Cost‐effective synthesis of unsymmetric tetrazines DOI Creative Commons
Jangsun Hwang, Bokyung Yoon, Sung‐Eun Suh

et al.

Bulletin of the Korean Chemical Society, Journal Year: 2024, Volume and Issue: 45(10), P. 867 - 872

Published: Oct. 1, 2024

Abstract 1,2,4,5‐Tetrazines serve as versatile two‐carbon synthons, essential for synthesizing a variety of (hetero)aromatic compounds. Their specific reactivity with certain dienophiles, without interfering biochemical processes, makes them ideal bioorthogonal ligation. Despite their broad utility, current synthetic methods are costly and raise safety concerns, particularly during scale‐up. This study introduces safer more cost‐effective strategies utilizing zinc chloride or boron trifluoride diethyl etherate catalysts. These alternatives significantly reduce costs enhance safety, potentially expanding the applicability tetrazine synthesis across broader research domains.

Language: Английский

Bioorthogonal Chemistry at Radboud University: Past, Present and Future DOI Creative Commons
Floris P. J. T. Rutjes, Kimberly M. Bonger, Kevin Neumann

et al.

Synlett, Journal Year: 2024, Volume and Issue: unknown

Published: March 14, 2024

Abstract Over the past two decades, bioorthogonal chemistry has profoundly impacted various chemistry-related fields, including chemical biology and drug delivery. This transformative progress stems from collaborative efforts involving chemists biologists, underscoring importance of interdisciplinary research. In this Account, we present developments in within our Institute for Molecules Materials at Radboud University. The disclosed here spans strained alkynes alkenes to release bioconjugation strategies, mirroring extensive scope provided by chemistry. By reflecting on originating University, Account emphasizes that teamwork is essential driving significant 1 Introduction 2 Providing BCN as a Robust Bioorthogonal Tool Chemical Biology Beyond 3 Towards Readily Available Click-to-Release trans-Cyclooctenes 4 Giving Guidance 5 Next Generation Bioconjugation Strategies: Dynamic Click Chemistry 6 Conclusions

Language: Английский

Citations

1

Functional 1,2,4,5‐Tetrazine Systems for Photocatalysis and Sensing DOI Open Access
M. Rajeswara Rao,

Aswani Raj K

Asian Journal of Organic Chemistry, Journal Year: 2024, Volume and Issue: unknown

Published: Nov. 13, 2024

Abstract s‐Tetrazines are aromatic heterocyclic systems with distinct structural and optoelectronic features, which have led to the design development of tetrazine‐derived in various applications. In this review, we summarize all research reported on subject applicability tetrazine derivatives for photocatalytic chemical transformation, hydrogen production, coordination‐based analyte detection.

Language: Английский

Citations

0

Cutting-edge bioorthogonal chemistry: Innovations, practical applications, and emerging trends DOI Open Access
Anup Basnet Chetry

European Journal of Chemistry, Journal Year: 2024, Volume and Issue: 15(4), P. 355 - 365

Published: Dec. 31, 2024

Bioorthogonal chemistry has emerged as a pivotal field in molecular science, offering transformative tools for applications drug discovery, imaging, and biology. This review provides comprehensive analysis of recent advancements bioorthogonal chemistry, emphasizing key innovations, practical applications, future research directions. We explore state-of-the-art reactions, including Staudinger ligation, strain-promoted azide-alkyne cycloaddition (SPAAC), tetrazine detailing their mechanisms, advantages, limitations. The highlights significant innovations such novel fluorogenic probes, improved catalysts, enhanced reaction conditions that have expanded the utility efficiency these reactions. Practical are examined, showing how advances revolutionized fields like live-cell targeted delivery, labeling. Looking to future, we discuss emerging trends potential avenues, integration with other advanced technologies development new methodologies. detailed overview current state outlines its potential, serving valuable resource researchers practitioners field.

Language: Английский

Citations

0

Cost‐effective synthesis of unsymmetric tetrazines DOI Creative Commons
Jangsun Hwang, Bokyung Yoon, Sung‐Eun Suh

et al.

Bulletin of the Korean Chemical Society, Journal Year: 2024, Volume and Issue: 45(10), P. 867 - 872

Published: Oct. 1, 2024

Abstract 1,2,4,5‐Tetrazines serve as versatile two‐carbon synthons, essential for synthesizing a variety of (hetero)aromatic compounds. Their specific reactivity with certain dienophiles, without interfering biochemical processes, makes them ideal bioorthogonal ligation. Despite their broad utility, current synthetic methods are costly and raise safety concerns, particularly during scale‐up. This study introduces safer more cost‐effective strategies utilizing zinc chloride or boron trifluoride diethyl etherate catalysts. These alternatives significantly reduce costs enhance safety, potentially expanding the applicability tetrazine synthesis across broader research domains.

Language: Английский

Citations

0