Organogel Polymer Electrocatalysts for Two‐Electron Oxygen Reduction DOI Open Access
Lili Li, Binbin Wang,

Hongni Chen

et al.

Small, Journal Year: 2024, Volume and Issue: unknown

Published: Dec. 20, 2024

Polymer gels, renowned for unparalleled chemical stability and self-sustaining properties, have garnered significant attention in electrocatalysis. Notably, organic polymer gels that exhibit temperature sensitivity incorporate suitable polar nonvolatile liquids, enhance electronic conductivity, impart distinct morphological features, but remain largely unexplored as electrocatalysts oxygen reduction reaction (ORR). To address this issue, an innovative strategy is proposed synergistic modulation of the rigidity mainchain molecular skeleton length alkyl sidechains, enabling development organogel polymers with a sol-gel temperature-sensitive phase transition promises high selectivity enhanced activity electrocatalytic processes. shortening sidechain can significantly affect gelation behavior internal microstructure catalyst, which modifies electron state, ultimately impacting catalytic gel catalysts. In particular, phenyl-containing Ph-FL1 short sidechains demonstrates outstanding 2e

Language: Английский

Organogel Polymer Electrocatalysts for Two‐Electron Oxygen Reduction DOI Open Access
Lili Li, Binbin Wang,

Hongni Chen

et al.

Small, Journal Year: 2024, Volume and Issue: unknown

Published: Dec. 20, 2024

Polymer gels, renowned for unparalleled chemical stability and self-sustaining properties, have garnered significant attention in electrocatalysis. Notably, organic polymer gels that exhibit temperature sensitivity incorporate suitable polar nonvolatile liquids, enhance electronic conductivity, impart distinct morphological features, but remain largely unexplored as electrocatalysts oxygen reduction reaction (ORR). To address this issue, an innovative strategy is proposed synergistic modulation of the rigidity mainchain molecular skeleton length alkyl sidechains, enabling development organogel polymers with a sol-gel temperature-sensitive phase transition promises high selectivity enhanced activity electrocatalytic processes. shortening sidechain can significantly affect gelation behavior internal microstructure catalyst, which modifies electron state, ultimately impacting catalytic gel catalysts. In particular, phenyl-containing Ph-FL1 short sidechains demonstrates outstanding 2e

Language: Английский

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