Machine learning accelerates the screening of single-atom catalysts towards CO2 electroreduction DOI
Yaxin Shi, Zhiqin Liang

Applied Catalysis A General, Journal Year: 2024, Volume and Issue: 676, P. 119674 - 119674

Published: March 13, 2024

Language: Английский

Comprehensive Insight into Construction of Active Sites toward Steering Photocatalytic CO2 Conversion DOI
Wa Gao,

Haoqing Chi,

Yujie Xiong

et al.

Advanced Functional Materials, Journal Year: 2023, Volume and Issue: 34(13)

Published: Dec. 21, 2023

Abstract Photoreduction of CO 2 into hydrocarbon fuels is a promising avenue for achieving sustainable alternative to the artificial carbon cycle. Photocatalytic conversion chemical transformation photogenerated carriers and adsorbed at active sites catalysts. Active can regulate kinetic process carriers, control adsorption intermediates, lower activation barriers, promote C‐C coupling. This review mainly concentrates on efficiency selectivity regulation target products through construction sites. First, principles photoreduction, such as influencing factors specific pathways monocarbon multicarbon (C 2+ ) formation, are discussed. Then, leading works focusing improving catalytic regulating product introduction highlighted, concerning underlying mechanism performance, especially C generation. Subsequently, an overview currently available in situ techniques theoretical calculation identifying provided. Finally, challenges emerging strategies achieve recycling from scientific, technical, economic perspectives considered. offers deep insight site with atomic precision efficient photocatalytic generation high selectivity.

Language: Английский

Citations

12

Br-doped Cu nanoparticle formed by in situ restructuring for highly efficient electrochemical reduction of CO2 to formate DOI
Xiaoxiao Wang,

Awei Guo,

Yunlong Wang

et al.

Journal of Colloid and Interface Science, Journal Year: 2023, Volume and Issue: 653, P. 238 - 245

Published: Sept. 11, 2023

Language: Английский

Citations

11

Electrocatalytic and Photocatalytic CO2 Methanation: From Reaction Fundamentals to Catalyst Developments DOI

Junbo Tian,

Wenqing Xu,

Jiajian Gao

et al.

ChemCatChem, Journal Year: 2024, Volume and Issue: 16(9)

Published: Jan. 5, 2024

Abstract Transitioning from fossil fuels to renewable energy sources is demanded due the gradual depletion of petroleum oil/gas and environmental impact carbon dioxide (CO 2 ) emissions into atmosphere. Electrocatalytic photocatalytic CO reduction methane (CH 4 using crucial for sustainable chemical/fuel production greenhouse gas reduction. In recent years, extensive research has focused on understanding fundamental aspects two approaches, such as reaction mechanisms active sites, exploring/designing novel catalytic materials. This review initially discusses fundamentals, including performance evaluation indexes, reactors, mechanisms, understand reactions. Subsequently, various catalyst preparation strategies characterization methods are summarized, trying outline design principle based obtained mechanisms. Finally, challenges perspectives future development in this area discussed presented. It expected provide a comprehensive photo/electrocatalytic methanation, valuable knowledge novice researchers, helpful reference endeavors.

Language: Английский

Citations

4

A Cu-Pd alloy catalyst with partial phase separation for the electrochemical CO2 reduction reaction DOI

Gyeong Ho Han,

Jung Yong Seo, Minji Kang

et al.

Journal of Energy Chemistry, Journal Year: 2024, Volume and Issue: 93, P. 8 - 15

Published: Feb. 8, 2024

Language: Английский

Citations

4

Machine learning accelerates the screening of single-atom catalysts towards CO2 electroreduction DOI
Yaxin Shi, Zhiqin Liang

Applied Catalysis A General, Journal Year: 2024, Volume and Issue: 676, P. 119674 - 119674

Published: March 13, 2024

Language: Английский

Citations

4