Rapid advances enabling high-performance inverted perovskite solar cells

Nature Reviews Materials, Journal Year: 2024, Volume and Issue: 9(6), P. 399 - 419

Published: May 17, 2024

Language: Английский

---

Optimizing Crystallization in Wide‐Bandgap Mixed Halide Perovskites for High‐Efficiency Solar Cells

Advanced Materials, Journal Year: 2023, Volume and Issue: 36(17)

Published: Sept. 7, 2023

Wide-bandgap (WBG) perovskites have attracted considerable attention due to their adjustable bandgap properties, making them ideal candidates for top subcells in tandem solar cells (TSCs). However, WBG often face challenges such as inhomogeneous crystallization and severe nonradiative recombination loss, leading high open-circuit voltage (V

Language: Английский

---

Triple-junction solar cells with cyanate in ultrawide-bandgap perovskites

Nature, Journal Year: 2024, Volume and Issue: 628(8007), P. 306 - 312

Published: March 4, 2024

Language: Английский

---

Mixed‐Halide Inorganic Perovskite Solar Cells: Opportunities and Challenges

Advanced Optical Materials, Journal Year: 2023, Volume and Issue: 11(20)

Published: Aug. 23, 2023

Abstract Recently, mixed‐halide inorganic CsPbI 3− x Br perovskite solar cells (PSCs) have had a rapid advancement, which offers balanced efficiency, stability, tunable bandgap, and potential for indoor photovoltaic applications. Despite these advantages, significant challenges remain in the phase segregation phenomena, trap state density, absorption range limitations. This review presents an analysis of crystal electronic structure optical properties , as well in‐depth look at high‐quality film preparation, inhibition solutions, interface engineering, highlighting critical role modification performance PSCs. Furthermore, how PSCs can be strong candidates photovoltaics because their adjustable bandgap that enables them to better match notable strength stability is discussed. Finally, provides perspectives address development bottlenecks inspires future research prospects concerning

Language: Английский

---

Highly Efficient Perovskite/Organic Tandem Solar Cells Enabled by Mixed‐Cation Surface Modulation

Advanced Materials, Journal Year: 2023, Volume and Issue: 35(49)

Published: Aug. 7, 2023

Perovskite/organic tandem solar cells (POTSCs) are gaining attention due to their easy fabrication, potential surpass the S-Q limit, and superior flexibility. However, low power conversion efficiencies (PCEs) of wide bandgap (Eg) perovskite (PVSCs) have hindered development. This work presents a novel effective mixed-cation passivation strategy (CE) passivate various types traps in wide-Eg perovskite. The complementary effect 4-trifluoro phenethylammonium (CF3 -PEA+ , denoted as CA+ ) ethylenediammonium (EDA2+ EA2+ reduces both electron/hole defect densities non-radiative recombination rate, resulting record open-circuit voltage (Voc PVSCs (1.35 V) high fill factor (FF) 83.29%. These improvements lead PCE 24.47% when applied fabricated POTSCs, highest date. Furthermore, unencapsulated POTSCs exhibit excellent photo thermal stability, retaining over 90% initial after maximum point (MPP) tracking or exposure 60 °C for 500 h. findings imply that synergic surface passivators is promising achieve high-efficiency stable corresponding POTSCs.

Language: Английский

---

Suppressing Halide Segregation via Pyridine‐Derivative Isomers Enables Efficient 1.68 eV Bandgap Perovskite Solar Cells

Advanced Materials, Journal Year: 2024, Volume and Issue: 36(21)

Published: Feb. 24, 2024

Light-induced phase segregation is one of the main issues restricting efficiency and stability wide-bandgap perovskite solar cells (WBG PSCs). Small organic molecules with abundant functional groups can passivate various defects, therefore suppress ionic migration channels for segregation. Herein, a series pyridine-derivative isomers containing amino carboxyl are applied to modify surface. The amino, carboxyl, N-terminal pyridine in all these interact undercoordinated Pb

Language: Английский

---

The physical attributes of rubidium-based Rb2TlRhF6 double perovskite halide: A first-principles investigation

Physica B Condensed Matter, Journal Year: 2024, Volume and Issue: 685, P. 416000 - 416000

Published: April 22, 2024

Language: Английский

---

Overcoming Phase Segregation in Wide‐Bandgap Perovskites: from Progress to Perspective

Advanced Functional Materials, Journal Year: 2024, Volume and Issue: unknown

Published: May 25, 2024

Abstract Wide‐bandgap (WBG) perovskite solar cells (PSCs) are recognized as promising candidates for diversified photovoltaics (PVs), such tandem devices, indoor PVs, and semitransparent building‐integrated PVs. However, these WBG perovskites made from a mixed‐halides strategy suffer severe phase segregation under continuous illumination, leading to exacerbated non‐radiative recombination, consequently decreased open‐circuit voltage efficiency. In this review, the generation reversal processes of in meticulously introduced. Additionally, major characterization techniques presented. A detailed summary recent progress enhancing photostability PSCs through various strategies is provided. These primarily concentrate on composition regulation, crystallization modulation, inhibition ion migration, strain regulation. Finally, perspectives potential directions carefully discussed promote further development high‐efficiency photostable PSCs.

Language: Английский

---

A review of chalcogenide-based perovskites as the next novel materials: Solar cell and optoelectronic applications, catalysis and future perspectives

Next Nanotechnology, Journal Year: 2024, Volume and Issue: 7, P. 100102 - 100102

Published: Sept. 11, 2024

Language: Английский

---

A review of interface engineering characteristics for high performance perovskite solar cells

Deleted Journal, Journal Year: 2024, Volume and Issue: 2, P. 100005 - 100005

Published: April 25, 2024

Language: Английский

---