Experimental study on Finding stable catalytic methane decomposition for hydrogen production DOI
Reiyu Chein,

Cheng-Chi Ou

International Journal of Hydrogen Energy, Journal Year: 2024, Volume and Issue: unknown

Published: July 1, 2024

Language: Английский

Thermocatalytic methane pyrolysis over iron-based catalysts for turquoise hydrogen production: activity and kinetic studies DOI Creative Commons

Piercosimo Vedele,

Enrico Sartoretti,

Giulia Torretti

et al.

Chemical Engineering Journal, Journal Year: 2025, Volume and Issue: unknown, P. 163392 - 163392

Published: May 1, 2025

Language: Английский

Citations

0

Role of MgO in Al2O3‐supported Fe catalysts for hydrogen and carbon nanotubes formation during catalytic methane decomposition DOI Creative Commons

Mohammed O. Bayazed,

Ahmed S. Al‐Fatesh, Anis H. Fakeeha

et al.

Energy Science & Engineering, Journal Year: 2024, Volume and Issue: unknown

Published: Sept. 1, 2024

Abstract Catalytic methane decomposition is a promising technology for reducing the reliance on fossil fuels and mitigating effects of climate change by producing clean hydrogen value‐added carbon without emission greenhouse gases. The aim study was to investigate use Al 2 O 3 ‐modified MgO doped iron‐based catalysts catalytic methane. were synthesized using impregnation method characterized various analysis techniques, including Brunauer, Emmett, Teller, temperature programmed reduction, oxidation, X‐ray diffraction, thermal gravimetric analysis, Raman, scanning electron microscopy, transmission microscopy. activity tested in packed‐bed reactor with gas flow rate 20 mL/min at 800°C. investigation focuses influence incorporating magnesium into alumina concentration ranging from (20%–70%), where higher levels improve creating more active sites, positively impacting decomposition. Enhanced catalyst reducibility increased particle dispersion lead improved properties despite reduced surface area. FA70M FA63M exhibited almost same characteristics highest stability conversion among investigated, reaching 87% 85% 800°C 120 min. Moreover, both showed yields 86% 85%, respectively. introduction further total yield 103% FA 39% FM 114% 120% respective (FA70M FA63M). During reaction, nanotubes varying diameters produced. Higher iron loading resulted positive trend.

Language: Английский

Citations

3

H2 and carbon production from CH4 decomposition and regeneration based on Fe/CaO-Ca12Al14O33 catalyst looping cycles DOI

Zhiwei Chu,

Jigang Zhang, Wenhan Zhao

et al.

Chemical Engineering Journal, Journal Year: 2024, Volume and Issue: 497, P. 154599 - 154599

Published: Aug. 18, 2024

Language: Английский

Citations

2

Methane Decomposition to Hydrogen Over Zirconia‐Supported Fe Catalysts–Effects of the Modified Support DOI Creative Commons

Mohammed O. Bayazed,

Anis H. Fakeeha, Ahmed A. Ibrahim

et al.

ChemistryOpen, Journal Year: 2023, Volume and Issue: 12(9)

Published: Sept. 1, 2023

Methane decomposition is a promising route to synthesize COx -free hydrogen and carbon nanomaterials (CNMs ). In this work, the impregnation method was employed for preparation of catalysts. Systematic investigations on activity stability Fe-based catalysts were carried out in packed-bed micro-activity reactor at 800 °C with feed gas flow rate 18 mL/min. The effect doping Y2 O3 , MgO, SiO2 TiO2 over ZrO2 catalytic performance also studied. BET revealed that specific surface areas pore volumes are increased after added while MgO had negative impact hence little decrease area observed. results showed catalyst supported -doped is, Fe-TiZr, demonstrated highest stability, maximum methane conversion 81.3 % during 180 min time-on-stream. At °C, initial 73 %, 38 64 69 final yield 121 wt. 55 354 174 achieved using Fe-MgZr, Fe-SiZr, Fe-TiZr Fe-YZr catalysts, respectively. Moreover, bulk deposition uniform nanotubes high degree graphitization different diameters observed

Language: Английский

Citations

6

Metal–Organic Framework-Templated Synthesis of Nickel–Alumina Nanocatalysts Improves Catalyst–Support Interaction for Higher Activity and Stability in Biogas Reforming under Controlled Oxidizing Conditions DOI
Arisha Sharma, Prakash Biswas, Meenesh R. Singh

et al.

ACS Applied Materials & Interfaces, Journal Year: 2024, Volume and Issue: unknown

Published: Nov. 26, 2024

Tri-reforming methane with CO

Language: Английский

Citations

1

The catalytic decomposition of CH4 using Ce-doped Fe/CaO-Ca12Al14O33 catalyst and its regeneration performance for H2 production DOI

Zhiwei Chu,

Wenhan Zhao,

Duo Xu

et al.

Separation and Purification Technology, Journal Year: 2024, Volume and Issue: unknown, P. 129670 - 129670

Published: Sept. 1, 2024

Language: Английский

Citations

0

Ni‐Co Bimetallic Catalysts Supported on Mixed Oxides (Sc‐Ce‐Zr) for Enhanced Methane Dry Reforming DOI Creative Commons
Ahmed E. Abasaeed, Ahmed A. Ibrahim, Anis H. Fakeeha

et al.

ChemistryOpen, Journal Year: 2024, Volume and Issue: unknown

Published: Nov. 12, 2024

Abstract Dry methane reforming (DRM) presents a viable pathway for converting greenhouse gases into useful syngas. Nevertheless, the procedure requires robust and reasonably priced catalysts. This study explored using cost‐effective cobalt nickel combined single catalyst with different metal ratios. The reaction was conducted in fixed reactor at 700 °C. findings indicate that incorporation of significantly enhances performance by preventing sintering, improving dispersion, promoting beneficial metal‐support interactions. best‐performing (3.75Ni+1.25Co‐ScCeZr) achieved good conversion rate CH 4 CO 2 46.8 %, 60 % respectively after 330 minutes while maintaining stability. TGA ‐TPD analysis results show addition Co to Ni reduces carbon formation, increases amount strong basic sites isolated O − species, total desorbed. These collectively highlight potential cobalt‐nickel catalysts practical DRM applications contribute developing sustainable energy technologies.

Language: Английский

Citations

0

Experimental study on Finding stable catalytic methane decomposition for hydrogen production DOI
Reiyu Chein,

Cheng-Chi Ou

International Journal of Hydrogen Energy, Journal Year: 2024, Volume and Issue: unknown

Published: July 1, 2024

Language: Английский

Citations

0