Robust and Temperature‐Sensitive Hydrogels for High‐Efficiency Water Harvesting Under Low Solar Energy Radiation DOI
Meng Wang, Zhiqiang Sun, Jianhua Zhou

et al.

Solar RRL, Journal Year: 2023, Volume and Issue: 7(9)

Published: Feb. 23, 2023

Solar‐driven evaporation using hydrogels and photothermal materials is a promising freshwater harvesting technology. Clean water generally collected through subsequent condensation, which requires high energy input due to the inherent vaporization enthalpy of water. Therefore, it great challenge harvest fresh efficiently under natural irradiation. Herein, temperature‐sensitive polyacrylamide‐poly( N ‐isopropylacrylamide) (A‐PNIPAm) gel designed pursue collection rate low conditions, where facile reversible hydrophilic/hydrophobic transition in gels enables quick acquisition liquid A multifunctional hydrogel (ADS‐PNIPAm) prepared polydopamine sodium alginate with excellent adsorption/filtration properties, can remove pollutants generate rapidly. Consequently, ADS‐PNIPAm reaches up 5.89 9.8 kg m −2 h −1 0.6 1 sun irradiation, respectively, are superior previously reported values. Furthermore, displays an effect on purifying sewage, such as oils, algae, dyes pollutants. material for rapid generation solar irradiation only, provides new avenue alleviate source scarcity.

Language: Английский

Dual‐Network Liquid Metal Hydrogel with Integrated Solar‐Driven Evaporation, Multi‐Sensory Applications, and Electricity Generation via Enhanced Light Absorption and Bénard–Marangoni Effect DOI

Zechang Wei,

Yibo Wang, Chenyang Cai

et al.

Advanced Functional Materials, Journal Year: 2022, Volume and Issue: 32(41)

Published: Aug. 21, 2022

Abstract Solar‐driven evaporation is a promising strategy to relieve fresh water stress in the world. For an evaporator, it necessary be equiped with novel photothermal conversion materials and regulate heat energy loss solar‐driven generation process for efficiency. Herein, eutectic gallium‐indium (EGaIn)/polyaniline (PANI) complex (EP) cellulose nanocrystals (CNCs) are explored as light absorber broadband absorbing dispersant particles uniformity. Based on Bénard–Marangoni effect, dual‐network poly(vinyl alcohol)/poly(acrylamide) (PM) hydrogel evaporator water/ethylene glycol solvent transfer. Specifically, CNCs EP incorporated, endowed excellent mechanical properties, performance, electrical characteristics. Surface temperature of can reach ≈38.7 °C under 1 sun illumination h. combination absorption its rate higher than 1.50 kg m –2 h –1 . The engineered synergy also gives hydrogels multiple sensory capabilities, skin‐like function, power generation. This work demonstrates EGaIn‐based new approach transfer highly evaporation, focus integration multifunctional solar systems.

Language: Английский

Citations

80

High Quantum Yield Nitrogen-Doped Carbon Quantum Dot-Based Fluorescent Probes for Selective Sensing of 2,4,6-Trinitrotoluene DOI Creative Commons
Ömer Kaan Koç, Ayşem Üzer, Reşat Apak

et al.

ACS Applied Nano Materials, Journal Year: 2022, Volume and Issue: 5(4), P. 5868 - 5881

Published: April 6, 2022

Fluorescent carbon quantum dots hold great promise for the determination of nitro-explosive 2,4,6-trinitrotoluene (TNT), a potential environmental pollutant. Here, nitrogen-doped dot (N-CQD)-based fluorometric probe with high yield (73.10%) was developed selective TNT. N-CQDs were synthesized by reflux method using citric acid (CA) as precursor and ethylenediamine (EDA) diaminocyclohexane (DACH) nitrogen precursors. N-CQDs, excitation emission wavelengths 360 460 nm, respectively, highly toward TNT among different types explosives [i.e., tetryl, 2,4,6-trinitrophenol (TNP), 2,4-dinitrotoluene (DNT), 4-amino-2,6-dinitrotoluene (ADNT), HMX, 1,3,5-trinitroperhydro-1,3,5-triazine (RDX), pentaerythritol tetranitrate (PETN)]. As result dominant FRET mechanism secondarily assisted ground-state donor–acceptor complexation, fluorescence showed excellent quenching in presence The structure elucidated X-ray photoelectron spectroscopy, diffraction, IR, Raman, high-resolution transmission electron microscopy, dynamic light scattering techniques, their interaction resolved Gaussian (i.e., highest occupied molecular orbital–lowest unoccupied orbital energy levels) program. limit detection quantification aqueous media 30.0 90.0 nM, while Benesi–Hildebrand binding constant 2.22 × 103. In common soil ions, explosive mixtures, camouflage materials, could determine recoveries between 94.9 104.9%. addition, sandy specimens artificially contaminated real samples, extracted from these samples determined both reference liquid chromatography tandem mass spectrometry to validate proposed method. To design field two support materials based on thin layer chromatography-paper hydrogel (N-CQD-gel) developed, visually at μM level materials. make potentially useful sensor applications sensitive sensing ability.

Language: Английский

Citations

73

Carbon Dot‐Based Hydrogels: Preparations, Properties, and Applications DOI
Yijie Wang,

Tingjie Lv,

Keyang Yin

et al.

Small, Journal Year: 2023, Volume and Issue: 19(17)

Published: Jan. 29, 2023

Hydrogels have extremely high moisture content, which makes it very soft and excellently biocompatible. They become an important material a wide range of applications in various fields such as biomedicine, bionic smart material, electrochemistry. Carbon dot (CD)-based hydrogels are based on carbon dots (CDs) auxiliary substances, forming gel with comprehensive properties individual components. CDs embedding could not only solve their aggregation-caused quenching (ACQ) effect, but also manipulate the even bring some novel properties, achieving win-win situation. In this review, preparation methods, formation mechanism, CD-based hydrogels, sensing, adsorption, energy storage, catalysis -are summarized. Finally, brief discussion future research directions will be given.

Language: Английский

Citations

65

Controllable synthesis of bifunctional magnetic carbon dots for rapid fluorescent detection and reversible removal of Hg2+ DOI

Ying Song,

Ruyan Xie, Miaomiao Tian

et al.

Journal of Hazardous Materials, Journal Year: 2023, Volume and Issue: 457, P. 131683 - 131683

Published: May 24, 2023

Language: Английский

Citations

62

Hydrogels as promising platforms for solar-driven water evaporators DOI

Xinyu Jing,

Fangfei Liu, Tursun Abdiryim

et al.

Chemical Engineering Journal, Journal Year: 2023, Volume and Issue: 479, P. 147519 - 147519

Published: Nov. 19, 2023

Language: Английский

Citations

46

Double-layered hydrogels based on phase change material and pen ink for continuous and efficient solar-driven seawater desalination DOI
Zhiheng Zheng, Huan Liu, Xiaodong Wang

et al.

Desalination, Journal Year: 2024, Volume and Issue: 574, P. 117276 - 117276

Published: Jan. 2, 2024

Language: Английский

Citations

38

Biomass-MOF composites in wastewater treatment, air purification, and electromagnetic radiation adsorption – A review DOI

Jinxuan Jiang,

Yang Shi,

Mingjun Wu

et al.

Chemical Engineering Journal, Journal Year: 2024, Volume and Issue: 494, P. 152932 - 152932

Published: June 7, 2024

Language: Английский

Citations

28

Current Developments in Chitosan‐Based Hydrogels for Water and Wastewater Treatment: A Comprehensive Review DOI Open Access

Ziao Zhang,

Yujie Lu,

Yiman Zhao

et al.

ChemistrySelect, Journal Year: 2025, Volume and Issue: 10(6)

Published: Feb. 1, 2025

Abstract The global shortage of fresh water is a critical issue, especially in regions with limited rainfall. Developing reliable and wastewater treatment technologies urgent. Among the available methods, adsorption stands out as highly effective, straightforward, cost‐efficient approach. It avoids use additional chemicals reduces risk contaminating source undesirable by‐products. Chitosan (CS)‐based hydrogels have gained attention for their excellent capacities pollutants water. These materials are also known bioavailability, biocompatibility, biodegradability, cost‐effectiveness, environmental friendliness, making them promising candidates treatment. This comprehensive review explores recent advancements CS‐based various applications, including pollutant removal, oil‐water separation, seawater desalination, atmospheric condensation. highlights benefits this material treatment, providing broader understanding potential research community. focuses on synthesis modification techniques these hydrogels, such cross‐linking, grafting, ion imprinting, which significantly enhance performance mechanical stability. Additionally, challenges faced by practical applications discussed, along solutions. paper concludes forecasting future directions field, offering valuable insights researchers. Overall, provides overview current state art into effective utilization emphasizing to address pollution challenges.

Language: Английский

Citations

3

Recyclable physical hydrogels as durable and efficient solar-driven evaporators DOI

Honglang Lu,

Min Li,

Xiaoyu Wang

et al.

Chemical Engineering Journal, Journal Year: 2022, Volume and Issue: 450, P. 138257 - 138257

Published: July 22, 2022

Language: Английский

Citations

49

Enhanced light trapping effect of hierarchical structure assembled from flower-like cobalt tetroxide and 3D-printed structure for efficient solar evaporation DOI

Tianyang Cui,

Wei Cai, Fukai Chu

et al.

Chemical Engineering Journal, Journal Year: 2022, Volume and Issue: 451, P. 139102 - 139102

Published: Sept. 8, 2022

Language: Английский

Citations

41