Metal-Exchanged Phosphomolybdic Acid Salts-Catalyzed Esterification of Levulinic Acid DOI Open Access
Márcio José da Silva, Alana Alves Rodrigues,

Wilton Keisuke Taba

et al.

Processes, Journal Year: 2024, Volume and Issue: 12(11), P. 2574 - 2574

Published: Nov. 17, 2024

We examined the effectiveness of metal-exchanged phosphomolybdic acid salts in converting levulinic acid, derived from biomass, into valuable products (alkyl levulinate). prepared using different metals (Fe3+, Al3+, Zn2+, Cu2+, Mn2+, Ni2+, and Co2+). The influence metal cations on conversion selectivity reactions was assessed. found that with iron aluminum phosphomolybdate were most effective catalysts for esterification methanol, tending towards 100% after 6 h reaction at a temperature 323 K. effect catalyst loading its recovery reuse evaluated; results remained similar four cycles use. investigated between 298 353 reactivity alcohols carbon chain size C1-C4 assessed conversions above 65% obtained all tested under conditions evaluated, except tert-butyl alcohol. These are promising alternative to traditional soluble corrosive Brønsted catalysts. superior performance these ascribed higher pH decline triggered by hydrolysis cations.

Language: Английский

Production of biodiesel from hemp oil and oleic acid with sulfonated camphor catalysts is to be evaluated with controlled tests in a diesel engine DOI
Manuel Sánchez‐Cárdenas,

Luis A. Sánchez‐Olmos,

Fernando Trejo

et al.

International Journal of Chemical Reactor Engineering, Journal Year: 2025, Volume and Issue: unknown

Published: Jan. 28, 2025

Abstract This research examines the performance variables, combustion, and amounts of NOx, CO, HC, K emissions in a diesel engine, using blends hemp biodiesel oleic acid with conventional diesel. To obtain from oil acid, heterogeneous sulfonated camphor catalyst (CASU-AL) was used for transesterification esterification respectively. Several characterization tests were performed on CASU-AL such as acid-base titration method quantification sites, XRD analysis to determine areas carbonaceous material, images composition obtained SEM EDX, porosity characteristics surface properties assessed BET analysis. Constant operating conditions autogenous reactor temperature 200 °C, reaction time 23 min, quantity 0.033 % w. analyses applied CASU-AL, several mixtures made diesel, different biodiesels laboratory. The (DIE-100), (BAC-100), (BAO-100), Diesel-BAC mixture 30 (MDBAC-30), Diesel-BAO (MDBAO-30). For three speed zones selected engine identify behavior at low 1,200 rpm, medium 1,400 high 1800 rpm. Combustion reveal that no significant variation is observed however, gaseous products derived reductions carbon monoxide, unburned hydrocarbon, an increase nitrogen oxide achieved when DIE-100 compared BAC-100 BAO-100. showed reduction K, smoke testing MDBAC-30 MDBAO-30 laboratory engine. A comparison oil-oleic BAO-100 revealed could be alone or blend 70 fuel engines by decreasing air pollutants promoting lubricity Our findings best lowest among all tested fuels. In other words, are ideal do not require any modification

Language: Английский

Citations

0

Vicinal diphosphorylation of enaminones with diaryl phosphine oxides via AlCl3-mediated C N bond cleavage DOI
Xin Jin,

An Yong,

Jia Chen

et al.

Tetrahedron Letters, Journal Year: 2025, Volume and Issue: 158, P. 155472 - 155472

Published: Feb. 20, 2025

Language: Английский

Citations

0

Optimization of selectively chloroacetic acid esterification in the presence of Amberlyst-15 catalyst using the response surface methodology DOI Creative Commons
Ahmad Nikseresht, Seyyed Hossein Hosseini,

Leila Matin

et al.

Results in Chemistry, Journal Year: 2025, Volume and Issue: unknown, P. 102147 - 102147

Published: Feb. 1, 2025

Language: Английский

Citations

0

Zirconium Phosphates and Phosphonates: Applications in Catalysis DOI Open Access
Anna Donnadio, Monica Pica, Morena Nocchetti

et al.

Catalysts, Journal Year: 2024, Volume and Issue: 14(10), P. 733 - 733

Published: Oct. 19, 2024

This review covers recent advancements in the use of zirconium phosphates and phosphonates (ZrPs) as catalysts or catalyst supports for a variety reactions, including biomass conversion, acid–base catalysis, hydrogenation, oxidation, C-C coupling from 2015 to present. The discussion emphasizes intrinsic catalytic properties ZrPs, focusing on how surface acidity, hydrophobic/hydrophilic balance, textural properties, particle morphology influence their performance across various reactions. Additionally, this thoroughly examines ZrPs species, ranging organometallic complexes metal ions noble metals oxide nanoparticles. In these applications, not only enhance dispersion stabilization active species but also facilitate recovery reuse due robust immobilization solid support. dual functionality underscores importance promoting efficient, selective, sustainable processes, making them essential advancement green chemistry.

Language: Английский

Citations

1

Metal-Exchanged Phosphomolybdic Acid Salts-Catalyzed Esterification of Levulinic Acid DOI Open Access
Márcio José da Silva, Alana Alves Rodrigues,

Wilton Keisuke Taba

et al.

Processes, Journal Year: 2024, Volume and Issue: 12(11), P. 2574 - 2574

Published: Nov. 17, 2024

We examined the effectiveness of metal-exchanged phosphomolybdic acid salts in converting levulinic acid, derived from biomass, into valuable products (alkyl levulinate). prepared using different metals (Fe3+, Al3+, Zn2+, Cu2+, Mn2+, Ni2+, and Co2+). The influence metal cations on conversion selectivity reactions was assessed. found that with iron aluminum phosphomolybdate were most effective catalysts for esterification methanol, tending towards 100% after 6 h reaction at a temperature 323 K. effect catalyst loading its recovery reuse evaluated; results remained similar four cycles use. investigated between 298 353 reactivity alcohols carbon chain size C1-C4 assessed conversions above 65% obtained all tested under conditions evaluated, except tert-butyl alcohol. These are promising alternative to traditional soluble corrosive Brønsted catalysts. superior performance these ascribed higher pH decline triggered by hydrolysis cations.

Language: Английский

Citations

1