Eco‐Friendly Self‐Adaptive Catalytic Strategy for Plastics Lifecycles: Achieving Green Preparation, Superior Flame Retardancy, and Self‐Driven Sustainability DOI
Yanan Wu, Haibo Zhao, Ming‐Jun Chen

et al.

Advanced Functional Materials, Journal Year: 2024, Volume and Issue: unknown

Published: Dec. 2, 2024

Abstract Semi‐rigid polyurethane foams (SPUF) with high deformation resistance and strength are indispensable for cushioning applications. However, fire risk cascaded pollutant effects, overused multifarious additives foam wastes exacerbate global environmental concerns. One option to address this issue is develop eco‐friendly multifunctional flame retardants that participate in the material lifecycles of preparation, safe service, waste management, sustainable recycling. Herein, a novel self‐adaptive catalytic strategy reported exploits temperature agent structure‐responsive ability sodium propionate (SP), reconciling often‐conflicting properties fabrication recycling while effectively mitigating combustion risks additive pollution. The adaptive function SP impressively involves all aspects life cycles: 1) catalyzing foaming without complex/hazardous catalysts; 2) providing superior flame‐retardant efficiency limiting oxygen index 25.5% relying on traditional retardants; 3) promoting situ network fragmentation reorganization into strong adhesives (5.8 MPa); 4) further newly formed self‐driven manner. A green presented addresses hazards, plastic pollution, unsustainability recycling, minimizing ecological foam, which will positively impact future design involving diverse additives.

Language: Английский

Selective Recycling of Mixed Polyesters via Heterogeneous Photothermal Catalysis DOI Open Access
Yu Liu,

Penglei Yan,

Xiaodong Li

et al.

Advanced Materials, Journal Year: 2025, Volume and Issue: unknown

Published: Jan. 2, 2025

The selective recycling of mixed plastic wastes with similar structural units is challenging. While heterogeneous catalysis shows potential for recycling, challenges such as complex mass transfer at multiphase interfaces and unclear catalytic mechanisms have slowed progress. In this study, a breakthrough in polyester introduced using photothermal catalysis. By adding co-solvents, the difficulties associated interfacial are overcome. Grain boundary (GB)-rich CeO

Language: Английский

Citations

1

Advanced Catalysts for the Chemical Recycling of Plastic Waste DOI

Jibo Qin,

Feiyan Wu, Yibo Dou

et al.

Advanced Materials, Journal Year: 2025, Volume and Issue: unknown

Published: Jan. 2, 2025

Abstract Plastic products bring convenience to various aspects of the daily lives due their lightweight, durability and versatility, but massive accumulation post‐consumer plastic waste is posing significant environmental challenges. Catalytic methods can effectively convert into value‐added feedstocks, with catalysts playing an important role in regulating yield selectivity products. This review explores latest advancements advanced applied thermal catalysis, microwave‐assisted photocatalysis, electrocatalysis, enzymatic catalysis reaction systems for chemical recycling valuable feedstocks. Specifically, pathways mechanisms involved plastics process are analyzed presented, strengths weaknesses employed across different described. In addition, structure‐function relationship these discussed. Herein, it provided insights design novel outline challenges future opportunities terms developing tackle “white pollution” crisis.

Language: Английский

Citations

1

Pd-doped CoNi-based bifunctional electrodes for upcycling of PET plastic with ultra-long stability DOI

Jinli Fan,

Bincheng Xu, Cheng Chen

et al.

Applied Catalysis B Environment and Energy, Journal Year: 2025, Volume and Issue: unknown, P. 125076 - 125076

Published: Jan. 1, 2025

Language: Английский

Citations

0

Fabrication of High-Strength Waste-Wind-Turbine-Blade-Powder-Reinforced Polypropylene Composite via Solid-State Stretching DOI Open Access
Tan Bo, Xiaotong Wang, Zhilong Pu

et al.

Sustainability, Journal Year: 2025, Volume and Issue: 17(3), P. 840 - 840

Published: Jan. 21, 2025

In recent years, wind energy has emerged as one of the fastest-growing green technologies globally, with projections indicating that decommissioned turbine blades (WTBs) will accumulate to millions tons by 2030s. Due their thermosetting nature and high glass/carbon fiber content, efficient recycling WTBs remains a challenge. this study, we utilized solid-state shear milling (S3M) produce fine WTB powder, which then underwent surface modification silane coupling agent (KH550), subsequently fabricated WTB-reinforced polypropylene (PP) composites enhanced mechanical performance through stretching. The stretching-process-induced orientation PP molecular chains glass fibers led orientation-induced crystallization significant improvements in properties PP/WTB@550 composites. With 30 wt. % composite achieved tensile strength 142.61 MPa Young’s modulus 3991.19 at stretching temperature 110 °C ratio 3, representing increases 268% 471%, respectively, compared unstretched sample. This work offers both theoretical insights experimental evidence supporting high-value reuse cost-effective, environmentally friendly, scalable approach. PP/WTB intrinsic waterproofing corrosion resistance PP, it is hoped such would be used road engineering building materials, geogrids, wall panels, floor boards, tiles.

Language: Английский

Citations

0

Sustainable thermochemical plastic valorization towards a circular economy: a critical review DOI
Liang Chen,

Can Zhao,

Xiangzhou Yuan

et al.

Green Chemistry, Journal Year: 2025, Volume and Issue: unknown

Published: Jan. 1, 2025

Emerging technologies-empowered thermochemical plastic valorization is developed for value-added products in green and practical manner, which are beneficial to achieving circular economy several UN sustainable development goals.

Language: Английский

Citations

0

Carbon Fiber Reinforced Thermoplastics: From Materials to Manufacturing and Applications DOI Creative Commons
Howard Wang, Siqi Huo, Venkata S. Chevali

et al.

Advanced Materials, Journal Year: 2025, Volume and Issue: unknown

Published: April 22, 2025

Abstract Carbon fiber reinforced thermoplastics (CFRTs) have witnessed a resurgence in recent times since their first industrial use over five decades ago, with revitalized interest from aerospace companies and other key sectors including energy automotive sectors. CFRTs are increasingly gaining footholds high volume rapid manufacturing nonaerospace owing to inherent recyclability. However, there has been lack of contemporary critical review on this topic so far. This work aims the advances emphasis performance thermoplastics. Both continuous discontinuous forms tape, organosheet short/long architectures discussed, processing postprocessing methods reviewed, state‐of‐the‐art welding techniques. Typical applications industry examined, fuselage, pressure vessel, components. Finally, insights provided into ongoing challenges, future development, roadmap for expediting development high‐performance CFRTs.

Language: Английский

Citations

0

Linear and Network-Forming Acetal Polymerization of Multifunctional Alcohols with Dichloromethane for Degradable and Recyclable Materials DOI
Joshua T. Kamps, Bruce E. Kirkpatrick, Sean P. Keyser

et al.

Macromolecules, Journal Year: 2025, Volume and Issue: unknown

Published: Jan. 29, 2025

Language: Английский

Citations

0

Upcycling wind turbine blades into durable Super-Hydrophobic coating for High-Efficiency Anti-Icing application DOI
Dawei Luo, Dali Gao, Nan Cheng

et al.

Chemical Engineering Journal, Journal Year: 2025, Volume and Issue: unknown, P. 160323 - 160323

Published: Feb. 1, 2025

Language: Английский

Citations

0

A Review of Hawaii and Plastic Pollution: Potential Innovations within Circular Economy? DOI
Prisca Ayassamy

Environmental Management, Journal Year: 2025, Volume and Issue: unknown

Published: March 10, 2025

Language: Английский

Citations

0

Recent advances in recycling and upcycling of hazardous plastic waste: A review DOI

Shahrani Anuar,

Abu Hassan Nordin, Siti Muhamad Nur Husna

et al.

Journal of Environmental Management, Journal Year: 2025, Volume and Issue: 380, P. 124867 - 124867

Published: March 12, 2025

Language: Английский

Citations

0