Optimization Strategies for Electrocatalytic CO2 Reduction Based on Atomically Dispersed Copper: A Review DOI
Yuan Li, Bin Guan, Zhongqi Zhuang

et al.

Advanced Functional Materials, Journal Year: 2024, Volume and Issue: unknown

Published: Dec. 26, 2024

Abstract The electroreduction reaction of CO 2 (eCO RR) is considered an effective pathway for clean fuel production, greenhouse gas reduction, and resource recycling. Atomically dispersed catalysts exhibit excellent catalytic activity due to the high dispersion atoms, especially atomically copper (AD Cu). Although copper‐based materials are major single component capable producing multi‐carbon products, mechanism usually not very clear. For AD Cu catalysts, dynamic transformation species in form (nano)clusters, ions during process significantly has effect on performance eCO RR. core issue that needs be addressed how control tune aggregation atoms make it most favorable desired product or pathways. This review summarizes optimization strategies recent years from three main perspectives: interface engineering, electrode external field coupling.

Language: Английский

Cu−based bimetallic sites' p-d orbital hybridization promotes CO asymmetric coupling conversion to C2 products DOI
Jiayong Xiao, Jofrey J. Masana, Ming Qiu

et al.

Materials Today Physics, Journal Year: 2024, Volume and Issue: 48, P. 101565 - 101565

Published: Oct. 10, 2024

Language: Английский

Citations

0
Optimization Strategies for Electrocatalytic CO2 Reduction Based on Atomically Dispersed Copper: A Review DOI
Yuan Li, Bin Guan, Zhongqi Zhuang

et al.

Advanced Functional Materials, Journal Year: 2024, Volume and Issue: unknown

Published: Dec. 26, 2024

Abstract The electroreduction reaction of CO 2 (eCO RR) is considered an effective pathway for clean fuel production, greenhouse gas reduction, and resource recycling. Atomically dispersed catalysts exhibit excellent catalytic activity due to the high dispersion atoms, especially atomically copper (AD Cu). Although copper‐based materials are major single component capable producing multi‐carbon products, mechanism usually not very clear. For AD Cu catalysts, dynamic transformation species in form (nano)clusters, ions during process significantly has effect on performance eCO RR. core issue that needs be addressed how control tune aggregation atoms make it most favorable desired product or pathways. This review summarizes optimization strategies recent years from three main perspectives: interface engineering, electrode external field coupling.

Language: Английский

Citations

0