Chemical Engineering Journal, Journal Year: 2025, Volume and Issue: unknown, P. 163139 - 163139
Published: April 1, 2025
Language: Английский
Chemical Engineering Journal, Journal Year: 2025, Volume and Issue: unknown, P. 163139 - 163139
Published: April 1, 2025
Language: Английский
International Journal of Hydrogen Energy, Journal Year: 2023, Volume and Issue: 49, P. 260 - 271
Published: Aug. 6, 2023
Language: Английский
Citations
11ACS Applied Materials & Interfaces, Journal Year: 2024, Volume and Issue: 16(32), P. 41734 - 41742
Published: Aug. 2, 2024
The development of sustainable and effective electrochemical nitrogen fixation catalysts is crucial for the mitigation terrible energy consumption resulting from Haber-Bosch process. Molybdenum disulfide (MoS2) exhibits promise toward reduction reaction (NRR) on account its similar structure to natural nitrogenases MoFe-co but still undergoes serious challenges with unsatisfactory catalytic performance resulted limited active sites, conductivity, selectivity. In this work, Fe/Co/B codoped MoS2 ultrathin nanosheets are synthesized verified as excellent NRR high activity, selectivity, durability. FeCoB-MoS2 demonstrates a ammonia yield 36.99 μg h–1 mgcat–1 at −0.15 V vs RHE Faraday efficiency (FE) 30.65% −0.10 in 0.1 M HCl. experimental results density functional theory (DFT) calculations emphasize that codoping Fe, Co, B into synergistically enhances conductivity optimizes electronic catalyst, which significantly improves electrocatalytic synthesis performance. This work broadens potential enlightens strategy designing efficient electrocatalysts field.
Language: Английский
Citations
4Chemical Engineering Journal, Journal Year: 2024, Volume and Issue: unknown, P. 155735 - 155735
Published: Sept. 1, 2024
Language: Английский
Citations
4International Journal of Hydrogen Energy, Journal Year: 2025, Volume and Issue: 111, P. 513 - 523
Published: Feb. 26, 2025
Language: Английский
Citations
0Chemical Engineering Journal, Journal Year: 2025, Volume and Issue: unknown, P. 163139 - 163139
Published: April 1, 2025
Language: Английский
Citations
0