International Journal of Hydrogen Energy, Journal Year: 2022, Volume and Issue: 47(91), P. 38533 - 38555
Published: Sept. 27, 2022
Language: Английский
Advanced Energy Materials, Journal Year: 2025, Volume and Issue: unknown
Published: Jan. 8, 2025
Abstract The escalating crisis of oceanic plastic pollution demands innovative and effective strategies for resolution. Photocatalysis offers a sustainable, green, energy‐efficient approach the upcycling waste into fuels value‐added chemicals. In this study, an atomically engineered GeS NS/ZnIn₂S₄ photocatalyst is employed to directly transform raw polyethylene terephthalate (PET), ubiquitous plastic, variety organic chemicals (13 917 µmol g⁻¹) using Earth's most abundant resources: sunlight, seawater, air. Advanced ex situ in characterization analyses reveal that sulfur vacancies (Vs) electrolyte‐assisted polarization effect seawater play crucial roles trapping photogenerated electrons accelerating charge carrier separation, respectively. These effects significantly enhance photocatalytic efficiency improve oxidative reactions. This research introduces methodology accounts real‐world conditions upcycling, utilizing natural resources paving way further exploration area.
Language: Английский
Citations
2
Chemical Engineering Journal, Journal Year: 2022, Volume and Issue: 453, P. 139957 - 139957
Published: Oct. 22, 2022
Language: Английский
Citations
62
Applied Catalysis B Environment and Energy, Journal Year: 2023, Volume and Issue: 339, P. 123103 - 123103
Published: July 27, 2023
Language: Английский
Citations
40
Journal of Colloid and Interface Science, Journal Year: 2023, Volume and Issue: 653, P. 1650 - 1661
Published: Oct. 4, 2023
Language: Английский
Citations
39
International Journal of Hydrogen Energy, Journal Year: 2023, Volume and Issue: 48(33), P. 12257 - 12287
Published: Jan. 4, 2023
Language: Английский
Citations
30
Small, Journal Year: 2023, Volume and Issue: 20(2)
Published: Sept. 5, 2023
Abstract Cyano‐rich g‐C 3 N 4 materials are widely used in various fields of photochemistry due to the very powerful electron‐absorbing ability and electron storage function cyano, as well its advantages improving light absorption, adjusting energy band structure, increasing polarization rate density active site concentration, promoting oxygen activation ability. Notwithstanding, there is yet a huge knowledge break design, preparation, detection, application, prospect cyano‐rich . Accordingly, an overall review arranged substantially comprehend research progress position materials. An overview current synthesis, characterization (determination their location quantity), reaction mechanism analysis provide quantity novel suggestions for cyano‐modified carbon nitride materials' construction provided. In view prevailing challenges outlooks materials, this paper will purify growth direction , achieve more in‐depth exploration broaden applications
Language: Английский
Citations
27
ACS Applied Nano Materials, Journal Year: 2023, Volume and Issue: 6(5), P. 3927 - 3935
Published: Feb. 27, 2023
How to realize on-site small-scale production and sustainable consumption of H2O2 is the focus attention this study. Photocatalysis technology can just meet demand, g-C3N4 one most popular catalysts employed. However, numerous defects in nanostructure seriously inhibit its catalytic activity, which act as recombination centers photogenerated carriers. Herein, we propose an anti-defect engineering strategy tailor a highly crystalline for efficient photocatalytic situ production, be further cascaded wastewater remediation. High-resolution transmission electron microscopy spin-resonance spectroscopy results demonstrate that successfully fabricated with extremely low defect concentrations. Transient surface photovoltage data shows exhibits rapid charge separation transfer slow decay. Therefore, activity significantly promoted by eliminating construct structure. Especially, prepared thiourea (CNT) maximum 2.48 mmol g–1 h–1 apparent quantum efficiency 22% (λ = 400 nm), along excellent cascade tetracycline removal effect. This work provides regulate crystal structure catalyst enhanced activity.
Language: Английский
Citations
25
Journal of Colloid and Interface Science, Journal Year: 2023, Volume and Issue: 637, P. 465 - 476
Published: Jan. 26, 2023
Language: Английский
Citations
24
Small, Journal Year: 2024, Volume and Issue: 20(26)
Published: Jan. 14, 2024
Abstract Featured with the attractive properties such as large surface area, unique atomic layer thickness, excellent electronic conductivity, and superior catalytic activity, layered metal chalcogenides (LMCs) have received considerable research attention in electrocatalytic applications. In this review, approaches developed to synthesize LMCs‐based electrocatalysts are summarized. Recent progress composites for electrochemical energy conversion applications including oxygen reduction reaction, carbon dioxide evolution hydrogen overall water splitting, nitrogen reaction is reviewed, potential opportunities practical obstacles development of high‐performing active substances also discussed. This review may provide an inspiring guidance developing high‐performance LMCs
Language: Английский
Citations
12
International Journal of Hydrogen Energy, Journal Year: 2024, Volume and Issue: 85, P. 598 - 624
Published: Aug. 28, 2024
Language: Английский
Citations
12