Journal of Alloys and Compounds, Journal Year: 2025, Volume and Issue: unknown, P. 180640 - 180640
Published: April 1, 2025
Language: Английский
Journal of Alloys and Compounds, Journal Year: 2025, Volume and Issue: unknown, P. 180640 - 180640
Published: April 1, 2025
Language: Английский
Journal of Colloid and Interface Science, Journal Year: 2025, Volume and Issue: 690, P. 137336 - 137336
Published: March 14, 2025
Language: Английский
Citations
1Inorganic Chemistry, Journal Year: 2025, Volume and Issue: unknown
Published: April 3, 2025
Electrocatalytic water splitting for hydrogen production represents a crucial pathway toward establishing sustainable energy infrastructure and addressing environmental concerns, with the development of high-performance nonprecious metal catalysts being central focus. While Ni3S2 demonstrates potential as an electrocatalyst, its limited functionality suboptimal performance necessitate further enhancement. In this study, drawing inspiration from natural hydrogenases, we engineered novel NiFeSe/Ni3S2 composite electrocatalyst through integration NiFeSe Ni3S2. The synthesized catalyst displayed outstanding overall water-splitting in alkaline media, realizing current densities 100 10 mA cm-2 at remarkably low overpotentials 267.4 mV (vs RHE) oxygen evolution reaction (OER) 105.6 (HER), respectively. Remarkably, two-electrode electrolyzer incorporating achieved density 20 substantially reduced cell voltage 1.586 V. Comprehensive analysis revealed that strategic construction biomimetic active centers heterogeneous interfaces significantly modulates electronic structure, improved charge transfer, redistribution electron catalytic sites. This investigation provides valuable insights promising framework rational design bifunctional electrocatalysts applications.
Language: Английский
Citations
0Chemical Engineering Journal, Journal Year: 2025, Volume and Issue: unknown, P. 162421 - 162421
Published: April 1, 2025
Language: Английский
Citations
0Applied Surface Science, Journal Year: 2025, Volume and Issue: unknown, P. 163282 - 163282
Published: April 1, 2025
Language: Английский
Citations
0Journal of Alloys and Compounds, Journal Year: 2025, Volume and Issue: unknown, P. 180640 - 180640
Published: April 1, 2025
Language: Английский
Citations
0