Partial Oxidation of CH4 in Plasma: The Effects of Oxidant and Catalyst Addition DOI Creative Commons
O. V. Golubev, A. L. Maximov

Molecules, Journal Year: 2025, Volume and Issue: 30(9), P. 1958 - 1958

Published: April 28, 2025

The partial oxidation of methane in cold atmospheric plasma represents an innovative and promising approach to energy conversion sustainable chemical processes for obtaining various chemicals fuels. In present work, dielectric barrier discharge is applied the CH4 combined with Cu-containing catalysts. catalysts different porous acidic properties were obtained, characterized by physico-chemical methods used plasma-catalytic reaction. influence oxidizing agent (oxygen vs. air) on products’ selectivity yield was studied. It found that using air as oxidizer beneficial terms gaseous products yield, N2 aided denser microdischarge formation. Using pure O2 resulted enhanced oxygenate (mainly CH3OH) generation. Furthermore, methanol compared plasma-only process, well efficiency process.

Language: Английский

Continuous methane selective oxidation to methanol over Cu-SAPO-34 DOI Creative Commons
Lanlan Sun, Yu Wang, Meng Zhao

et al.

Molecular Catalysis, Journal Year: 2025, Volume and Issue: 577, P. 114954 - 114954

Published: Feb. 28, 2025

Language: Английский

Citations

0

Partial Oxidation of CH4 in Plasma: The Effects of Oxidant and Catalyst Addition DOI Creative Commons
O. V. Golubev, A. L. Maximov

Molecules, Journal Year: 2025, Volume and Issue: 30(9), P. 1958 - 1958

Published: April 28, 2025

The partial oxidation of methane in cold atmospheric plasma represents an innovative and promising approach to energy conversion sustainable chemical processes for obtaining various chemicals fuels. In present work, dielectric barrier discharge is applied the CH4 combined with Cu-containing catalysts. catalysts different porous acidic properties were obtained, characterized by physico-chemical methods used plasma-catalytic reaction. influence oxidizing agent (oxygen vs. air) on products’ selectivity yield was studied. It found that using air as oxidizer beneficial terms gaseous products yield, N2 aided denser microdischarge formation. Using pure O2 resulted enhanced oxygenate (mainly CH3OH) generation. Furthermore, methanol compared plasma-only process, well efficiency process.

Language: Английский

Citations

0