Layered oxyiodide CdBiO2I: An efficient visible light responsive and scalable photocatalyst DOI Creative Commons

Weishan Zheng,

Zijian Zhu,

Rui Sha

et al.

Journal of Materiomics, Journal Year: 2024, Volume and Issue: unknown, P. 100928 - 100928

Published: Aug. 1, 2024

Developing high-performance visible-light driven photocatalyst (λ≥420 nm) makes significance for the efficient utilization of solar energy. Mass production and easy recycling are equally important practical application powdery photocatalyst. However, it is challenging to meet above requirements at same time. In this work, we develop an responsive layered oxyiodide CdBiO2I nanosheets prepared by a facile direct precipitation method ambient atmosphere, demonstrate its upgradable features well fitting potential application. has crystal structure consisting [CdBiO2]+ layer I– single layer, differing from that BiOI composed [BiO2]2+ I- double layers. It displays absorption edge 520 nm in visible region, with band gap 2.52 eV. large intrinsic effective mass difference hole/electron, exceeding 8-fold, which results much higher charge separation efficiency more reactive species (superoxide radicals holes). The degradation tetracycline hydrochloride reaches 84% under light irradiation within 1 h, rate 10 times BiOI. addition, (12 g catalyst one time) immobilization onto porous polyurethane foam powder also demonstrated, indicates scalable properties recovery catalyst, highlighting advantages current preparation prefiguring applications. This work may enlighten future research on exploitation solar-driven high strong applicability.

Language: Английский

Harvesting the Vibration Energy of CdS for High‐Efficient Piezo‐Photocatalysis Removal of U(VI): Roles of Shape Dependent and Piezoelectric Polarization DOI Creative Commons

Zhimin Dong,

Donglin Gao,

Zifan Li

et al.

Energy & environment materials, Journal Year: 2024, Volume and Issue: 7(5)

Published: Jan. 22, 2024

Piezo‐photocatalysis could coalesce the advantages of mechanical vibration and solar energy perfectly to achieve high‐efficiency catalytic activity. Herein, quintessential piezoelectric material CdS nanowires with different aspect ratios are precisely constructed applied for piezo‐photocatalytic reduction U(VI) first time. The ultrasonic (60 kHz, 100 W) induces potential generate a 0.57 eV A −1 electric field, which is added direction (010) as driving force efficiently separate photogenerated charges. alliance between effect photocatalytic activity endows NW‐3 fastest rate under 5 W LED irradiation, relevant constant (0.042 min ) about 12 53.8 times than that ultrasonication. More importantly, 93.74% be removed from natural uranium mine wastewater. Therefore, this piezo‐photocatalysis system reduces easily separable (UO 2 )O ·2H O(s) provides valuable input disposal applications radioactive wastewater broadens horizons nuclear utilization toward advancement carbon neutrality.

Language: Английский

Citations

20

Boosting tetracycline degradation of BaTiO3-based piezo-catalysts via modulating phase boundary and band structure DOI

Runtian Xu,

Zhiyong Liu, Bing Xie

et al.

Journal of Colloid and Interface Science, Journal Year: 2024, Volume and Issue: 665, P. 888 - 897

Published: March 30, 2024

Language: Английский

Citations

19

Selective removal of antibiotics over MgAl2O4/C3N4/YMnO3 photocatalysts: Performance prediction and mechanism insight DOI Open Access
Maoyuan Li, Shifa Wang, Huajing Gao

et al.

Journal of the American Ceramic Society, Journal Year: 2022, Volume and Issue: 106(4), P. 2420 - 2442

Published: Dec. 15, 2022

Abstract A simple polyacrylamide gel method combined with low temperature sintering technology has been used to synthesize the C–O functional groups grafted MgAl 2 O 4 /C 3 N /YMnO (MAO–CN–YMO) heterojunction photocatalysts enhanced visible‐light‐induced photodegradation toward oxytetracycline hydrochloride (OTC‐HCl). variety of characterization methods are gain insight into phase purity, crystal structure, microstructure, group information, elemental composition, surface defect, light response capability, and photocatalytic activity as‐synthesized samples. The influences mass ratios m CN / YMO , MAO /( + ) in CN–YMO, CN–MAO, MAO–CN–YMO on for degradation OTC‐HCl was also discussed, optimal ratio is identified as 15 wt%. experiments confirmed that had high selectivity antibiotics. prediction made by a intelligent algorithm models. results whale optimization highly consistent experimental results. Combined energy band theory high‐performance liquid chromatography–tandem spectrometry, free radicals reaction solution preferentially attacked –CH –NCH –OH during heterostructure photocatalysts, then attack –C=O –C=O–NH finally perform ring‐opening degrade nontoxic harmless products small molecules such CO H O, NH . This work provides new idea development novel double p–n junction antibiotic multiple algorithms.

Language: Английский

Citations

45

Preparation of magnetic N-doped iron sludge based biochar and its potential for persulfate activation and tetracycline degradation DOI
Huiping Zeng,

Jianxue Li,

Jiaxin Xu

et al.

Journal of Cleaner Production, Journal Year: 2022, Volume and Issue: 378, P. 134519 - 134519

Published: Oct. 10, 2022

Language: Английский

Citations

43

Photo-/electro-/piezo-catalytic elimination of environmental pollutants DOI
Sufei Wang, Yang Li, Qing Liu

et al.

Journal of Photochemistry and Photobiology A Chemistry, Journal Year: 2022, Volume and Issue: 437, P. 114435 - 114435

Published: Nov. 24, 2022

Language: Английский

Citations

38

Progress in defect engineering strategies to enhance piezoelectric catalysis for efficient water treatment and energy regeneration DOI Open Access

Hongpu Shi,

Yanan Liu,

Yubin Bai

et al.

Separation and Purification Technology, Journal Year: 2023, Volume and Issue: 330, P. 125247 - 125247

Published: Oct. 5, 2023

Language: Английский

Citations

37

Piezoelectric materials: Advanced applications in electro-chemical processes DOI Creative Commons

Hamna Shaukat,

Ahsan Ali, Saira Bibi

et al.

Energy Reports, Journal Year: 2023, Volume and Issue: 9, P. 4306 - 4324

Published: March 22, 2023

This review article provides a detailed overview of the advanced applications piezoelectric material in electrochemical processes. Energy harvesting, potential topic, aims to transform ambient energy sources, including heat, light, and mechanical motion, into useful that would otherwise be wasted. focuses on an innovative developing field intends connect-directly energy-harvesting devices materials systems. To regulate processes presence materials, reactions are dominantly influenced by produced electric charge under stress. In detail, electrochemistry involved for dye degradation, hydrogen production, self-charging power cells, nanogenerator water splitting is discussed umbrella piezocatalysis. A very focused data presented piezo hybrid systems from future perspective current enhancement induced internal effect also highlighted.

Language: Английский

Citations

36

Molecular oxygen activation: Innovative techniques for environmental remediation DOI
Lili Zhou, Yuting Liu,

Hao Shi

et al.

Water Research, Journal Year: 2023, Volume and Issue: 250, P. 121075 - 121075

Published: Dec. 27, 2023

Language: Английский

Citations

30

A one-step soft-template hydrothermal preparation and piezoelectric catalytic activity of flowers-like Co-doped MoS2 microspheres DOI

Minghu Shen,

Binghua Yao,

Wen Zhang

et al.

Journal of Alloys and Compounds, Journal Year: 2023, Volume and Issue: 945, P. 169328 - 169328

Published: Feb. 20, 2023

Language: Английский

Citations

26

Piezoelectric polarization and interfacial electric field synergistically promote piezo-photocatalysis of in-situ transformed heterojunction DOI
Tong Li, Cheng Hu, Haitao Li

et al.

Applied Surface Science, Journal Year: 2023, Volume and Issue: 630, P. 157478 - 157478

Published: May 9, 2023

Language: Английский

Citations

23