Mesogenic Unit based Low Melting Point Solid Additive for Efficient and Stable Organic Solar Cells DOI
Jiali Wang, Qian Xie, Jie Fang

et al.

Journal of Materials Chemistry C, Journal Year: 2024, Volume and Issue: 13(5), P. 2183 - 2189

Published: Dec. 3, 2024

In this work, a novel low melting temperature solid additive CB8-Br was designed and synthesized through simple reliable method, superior PCE of 18.12% with excellent device stability obtained in CB8-Br-processed devices.

Language: Английский

Rational Design of Terpolymer Acceptors for High-Efficiency All-Polymer Solar Cells DOI
Jiawei Huang,

Xintong Shi,

Xiaoping Wang

et al.

Chemical Communications, Journal Year: 2025, Volume and Issue: unknown

Published: Jan. 1, 2025

Three terpolymers were developed via a ternary polymerization strategy. Owing to appropriate aggregation behavior and improved compatibility, the J2-based all polymer device offers an excellent power conversion efficiency up 16.5%.

Language: Английский

Citations

0

Flexible Spacer Units Enhance 3D Terpolymer Acceptors’ Optoelectronic Performance in Rigid and Flexible Devices DOI

Xiaoping Wang,

Yu Fang,

Bin Huang

et al.

Macromolecules, Journal Year: 2025, Volume and Issue: unknown

Published: March 9, 2025

Language: Английский

Citations

0

Enhancing the Electrostatic Potential To Develop High-Performance Polymer Donors via a Ternary Copolymerization Strategy DOI

Xintong Shi,

Jiawei Huang,

Xiaoping Wang

et al.

ACS Applied Materials & Interfaces, Journal Year: 2025, Volume and Issue: unknown

Published: April 10, 2025

Ternary copolymerization has been proven to be an effective method regulate the photovoltaic properties of polymer donors. However, terpolymers synthesized using ternary strategy inevitably disrupt periodic sequence distribution backbone, resulting in increased molecular disorder and heightened main-chain entropy. Herein, we developed two terpolymer donors by introducing electron-deficient fused-ring skeleton unit BTP with a large dipole moment into main chain PM6 via copolymerization. We found that presence enables exhibit enhanced crystallinity electrostatic potential, leading excellent miscibility more ordered packing than PM6. As result, maximum PCE 19.40% was achieved for PY5:L8-BO-based device. Overall, this work introduces novel approach developing high-performance combining third component moments restrain enhance intermolecular interaction force between acceptors.

Language: Английский

Citations

0

Binary all-polymer solar cells with 19.30% efficiency enabled by bromodibenzothiophene-based solid additive DOI

Haisheng Ma,

Jiali Song,

Jiawei Qiao

et al.

Energy & Environmental Science, Journal Year: 2024, Volume and Issue: unknown

Published: Nov. 15, 2024

Two volatile solid additives were developed to modulate the active-layer morphology of all-polymer solar cells (all-PSCs). Among them, 4-BDBTP-treated all-PSC achieved an outstanding efficiency 19.30%.

Language: Английский

Citations

3

Mesogenic Unit based Low Melting Point Solid Additive for Efficient and Stable Organic Solar Cells DOI
Jiali Wang, Qian Xie, Jie Fang

et al.

Journal of Materials Chemistry C, Journal Year: 2024, Volume and Issue: 13(5), P. 2183 - 2189

Published: Dec. 3, 2024

In this work, a novel low melting temperature solid additive CB8-Br was designed and synthesized through simple reliable method, superior PCE of 18.12% with excellent device stability obtained in CB8-Br-processed devices.

Language: Английский

Citations

0