Molecular Regulation and Intermolecular Chemistry in Gel Polymer Electrolytes for High‐Voltage Lithium Batteries DOI Creative Commons
Qingjie Zhou,

Mengxue He,

Shuyang Gao

et al.

Advanced Science, Journal Year: 2025, Volume and Issue: unknown

Published: April 9, 2025

Abstract Gel polymer electrolyte (GPE) has garnered widespread attention in the field of lithium batteries because its low interfacial impedance, high thermal stability, and flexibility. However, high‐voltage compatibility Li + transport kinetics GPE have yet to meet requirements future high‐energy secondary battery systems. In this regard, a comprehensive insightful review with attracted significant attention, focusing on molecular design intermolecular interactions. Molecular regulation involves customizing matrix, solvent, additive, salt, while interactions encompass hydrogen bond interactions, Lewis acid‐base electrostatic π–π stacking Besides, strategies enhance stability cathode interphase are summarized. It is hoped that will provide deeper understanding direct at level, further accelerating commercialization batteries.

Language: Английский

Molecular Regulation and Intermolecular Chemistry in Gel Polymer Electrolytes for High‐Voltage Lithium Batteries DOI Creative Commons
Qingjie Zhou,

Mengxue He,

Shuyang Gao

et al.

Advanced Science, Journal Year: 2025, Volume and Issue: unknown

Published: April 9, 2025

Abstract Gel polymer electrolyte (GPE) has garnered widespread attention in the field of lithium batteries because its low interfacial impedance, high thermal stability, and flexibility. However, high‐voltage compatibility Li + transport kinetics GPE have yet to meet requirements future high‐energy secondary battery systems. In this regard, a comprehensive insightful review with attracted significant attention, focusing on molecular design intermolecular interactions. Molecular regulation involves customizing matrix, solvent, additive, salt, while interactions encompass hydrogen bond interactions, Lewis acid‐base electrostatic π–π stacking Besides, strategies enhance stability cathode interphase are summarized. It is hoped that will provide deeper understanding direct at level, further accelerating commercialization batteries.

Language: Английский

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