S-Scheme Heterojunction ZnCdS Nanoparticles on Layered Ni–Co Hydroxide for Photocatalytic Hydrogen Evolution DOI
Bo Wen, Xin Guo, Yafeng Liu

et al.

ACS Applied Nano Materials, Journal Year: 2024, Volume and Issue: 7(6), P. 6056 - 6067

Published: March 1, 2024

Photocatalytic hydrogen evolution technology faces great challenges in designing efficient and stable catalysts that absorb visible light. In this study, a catalyst with S-scheme heterojunction built-in electric fields was successfully prepared by electrostatic self-assembly to load ZnCdS nanoparticles on layered Ni–Co. The ZnCdS/NiCo double hydroxide (NiCo-LDH) test demonstrates the effectively inhibit recombination of photogenerated electrons holes, lowering impedance increasing photocurrent. Additionally, more can take part reduction reaction, producing H2. It is worth noting ZnCdS/NiCo-LDH 1153 μmol 5 h, which 10 times ZnCdS. We analyze electron transport process, construction field, formation during situ X-ray photoelectron spectroscopy. This study provides new perspective for application LDH photocatalysis direction breakthrough photocatalytic research.

Language: Английский

Hollow dodecahedron K3PW12O40/CdS core-shell S-scheme heterojunction for photocatalytic synergistic H2 evolution and benzyl alcohol oxidation DOI
Lijuan Sun, Xiaohui Yu,

Liyong Tang

et al.

CHINESE JOURNAL OF CATALYSIS (CHINESE VERSION), Journal Year: 2023, Volume and Issue: 52, P. 164 - 175

Published: Sept. 1, 2023

Language: Английский

Citations

104

Solvent Engineering of Oxygen‐Enriched Carbon Dots for Efficient Electrochemical Hydrogen Peroxide Production DOI
Xiaoyu Shen, Zeming Wang, Huazhang Guo

et al.

Small, Journal Year: 2023, Volume and Issue: 19(43)

Published: June 27, 2023

The development of cost-effective and reliable metal-free carbon-based electrocatalysts has gained significant attention for electrochemical hydrogen peroxide (H2 O2 ) generation through a two-electron oxygen reduction reaction. In this study, scalable solvent engineering strategy is employed to fabricate oxygen-doped carbon dots (O-CDs) that exhibit excellent performance as electrocatalysts. By adjusting the ratio ethanol acetone solvents during synthesis, surface electronic structure resulting O-CDs can be systematically tuned. amount edge active CO group was strongly correlated with selectivity activity O-CDs. optimum O-CDs-3 exhibited extraordinary H2 up 96.55% (n = 2.06) at 0.65 V (vs RHE) achieved remarkably low Tafel plot 64.8 mV dec-1 . Furthermore, realistic productivity yield flow cell measured high 111.18 mg h-1 cm-2 duration 10 h. findings highlight potential universal approach enabling electrocatalytic materials improved performance. Further studies will undertaken explore practical implications advancing field electrocatalysis.

Language: Английский

Citations

71

Challenges in photocatalytic hydrogen evolution: Importance of photocatalysts and photocatalytic reactors DOI Creative Commons

Abhishek Burri,

A. Jayarama,

Arjun Sunil Rao

et al.

International Journal of Hydrogen Energy, Journal Year: 2024, Volume and Issue: 81, P. 1442 - 1466

Published: Aug. 5, 2024

Language: Английский

Citations

45

Atomic-level coordination structures meet graphitic carbon nitride (g-C3N4) for photocatalysis: Energy conversion and environmental remediation DOI

Haiwei Su,

Haibo Yin, Rong Wang

et al.

Applied Catalysis B Environment and Energy, Journal Year: 2024, Volume and Issue: unknown, P. 123683 - 123683

Published: Jan. 1, 2024

Language: Английский

Citations

42

Strategically designing and fabricating nitrogen and sulfur Co-doped g-C3N4 for accelerating photocatalytic H2 evolution DOI
Haitao Wang,

Lianglang Yu,

Jiahe Peng

et al.

Journal of Material Science and Technology, Journal Year: 2024, Volume and Issue: 208, P. 111 - 119

Published: May 17, 2024

Language: Английский

Citations

29

Application of graphdiyne for promote efficient photocatalytic hydrogen evolution DOI Creative Commons
Tian Wang, Zhiliang Jin

Results in Surfaces and Interfaces, Journal Year: 2024, Volume and Issue: 14, P. 100188 - 100188

Published: Jan. 23, 2024

The photocatalytic hydrogen evolution technology converts solar energy into clean and environmentally friendly energy, which is considered an effective means to solve environmental pollution crisis. unique sp sp2 hybrid carbon network structure of graphdiyne endows it with excellent carrier mobility, high porosity, making a promising material for conversion. This article provides detailed description the structural properties adjustable bandgap graphdiyne. In addition, review was provided on modification strategies based catalysts evolution, including titanium photocatalysts, metal oxide double hydroxide catalysts, organic framework photocatalysts other typical semiconductors. Finally, challenges opportunities developing semiconductors water splitting were proposed. Timely expected contribute rapid development in field evolution.

Language: Английский

Citations

28

Recent Progress of Quantum Dots Light‐Emitting Diodes: Materials, Device Structures, and Display Applications DOI
Junpeng Fan, Changfeng Han, Guojian Yang

et al.

Advanced Materials, Journal Year: 2024, Volume and Issue: 36(37)

Published: May 30, 2024

Abstract Colloidal quantum dots (QDs), as a class of 0D semiconductor materials, have generated widespread interest due to their adjustable band gap, exceptional color purity, near‐unity yield, and solution‐processability. With decades dedicated research, the potential applications garnered significant recognition in both academic industrial communities. Furthermore, related dot light‐emitting diodes (QLEDs) stand out one most promising contenders for next‐generation display technologies. Although QD‐based conversion films are applied improve gamut existing technologies, broader application QLED devices remains its nascent stages, facing many challenges on path commercialization. This review encapsulates historical discovery subsequent research advancements QD materials synthesis methods. Additionally, working mechanisms architectural design prototype discussed. surveys latest within industry. The narrative concludes with an examination perspectives technology foreseeable future.

Language: Английский

Citations

22

Programmed Transformation of Osteogenesis Microenvironment by a Multifunctional Hydrogel to Enhance Repair of Infectious Bone Defects DOI Creative Commons
En Xie,

Zhangqin Yuan,

Qianglong Chen

et al.

Advanced Science, Journal Year: 2025, Volume and Issue: unknown

Published: Jan. 22, 2025

Abstract Repair of infectious bone defects remains a serious problem in clinical practice owing to the high risk infection and excessive reactive oxygen species (ROS) during early stage, residual bacteria delayed Osseo integrated interface later which jointly creates complex dynamic microenvironment leads non‐union. The melatonin carbon dots (MCDs) possess antibacterial osteogenesis abilities, greatly simplifying composition multifunctional material. Therefore, hydrogel containing MCDs (GH‐MCD) is developed meet multi‐stage repair needs injury this study. GH‐MCD can intelligently release responding acidic scavenge intracellular ROS exhibit good activity by inducing production inhibiting expression secA2 . Moreover, it has long‐lasting antimicrobial repair. RNA‐seq results reveal that hydrogels promote infected healing enhancing cellular resistance bacteria, balancing osteoclastogenesis, regulating immune microenvironment. In conclusion, through programmed transformation microenvironment, providing novel strategy for defects.

Language: Английский

Citations

2

An S-scheme heterointerface-engineered high-performance ternary NiAl-LDH@TiO2/Ti3C2 MXene photocatalytic system for solar-powered CO2 reduction to produce energy-rich fuels DOI
Dong‐Eun Lee, Devthade Vidyasagar, B. Moses Abraham

et al.

Chemical Engineering Journal, Journal Year: 2023, Volume and Issue: 480, P. 148227 - 148227

Published: Dec. 22, 2023

Language: Английский

Citations

27

Current trends in environmental and energy photocatalysis and ISO standardization DOI
Hassan Ali, Milan Masař, Muhammad Yasir

et al.

Journal of environmental chemical engineering, Journal Year: 2023, Volume and Issue: 11(6), P. 111541 - 111541

Published: Nov. 23, 2023

Language: Английский

Citations

25