Trends in biotechnology, Journal Year: 2022, Volume and Issue: 40(8), P. 974 - 986
Published: Feb. 22, 2022
Language: Английский
Chemical Reviews, Journal Year: 2022, Volume and Issue: 123(5), P. 2349 - 2419
Published: Dec. 13, 2022
Recent advances in synthetic biology and materials science have given rise to a new form of materials, namely engineered living (ELMs), which are composed matter or cell communities embedded self-regenerating matrices their own artificial scaffolds. Like natural such as bone, wood, skin, ELMs, possess the functional capabilities organisms, can grow, self-organize, self-repair when needed. They also spontaneously perform programmed biological functions upon sensing external cues. Currently, ELMs show promise for green energy production, bioremediation, disease treatment, fabricating advanced smart materials. This review first introduces dynamic features systems potential developing novel We then summarize recent research progress on emerging design strategies from both perspectives. Finally, we discuss positive impacts promoting sustainability key future directions.
Language: Английский
Citations
118
Journal of the American Chemical Society, Journal Year: 2022, Volume and Issue: 144(14), P. 6434 - 6441
Published: April 4, 2022
The biotic–abiotic photosynthetic system integrating inorganic light absorbers with whole-cell biocatalysts innovates the way for sustainable solar-driven chemical transformation. Fundamentally, electron transfer at interface, which may induce biological response to photoexcited stimuli, plays an essential role in solar energy conversion. Herein, we selected electro-active bacterium Shewanella oneidensis MR-1 as a model, constitutes hybrid self-assembled CdS semiconductor, demonstrate unique interfacial behavior. electrons from nanoparticles can reverse extracellular (EET) chain within S. MR-1, realizing activation of bacterial catalytic network illumination. As compared bare significant upregulation hydrogen yield (711-fold), ATP, and reducing equivalent (NADH/NAD+) was achieved MR-1-CdS under visible light. This work sheds on fundamental mechanism provides design guidelines systems.
Language: Английский
Citations
80
Chemical Society Reviews, Journal Year: 2023, Volume and Issue: 53(3), P. 1375 - 1446
Published: Dec. 20, 2023
The excessive consumption of fossil fuels causes massive emission CO
Language: Английский
Citations
43
Coordination Chemistry Reviews, Journal Year: 2023, Volume and Issue: 494, P. 215272 - 215272
Published: July 17, 2023
Language: Английский
Citations
41
Chemical Reviews, Journal Year: 2024, Volume and Issue: 124(15), P. 9081 - 9112
Published: June 20, 2024
Nanomaterial-microorganism hybrid systems (NMHSs), integrating semiconductor nanomaterials with microorganisms, present a promising platform for broadband solar energy harvesting, high-efficiency carbon reduction, and sustainable chemical production. While studies underscore its potential in diverse solar-to-chemical conversions, prevailing NMHSs grapple suboptimal conversion efficiency. Such limitations stem predominantly from an insufficient systematic exploration of the mechanisms dictating flow. This review provides overview notable advancements this nascent field, particular focus on discussion three pivotal steps flow: capture, cross-membrane transport, into chemicals. key challenges faced each stage are independently identified discussed, viable solutions correspondingly postulated. In view interplay affecting overall efficiency conversion, subsequent discussions thus take integrative viewpoint to comprehend, analyze improve flow current different configurations, highlighting contemporary techniques that can be employed investigate various aspects within NMHSs. Finally, concluding section summarizes opportunities future research, providing roadmap continued development optimization
Language: Английский
Citations
20
Applied Catalysis B Environment and Energy, Journal Year: 2021, Volume and Issue: 301, P. 120755 - 120755
Published: Sept. 29, 2021
Language: Английский
Citations
93
Energy & Environmental Science, Journal Year: 2021, Volume and Issue: 15(2), P. 529 - 549
Published: Dec. 17, 2021
This review comprehensively elaborates the modes of semi-artificial photosynthetic systems (SAPSs) based on different combinations photosensitizers and catalytic centers for energy environmental application.
Language: Английский
Citations
57
International Journal of Hydrogen Energy, Journal Year: 2022, Volume and Issue: 47(27), P. 13340 - 13350
Published: March 1, 2022
Language: Английский
Citations
53
Renewable and Sustainable Energy Reviews, Journal Year: 2023, Volume and Issue: 178, P. 113271 - 113271
Published: March 21, 2023
Language: Английский
Citations
27
ACS Applied Materials & Interfaces, Journal Year: 2023, Volume and Issue: 15(5), P. 6235 - 6259
Published: Jan. 26, 2023
By simulating natural photosynthesis, the desirable high-value chemical products and clean fuels can be sustainably generated with solar energy. Whole-cell-based photosensitized biohybrid system, which innovatively couples excellent light-harvesting capacity of semiconductor materials efficient catalytic ability intracellular biocatalysts, is an appealing interdisciplinary creature to realize photodriven synthesis. In this review, we summarize constructed whole-cell-based systems in different application fields, including carbon dioxide fixation, nitrogen hydrogen production, other Moreover, elaborate charge transfer mechanism studies representative biohybrids, help deepen current understanding synergistic process between photosensitizers microorganisms, provide schemes for building novel biohybrids less electron resistance, advanced productive efficiency, functional diversity. Further exploration field has prospect making a breakthrough on biotic–abiotic interface that will opportunities multidisciplinary research.
Language: Английский
Citations
23