Advanced Sensor and Energy Materials,
Journal Year:
2024,
Volume and Issue:
3(3), P. 100116 - 100116
Published: June 28, 2024
The
exploration
of
efficient
lead-free
perovskite
photoelectric
active
materials
to
develop
high-performance
photoelectrochemical
(PEC)
systems
in
aqueous
solution
is
crucial
expand
their
PEC
applications.
Herein,
we
successfully
constructed
a
platform
using
ligand-free
Cs2PdBr6
microcrystals
(MCs)
as
the
photoactive
substance.
MCs
showed
narrow
bandgap,
wide
absorption
range,
high
electronic
mobility
and
good
stability
solutions.
Particularly,
exhibited
an
excellent
photoresponse,
photocurrent
density
could
reach
98
μA/cm2
under
10.18
mW/cm2
light
irradiation
absence
other
electron
acceptors.
In
addition
extremely
range
response
wavelength,
pH
accelerated
interfacial
carrier
transfer,
demonstrated
significant
potential
photocathode
material
for
applications
sensors
optoelectronic
devices.
Therefore,
this
work
indicates
that
design
highly
way
solve
intrinsic
issues
material,
predicting
promising
strategy
performance
application
ambience.
Advanced Sensor and Energy Materials,
Journal Year:
2024,
Volume and Issue:
3(3), P. 100116 - 100116
Published: June 28, 2024
The
exploration
of
efficient
lead-free
perovskite
photoelectric
active
materials
to
develop
high-performance
photoelectrochemical
(PEC)
systems
in
aqueous
solution
is
crucial
expand
their
PEC
applications.
Herein,
we
successfully
constructed
a
platform
using
ligand-free
Cs2PdBr6
microcrystals
(MCs)
as
the
photoactive
substance.
MCs
showed
narrow
bandgap,
wide
absorption
range,
high
electronic
mobility
and
good
stability
solutions.
Particularly,
exhibited
an
excellent
photoresponse,
photocurrent
density
could
reach
98
μA/cm2
under
10.18
mW/cm2
light
irradiation
absence
other
electron
acceptors.
In
addition
extremely
range
response
wavelength,
pH
accelerated
interfacial
carrier
transfer,
demonstrated
significant
potential
photocathode
material
for
applications
sensors
optoelectronic
devices.
Therefore,
this
work
indicates
that
design
highly
way
solve
intrinsic
issues
material,
predicting
promising
strategy
performance
application
ambience.