Excellent laccase mimic activity of Cu-melamine and its applications in the degradation of Congo red DOI Creative Commons
Siyuan Chai, Enze Huang, Jinsheng Zeng

et al.

Research Square (Research Square), Journal Year: 2024, Volume and Issue: unknown

Published: Dec. 4, 2024

Abstract Copper-based nanozyme has shown the superior in oxidase-like activities due to its electron transfer ability between Cu (I) and (II) sites during catalytic reactions. Herein, a Cu(I)-MOF (Cu-Mel) was readily synthesized by traditional hydrothermal process using precursors of Cu+ melamine, which then used laccase-like reactions for first time. Some means, such as X-ray diffraction (XRD), scanning microscope (SEM), Fourier transform infrared spectroscopy (FTIR) photoelectron (XPS) were employed character microstructure Cu-Mel. The oxidation 4-aminoantipyrine (4-AP) 2,4-dichlorophenol (2,4-DP) adopted evaluate resulting conditions including temperatures, presence alcohols ionic concentrations, varied optimize activities, based on that, highest activity is presented with higher maximum reaction rate (Vmax). good storage stability also Cu-Mel utilized degradation Congo red, showing efficiency. These findings facilitate development laccase mimics serve foundation design applications Cu-MOFs realm.

Language: Английский

Excellent Laccase Mimic Activity of Cu-Melamine and Its Applications in the Degradation of Congo Red DOI
Siyuan Chai, Enze Huang, Jinsheng Zeng

et al.

Applied Biochemistry and Biotechnology, Journal Year: 2025, Volume and Issue: unknown

Published: Feb. 1, 2025

Language: Английский

Citations

2
A Colorimetric and Fluorescent Dual-Mode Sensor Based on a Smartphone-Assisted Laccase-like Nanoenzyme for the Detection of Tetracycline Antibiotics DOI Creative Commons
Hongyue Chen, Zining Wang, Qi Shi

et al.

Nanomaterials, Journal Year: 2025, Volume and Issue: 15(3), P. 162 - 162

Published: Jan. 22, 2025

A copper-based nanoenzyme (Cu-BL) co-modified by L-L-lysine and 2-2-amino terephthalic acid has laccase-like activity fluorescence characteristics. Based on this, a colorimetric fluorescent dual-mode sensor was developed to visually quantitatively detect tetracycline antibiotics (TCs), including (TC), chlortetracycline (CTC), oxytetracycline (OTC). In the detection system, TCs can inhibit generation of singlet oxygen (1O2) weaken ability 2,4-dichlorophenol (2,4-DP) be oxidized into pink-colored quinone substances. The linear ranges are 0.5–80 μM, 1–80 0.25–80 limits 0.27 0.22 0.26μM, respectively. addition, due inner filter effect, interact with Cu-BL, increase in antibiotic concentration, intensity will decrease. smartphone sensing platform is combined signal for rapid visual quantitative antibiotics. Generally speaking, colorimetric/fluorescence demonstrates good stability, high specificity, strong anti-interference capabilities, highlighting its practical application potential. This work expected offer novel insights development multifunctional nanoenzymes integration multi-mode platform.

Language: Английский

Citations

1
DNAzyme@MOF breaking pH limitation for the detection of dopamine in the interstitial fluid DOI

Jiuhong Zhao,

Jun‐Wu Zhao, Xiaoyu Zhang

et al.

Biosensors and Bioelectronics, Journal Year: 2025, Volume and Issue: unknown, P. 117367 - 117367

Published: March 1, 2025

Language: Английский

Citations

1
Laccase-mimicking enzyme with fluorescent properties for dual-mode detection of epinephrine and degradation of phenolic pollutants DOI

Huizhu Fan,

Luxi Huang,

Yin Dai

et al.

Microchimica Acta, Journal Year: 2025, Volume and Issue: 192(4)

Published: March 28, 2025

Language: Английский

Citations

0
Two novel laccase-like nanozymes based on azole ligands for constructing pH-dependent sensor array for recognizing halogenated phenolic pollutants DOI

Qing Han,

Xixingchi Chen,

Yunlong Wang

et al.

Journal of Hazardous Materials, Journal Year: 2025, Volume and Issue: 494, P. 138436 - 138436

Published: April 28, 2025

Language: Английский

Citations

0
Mixed-valence Ce-Fe bimetallic MOFs with multi-enzyme-like activities for colorimetric biosensing and catalytic degradation DOI
Xinyu Wang,

K.L. Jiao,

Yingli

et al.

Journal of Colloid and Interface Science, Journal Year: 2025, Volume and Issue: 695, P. 137784 - 137784

Published: May 3, 2025

Language: Английский

Citations

0
Excellent laccase mimic activity of Cu-melamine and its applications in the degradation of Congo red DOI Creative Commons
Siyuan Chai, Enze Huang, Jinsheng Zeng

et al.

Research Square (Research Square), Journal Year: 2024, Volume and Issue: unknown

Published: Dec. 4, 2024

Abstract Copper-based nanozyme has shown the superior in oxidase-like activities due to its electron transfer ability between Cu (I) and (II) sites during catalytic reactions. Herein, a Cu(I)-MOF (Cu-Mel) was readily synthesized by traditional hydrothermal process using precursors of Cu+ melamine, which then used laccase-like reactions for first time. Some means, such as X-ray diffraction (XRD), scanning microscope (SEM), Fourier transform infrared spectroscopy (FTIR) photoelectron (XPS) were employed character microstructure Cu-Mel. The oxidation 4-aminoantipyrine (4-AP) 2,4-dichlorophenol (2,4-DP) adopted evaluate resulting conditions including temperatures, presence alcohols ionic concentrations, varied optimize activities, based on that, highest activity is presented with higher maximum reaction rate (Vmax). good storage stability also Cu-Mel utilized degradation Congo red, showing efficiency. These findings facilitate development laccase mimics serve foundation design applications Cu-MOFs realm.

Language: Английский

Citations

0