing.
Here,
we
propose
strong/weak
interaction
strategy
develop
poly(ionic
liquid)
(PILEs)
through
copolymerization
imidazolium
liquid
monomers
acrylate
monomers.
The
design
allows
weak
interactions
impart
softness
network,
while
strong
stiffen
network
during
stretching.
resulting
transparent
PILE
possesses
ultrastretchability,
immense
strain
stiffening,
elasticity,
toughness,
puncture
resistance.
also
shows
antibacterial
adhesion
due
high-content
charge
groups
network.
These
combined
make
an
excellent
candidate
sensors,
stability
sensitivity
temperature
strain,
demonstrating
potential
human–machine
interfaces.
Advanced Materials,
Journal Year:
2023,
Volume and Issue:
36(11)
Published: Dec. 14, 2023
Abstract
Self‐adhesive
materials
that
can
directly
adhere
to
diverse
solid
surfaces
are
indispensable
in
modern
life
and
technologies.
However,
it
remains
a
challenge
develop
self‐adhesive
with
strong
adhesion
while
maintaining
its
intrinsic
softness
for
efficient
tackiness.
Here,
peeling–stiffening
ionogel
reconciles
the
seemingly
contradictory
properties
of
is
reported.
The
contains
two
ionophilic
repeating
units
distinct
associating
affinities,
which
allows
adaptively
wet
rough
surface
soft
dissipating
state
adhering,
dramatically
stiffen
glassy
upon
peeling.
corresponding
modulus
increases
by
117
times
driven
strain‐rate‐induced
phase
separation,
greatly
suppresses
crack
propagation
results
super
high
interfacial
toughness
8046
J
m
−2
.
also
transparent,
self‐healable,
recyclable,
be
easily
removed
simple
moisture
treatment.
This
strategy
provides
new
way
design
high‐performance
intelligent
devices.
Advanced Functional Materials,
Journal Year:
2023,
Volume and Issue:
33(41)
Published: Aug. 24, 2023
Abstract
This
study
presents
an
intelligent
soft
robotic
system
capable
of
perceiving,
describing,
and
sorting
objects
based
on
their
physical
properties.
work
introduces
a
bimodal
self‐powered
flexible
sensor
(BSFS)
the
triboelectric
nanogenerator
giant
magnetoelastic
effect.
The
BSFS
features
simplified
structure
comprising
conductive
film
packaged
liquid
metal
coil.
can
precisely
detect
distinguish
touchless
tactile
models,
with
response
time
10
ms.
By
seamlessly
integrating
BSFSs
into
fingers,
this
realizes
anthropomorphic
hand
remarkable
multimodal
perception
capabilities.
signals
provide
valuable
insights
object
shape
material
composition,
while
offer
precise
information
regarding
surface
roughness.
Utilizing
convolutional
neural
network
(CNN),
integrates
all
sensing
information,
resulting
in
that
accurately
describes
properties,
including
materials,
roughness,
shapes,
accuracy
rate
up
to
97%.
may
lay
foundation
for
hardware
general
artificial
intelligence
capacities
interpret
interact
world,
which
also
serves
as
interface
between
robots.
Nano Letters,
Journal Year:
2024,
Volume and Issue:
24(12), P. 3826 - 3834
Published: March 18, 2024
Lightweight,
easily
processed,
and
durable
polymeric
materials
play
a
crucial
role
in
wearable
sensor
devices.
However,
achieving
simultaneously
high
strength
toughness
remains
challenge.
This
study
addresses
this
by
utilizing
an
ion-specific
effect
to
control
crystalline
domains,
enabling
the
fabrication
of
triboelectric
material
with
tunable
mechanical
properties.
The
dense
crystal-domain
cross-linking
enhances
energy
dissipation,
resulting
boasting
both
tensile
(58.0
MPa)
(198.8
MJ
m–3),
alongside
remarkable
416.7%
fracture
elongation
545.0
MPa
modulus.
Leveraging
these
properties,
is
successfully
integrated
into
self-powered
devices,
real-time
feedback
on
human
joint
movement.
work
presents
valuable
strategy
for
overcoming
strength-toughness
trade-off
materials,
paving
way
their
enhanced
applicability
broader
use
diverse
sensing
applications.
ACS Nano,
Journal Year:
2024,
Volume and Issue:
18(14), P. 9980 - 9996
Published: Feb. 22, 2024
Human
hands
are
amazingly
skilled
at
recognizing
and
handling
objects
of
different
sizes
shapes.
To
date,
soft
robots
rarely
demonstrate
autonomy
equivalent
to
that
humans
for
fine
perception
dexterous
operation.
Here,
an
intelligent
robotic
system
with
autonomous
operation
multimodal
ability
is
developed
by
integrating
capacitive
sensors
triboelectric
sensor.
With
distributed
multiple
sensors,
our
robot
can
not
only
sense
memorize
information
but
also
enable
adaptive
grasping
method
positioning
grasp
control,
during
which
the
sensory
be
captured
sensitively
fused
feature
level
crossmodally
objects,
leading
a
highly
enhanced
recognition
capability.
The
proposed
system,
combining
performance
physical
intelligence
biological
systems
(i.e.,
self-adaptive
behavior
perception),
will
greatly
advance
integration
actuators
robotics
in
many
fields.
ACS Nano,
Journal Year:
2024,
Volume and Issue:
18(5), P. 4579 - 4589
Published: Jan. 23, 2024
To
achieve
a
highly
realistic
robot,
closely
mimicking
human
skin
in
terms
of
materials
and
functionality
is
essential.
This
paper
presents
an
all-protein
silk
fibroin
bionic
(SFBS)
that
emulates
both
fast-adapting
(FA)
slow-adapting
(SA)
receptors.
The
mechanically
different
film
hydrogel,
which
exhibited
skin-like
properties,
such
as
stretchability
(>140%),
elasticity,
low
modulus
(<10
kPa),
biocompatibility,
degradability,
were
prepared
through
mesoscopic
reconstruction
engineering
to
mimic
the
epidermis
dermis.
Our
SFBS,
incorporating
SA
FA
sensors,
demonstrated
sensitive
(1.083
kPa–1)
static
pressure
sensing
performance
(in
vitro
vivo),
showed
ability
sense
high-frequency
vibrations
(50–400
Hz),
could
discriminate
sliding,
even
identify
fine
morphological
differences
between
objects.
As
proof
concept,
SFBS-integrated
rehabilitation
glove
was
synthesized,
help
stroke
patients
regain
sensory
feedback.
In
conclusion,
this
work
provides
practical
approach
for
developing
equivalents,
prostheses,
smart
robots.
Nano-Micro Letters,
Journal Year:
2024,
Volume and Issue:
16(1)
Published: July 29, 2024
Abstract
Post-earthquake
rescue
missions
are
full
of
challenges
due
to
the
unstable
structure
ruins
and
successive
aftershocks.
Most
current
robots
lack
ability
interact
with
environments,
leading
low
efficiency.
The
multimodal
electronic
skin
(e-skin)
proposed
not
only
reproduces
pressure,
temperature,
humidity
sensing
capabilities
natural
but
also
develops
functions
beyond
it—perceiving
object
proximity
NO
2
gas.
Its
multilayer
stacked
based
on
Ecoflex
organohydrogel
endows
e-skin
mechanical
properties
similar
skin.
Rescue
integrated
artificial
intelligence
(AI)
algorithms
show
strong
environmental
perception
can
accurately
distinguish
objects
identify
human
limbs
through
grasping,
laying
foundation
for
automated
post-earthquake
rescue.
Besides,
combination
wireless
alarm
circuits
allows
sense
toxic
gases
in
environment
real
time,
thereby
adopting
appropriate
measures
protect
trapped
people
from
environment.
Multimodal
powered
by
AI
hardware
exhibits
powerful
information
processing
capabilities,
which,
as
an
interface
interaction
physical
world,
dramatically
expands
intelligent
robots’
application
scenarios.
Small,
Journal Year:
2024,
Volume and Issue:
20(30)
Published: March 12, 2024
Abstract
Flexible
wearable
sensors
recently
have
made
significant
progress
in
human
motion
detection
and
health
monitoring.
However,
most
still
face
challenges
terms
of
single
targets,
application
environments,
non‐recyclability.
Lipoic
acid
(LA)
shows
a
great
prospect
soft
materials
due
to
its
unique
properties.
Herein,
ionic
conducting
elastomers
(ICEs)
based
on
polymerizable
deep
eutectic
solvents
consisting
LA
choline
chloride
are
prepared.
In
addition
the
good
mechanical
strength,
high
transparency,
conductivity,
self‐healing
efficiency,
ICEs
exhibit
swelling‐strengthening
behavior
enhanced
adhesion
strength
underwater
environments
moisture‐induced
association
poly(LA)
hydrophobic
chains,
thus
making
it
possible
for
sensing
applications,
such
as
communication.
As
strain
sensor,
exhibits
highly
sensitive
response
with
repeatability
durability,
enabling
monitoring
both
large
fine
motions,
including
joint
movements,
facial
expressions,
pulse
waves.
Furthermore,
enhancement
ion
mobility
at
higher
temperatures,
also
possesses
excellent
temperature‐sensing
performance.
Notably,
can
be
fully
recycled
reused
new
strain/temperature
sensor
through
heating.
This
study
provides
novel
strategy
enhancing
fabrication
multifunctional
sensors.
Advanced Materials,
Journal Year:
2024,
Volume and Issue:
unknown
Published: Aug. 11, 2024
Abstract
Electronic
skins
(E‐Skins)
are
crucial
for
future
robotics
and
wearable
devices
to
interact
with
perceive
the
real
world.
Prior
research
faces
challenges
in
achieving
comprehensive
tactile
perception
versatile
functionality
while
keeping
system
simplicity
lack
of
multimodal
sensing
capability
a
single
sensor.
Two
kinds
sensors,
transient
voltage
artificial
neuron
(TVAN)
sustained
potential
(SPAN),
featuring
self‐generated
zero‐biased
signals
developed
realize
synergistic
information
(vibration,
material,
texture,
pressure,
temperature)
device
instead
complex
sensor
arrays.
Simultaneously,
machine
learning
feature
fusion
is
applied
fully
decode
their
output
compensate
inevitable
instability
force,
speed,
etc,
applications.
Integrating
TVAN
SPAN,
formed
E‐Skin
achieves
holistic
touch
awareness
only
unit.
It
can
thoroughly
an
object
through
simple
without
strictly
controlled
testing
conditions,
discern
surface
roughness
from
0.8
1600
µm,
hardness
6HA
85HD,
correctly
distinguish
16
objects
temperature
variance
0
80
°C.
The
E‐skin
also
features
scalable
fabrication
process,
which
be
integrated
into
various
broad