Stimuli‐Responsive Optical Materials Based on Hypervalent Antimony‐Containing Conjugated Molecules DOI Open Access
Kazuya Tanimura, Masayuki Gon, Kazuo Tanaka

et al.

Advanced Functional Materials, Journal Year: 2024, Volume and Issue: unknown

Published: Nov. 17, 2024

Abstract Stimuli‐responsive materials have been applied for sensor devices because they can transform and amplify various target stimuli into observable signals. Much effort has devoted to exploring effective molecular designs obtaining stimuli‐responsive behaviors by taking advantage of the unique optoelectronic properties π‐conjugated molecules involving elements. This study focuses on modulation electronic state scaffolds oxidation number change hypervalent antimony. demonstrate that strength intramolecular interaction between antimony framework be tuned with ligand structure, substituent effect, shifts In particular, color changes represented hypsochromic bathochromic wavelength optical bands are achieved oxidative reaction in solid state. Significantly, direction confidently predicted quantum chemical calculations. The findings, based main‐group elements, provide logical design strategies advanced materials.

Language: Английский

Applications of Luminescent Cyclometalated Metal Complexes as Sensors and Switches DOI
Poonam Kaswan, Miklesh Prasad Yadav,

Shaila Dhotre

et al.

Synlett, Journal Year: 2025, Volume and Issue: unknown

Published: March 19, 2025

Abstract Cyclometalated complexes, including those with pincer ligands and other chelating frameworks, such as porphyrin rings polyenes, have garnered significant attention due to their diverse applications in ion analyte detection across synthetic chemistry, environmental monitoring, medicine, electronics. These complexes exhibit fascinating chromic behaviors, mechanochromism, chemochromism, vapochromism, which are particularly useful sensing applications. Of particular interest photophysical properties, especially involving lanthanides, offer unique luminescent optical characteristics. Metals nickel (Ni), palladium (Pd), ruthenium (Ru), gold (Au), rhodium (Rh) been extensively studied order understand photochemical activity explore potential light-emitting devices, photo-induced electron transfer, technologies. Their vapochromic mechanochromic properties make them highly attractive for sensing, while photoluminescent capabilities enhance utility optoelectronic devices practical This review provides a comprehensive overview of applications, gas, cation, anion sensing. The discussion also highlights the need incorporate specific examples that demonstrate suitability these targeted tasks, further emphasizing promise advancing sensor device 1 Introduction 2 Strategies 3 Applications 4 Other Miscellaneous Examples 5 Drawbacks Limitations 6 Conclusion Perspectives 7 List Abbreviations Definitions

Language: Английский

Citations

1

Functional polymer materials containing heavy group‐14 elements focusing on germanium and tin DOI Creative Commons
Masayuki Gon, Kazuo Tanaka

Smart Molecules, Journal Year: 2025, Volume and Issue: unknown

Published: March 16, 2025

Abstract In this review, the synthesis, functions, and applications of polymers containing germanium tin, which are heavy group 14 elements, in their polymer frameworks summarized. Germanium tin can form similar skeletal structures with homologues carbon silicon, whereas show unique properties derived from large atomic radii weak binding energies. For example, polygermane polystannane exhibited light absorption UV–visible region conductivity because σ‐conjugation through main‐chain constructed by σ‐bonds between elements. The was affected conformational change main‐chain, thermochromic be induced. Furthermore, bonds were able to cleaved homolytically upon photoirradiation, radicals subsequently generated. By incorporating hypervalent elements into π‐conjugated system, it possible modulate electronic system σ*–π* conjugation highly coordinated Finally, for organic solar cells, light‐emitting materials, chemical sensors have been achieved. Herein, representative synthetic methods creating smart materials will explained.

Language: Английский

Citations

0

Stimuli‐Responsive Optical Materials Based on Hypervalent Antimony‐Containing Conjugated Molecules DOI Open Access
Kazuya Tanimura, Masayuki Gon, Kazuo Tanaka

et al.

Advanced Functional Materials, Journal Year: 2024, Volume and Issue: unknown

Published: Nov. 17, 2024

Abstract Stimuli‐responsive materials have been applied for sensor devices because they can transform and amplify various target stimuli into observable signals. Much effort has devoted to exploring effective molecular designs obtaining stimuli‐responsive behaviors by taking advantage of the unique optoelectronic properties π‐conjugated molecules involving elements. This study focuses on modulation electronic state scaffolds oxidation number change hypervalent antimony. demonstrate that strength intramolecular interaction between antimony framework be tuned with ligand structure, substituent effect, shifts In particular, color changes represented hypsochromic bathochromic wavelength optical bands are achieved oxidative reaction in solid state. Significantly, direction confidently predicted quantum chemical calculations. The findings, based main‐group elements, provide logical design strategies advanced materials.

Language: Английский

Citations

0