Journal of environmental chemical engineering, Journal Year: 2024, Volume and Issue: 13(1), P. 115058 - 115058
Published: Dec. 8, 2024
Language: Английский
Journal of environmental chemical engineering, Journal Year: 2024, Volume and Issue: 13(1), P. 115058 - 115058
Published: Dec. 8, 2024
Language: Английский
Advanced Functional Materials, Journal Year: 2024, Volume and Issue: unknown
Published: Dec. 26, 2024
Abstract Returning CO 2 to liquid ethanol powered by clean energy offers considerable economic benefits and contributes reaching the goal of carbon neutrality, but it remains a formidable challenge achieve high selectivity due inevitable strong competition among various pathways. Herein, an investigation is presented accelerate electroreduction via preferentially stabilizing precarious watershed intermediates ( * CHCOH) creating adsorbate‐adsorbate interaction. The highly ordered CuOx nanoplates (HO‐CuOx NPLs) featuring abundant amorphous‐crystalline interface exhibit exceptional Faradaic efficiency (FE EtOH ) 63.8% ethanol‐to‐ethylene ratio 6.1 at large partial current density j 232.8 mA cm −2 . findings decipher that in‐between nanogaps in enhance adsorption OH, which can strengthen C─O bonds while weakening Cu─C interaction CHCOH through interaction, thereby enabling predilection for conversion. Beyond efficient ethanol‐oriented RR electrocatalyst, investigations provide in‐depth understanding on key steps precise regulation, be extended range conversion technologies.
Language: Английский
Citations
2Journal of Energy Chemistry, Journal Year: 2024, Volume and Issue: unknown
Published: Oct. 1, 2024
Language: Английский
Citations
1Journal of Colloid and Interface Science, Journal Year: 2024, Volume and Issue: 679, P. 50 - 59
Published: Oct. 18, 2024
Language: Английский
Citations
0Journal of environmental chemical engineering, Journal Year: 2024, Volume and Issue: 13(1), P. 115058 - 115058
Published: Dec. 8, 2024
Language: Английский
Citations
0