Applied Catalysis B Environment and Energy, Journal Year: 2024, Volume and Issue: unknown, P. 124990 - 124990
Published: Dec. 1, 2024
Language: Английский
Applied Catalysis B Environment and Energy, Journal Year: 2024, Volume and Issue: unknown, P. 124990 - 124990
Published: Dec. 1, 2024
Language: Английский
Advanced Science, Journal Year: 2024, Volume and Issue: 11(39)
Published: Aug. 19, 2024
Abstract Single‐atom catalysts (SACs) with edge‐located metal active sites exhibit superior oxygen reduction reaction (ORR) performance due to their narrower energy gap and higher electron density. However, controllably designing such fully reveal advantages remains challenging. Herein, rich Fe‐N 4 anchored in hierarchically porous carbon nanofibers (denoted as e 1 ‐Fe‐N‐C) are fabricated via an situ zinc‐assisted thermal etching strategy. The ‐Fe‐N‐C catalyst demonstrates alkaline ORR activity compared counterparts fewer commercial Pt/C. Density functional theory calculations show that the accumulation of more negative charges near formation partially reduced Fe state reduce barrier for process. Additionally, unique structures mesopores macropores facilitate full utilization enhance long‐range mass transfer. zinc–air battery (ZAB) assembled has a peak power density 198.9 mW cm −2 , Pt/C (152.3 ). present strategy by facile controlling amount zinc acetate template systematically superiority sites, providing new design avenue rational defect engineering achieve high‐performance ORR.
Language: Английский
Citations
6Applied Surface Science, Journal Year: 2025, Volume and Issue: 688, P. 162369 - 162369
Published: Jan. 11, 2025
Language: Английский
Citations
0Journal of Alloys and Compounds, Journal Year: 2025, Volume and Issue: unknown, P. 179737 - 179737
Published: March 1, 2025
Language: Английский
Citations
0Applied Catalysis B Environment and Energy, Journal Year: 2025, Volume and Issue: 367, P. 125116 - 125116
Published: Feb. 2, 2025
Language: Английский
Citations
0Journal of Colloid and Interface Science, Journal Year: 2025, Volume and Issue: 693, P. 137620 - 137620
Published: April 16, 2025
Language: Английский
Citations
0Applied Catalysis B Environment and Energy, Journal Year: 2024, Volume and Issue: unknown, P. 124990 - 124990
Published: Dec. 1, 2024
Language: Английский
Citations
0